Ultrahigh‑Q Lead Halide Perovskite Microlasers

Lead halide perovskites have been promising platforms for micro- and nanolasers. However, the fragile nature of perovskites poses an extreme challenge to engineering a cavity boundary and achieving high-quality (Q) modes, severely hindering their practical applications. Here, we combine an etchless...

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Veröffentlicht in:Nano letters 2023-04, Vol.23 (8), p.3418-3425
Hauptverfasser: Tang, Haijun, Wang, Yuhan, Chen, Yimu, Wang, Kaiyang, He, Xianxiong, Huang, Can, Xiao, Shumin, Yu, Shaohua, Song, Qinghai
Format: Artikel
Sprache:eng
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Zusammenfassung:Lead halide perovskites have been promising platforms for micro- and nanolasers. However, the fragile nature of perovskites poses an extreme challenge to engineering a cavity boundary and achieving high-quality (Q) modes, severely hindering their practical applications. Here, we combine an etchless bound state in the continuum (BIC) and a chemically synthesized single-crystalline CsPbBr3 microplate to demonstrate on-chip integrated perovskite microlasers with ultrahigh Q factors. By pattering polymer microdisks on CsPbBr3 microplates, we show that record high-Q BIC modes can be formed by destructive interference between different in-plane radiation from whispering gallery modes. Consequently, a record high Q-factor of 1.04 × 105 was achieved in our experiment. The high repeatability and high controllability of such ultrahigh Q BIC microlasers have also been experimentally confirmed. This research provides a new paradigm for perovskite nanophotonics.
ISSN:1530-6984
1530-6992
DOI:10.1021/acs.nanolett.3c00463