Effective adsorptive removal of sulfamethoxazole (SMX) from aqueous solution by ZIF-8 derived adsorbent ZC-0.5
Efficient removal of antibiotics from the aquatic environment is urgently needed due to their obstinate accumulation and non-biodegradability. In this study, a mesoporous carbon material (ZC-0.5) was successfully synthesized for the adsorption of sulfamethoxazole (SMX), one of the major antibiotics...
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| Veröffentlicht in: | Environmental science and pollution research international 2023-05, Vol.30 (21), p.60704-60716 |
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| creator | Zhang, Nizi Tang, Chenliu Bi, Weixia Sun, Zhirong Hu, Xiang |
| description | Efficient removal of antibiotics from the aquatic environment is urgently needed due to their obstinate accumulation and non-biodegradability. In this study, a mesoporous carbon material (ZC-0.5) was successfully synthesized for the adsorption of sulfamethoxazole (SMX), one of the major antibiotics for the treatment of human and animal infections. ZIF-8 as the precursor of ZC-0.5, specifically, using cetyl trimethyl ammonium bromide (CTAB) and sodium laurate (SL) as dual templates and carbonizing at 800 ℃. This novel adsorbent exhibited a high proportion of mesopore (75.64%) and a large specific surface area (1459.73 m
2
·g
−1
). The adsorption experiment examined the reusability of ZC-0.5 and that it could retain superior maximum adsorption capacities (167.45 mg∙L
−1
) after five cycles of adsorption and desorption. The adsorption process satisfied the pseudo-second-order kinetic (PSO) and mixed first- and second-order kinetic (MOE). It also satisfied the Freundlich and Sips isotherm models. Moreover, thermodynamic calculation indicated the adsorption process was spontaneous, endothermal, and entropy-increasing. Furthermore, plausible adsorption mechanisms were explained through van der Waals force, electrostatic interaction, hydrophobic force, π-π interaction, and hydrogen bond. This work offers a new efficient adsorbent for antibiotic elimination. |
| doi_str_mv | 10.1007/s11356-023-26588-z |
| format | Article |
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2
·g
−1
). The adsorption experiment examined the reusability of ZC-0.5 and that it could retain superior maximum adsorption capacities (167.45 mg∙L
−1
) after five cycles of adsorption and desorption. The adsorption process satisfied the pseudo-second-order kinetic (PSO) and mixed first- and second-order kinetic (MOE). It also satisfied the Freundlich and Sips isotherm models. Moreover, thermodynamic calculation indicated the adsorption process was spontaneous, endothermal, and entropy-increasing. Furthermore, plausible adsorption mechanisms were explained through van der Waals force, electrostatic interaction, hydrophobic force, π-π interaction, and hydrogen bond. This work offers a new efficient adsorbent for antibiotic elimination.</description><identifier>ISSN: 1614-7499</identifier><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-023-26588-z</identifier><identifier>PMID: 37041353</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorbents ; Adsorption ; Adsorptivity ; Ammonium ; Anti-Bacterial Agents - chemistry ; Antibiotics ; Aquatic environment ; Aquatic Pollution ; Aqueous solutions ; Atmospheric Protection/Air Quality Control/Air Pollution ; Biodegradability ; Biodegradation ; carbon ; Cetyltrimethylammonium bromide ; desorption ; Earth and Environmental Science ; Ecotoxicology ; Electrostatic properties ; Entropy ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Humans ; hydrogen bonding ; Hydrogen bonds ; Hydrogen-Ion Concentration ; Hydrophobicity ; Kinetics ; Lauric acid ; porous media ; Research Article ; sodium ; Sulfamethoxazole ; Sulfamethoxazole - chemistry ; surface area ; Thermodynamics ; Van der Waals forces ; Waste Water Technology ; Water ; Water Management ; Water Pollutants, Chemical - analysis ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2023-05, Vol.30 (21), p.60704-60716</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><rights>2023. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c408t-5fda78d5b25ce83f25e56f18e9a0f15d5252dbe6c0e35e739b831c80307c2c363</citedby><cites>FETCH-LOGICAL-c408t-5fda78d5b25ce83f25e56f18e9a0f15d5252dbe6c0e35e739b831c80307c2c363</cites><orcidid>0000-0003-4699-7136</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-023-26588-z$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-023-26588-z$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27903,27904,41467,42536,51297</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/37041353$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhang, Nizi</creatorcontrib><creatorcontrib>Tang, Chenliu</creatorcontrib><creatorcontrib>Bi, Weixia</creatorcontrib><creatorcontrib>Sun, Zhirong</creatorcontrib><creatorcontrib>Hu, Xiang</creatorcontrib><title>Effective adsorptive removal of sulfamethoxazole (SMX) from aqueous solution by ZIF-8 derived adsorbent ZC-0.5</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Efficient removal of antibiotics from the aquatic environment is urgently needed due to their obstinate accumulation and non-biodegradability. In this study, a mesoporous carbon material (ZC-0.5) was successfully synthesized for the adsorption of sulfamethoxazole (SMX), one of the major antibiotics for the treatment of human and animal infections. ZIF-8 as the precursor of ZC-0.5, specifically, using cetyl trimethyl ammonium bromide (CTAB) and sodium laurate (SL) as dual templates and carbonizing at 800 ℃. This novel adsorbent exhibited a high proportion of mesopore (75.64%) and a large specific surface area (1459.73 m
2
·g
−1
). The adsorption experiment examined the reusability of ZC-0.5 and that it could retain superior maximum adsorption capacities (167.45 mg∙L
−1
) after five cycles of adsorption and desorption. The adsorption process satisfied the pseudo-second-order kinetic (PSO) and mixed first- and second-order kinetic (MOE). It also satisfied the Freundlich and Sips isotherm models. Moreover, thermodynamic calculation indicated the adsorption process was spontaneous, endothermal, and entropy-increasing. Furthermore, plausible adsorption mechanisms were explained through van der Waals force, electrostatic interaction, hydrophobic force, π-π interaction, and hydrogen bond. This work offers a new efficient adsorbent for antibiotic elimination.</description><subject>Adsorbents</subject><subject>Adsorption</subject><subject>Adsorptivity</subject><subject>Ammonium</subject><subject>Anti-Bacterial Agents - chemistry</subject><subject>Antibiotics</subject><subject>Aquatic environment</subject><subject>Aquatic Pollution</subject><subject>Aqueous solutions</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Biodegradability</subject><subject>Biodegradation</subject><subject>carbon</subject><subject>Cetyltrimethylammonium bromide</subject><subject>desorption</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Electrostatic properties</subject><subject>Entropy</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Humans</subject><subject>hydrogen bonding</subject><subject>Hydrogen bonds</subject><subject>Hydrogen-Ion Concentration</subject><subject>Hydrophobicity</subject><subject>Kinetics</subject><subject>Lauric acid</subject><subject>porous media</subject><subject>Research Article</subject><subject>sodium</subject><subject>Sulfamethoxazole</subject><subject>Sulfamethoxazole - chemistry</subject><subject>surface area</subject><subject>Thermodynamics</subject><subject>Van der Waals forces</subject><subject>Waste Water Technology</subject><subject>Water</subject><subject>Water Management</subject><subject>Water Pollutants, Chemical - analysis</subject><subject>Water Pollution Control</subject><issn>1614-7499</issn><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNqFkcFuFSEUhonR2Fp9AReGxE1dUA8wMMzS3LTapKaLamK6IQxz0NvMDFeYadr79OV2qjUudMVJ-P6PQ35CXnM44gD1-8y5VJqBkExoZQzbPiH7XPOK1VXTPP1j3iMvcr4CENCI-jnZkzVUJSv3yXgcAvppfY3UdTmmzf2YcIjXrqcx0Dz3wQ04_Yg3bht7pIcXn7-9oyHFgbqfM8Y50xz7eVrHkba39PL0hBnaYSqebnG2OE70csXgSL0kz4LrM756OA_I15PjL6tP7Oz84-nqwxnzFZiJqdC52nSqFcqjkUEoVDpwg42DwFWnhBJdi9oDSoW1bFojuTcgofbCSy0PyOHi3aRYlsyTHdbZY9-7cbexlVxJrqtKwX9RYQB4pTXwgr79C72KcxrLR3ZU0xjBq51QLJRPMeeEwW7SenDp1nKwu-LsUpwtxdn74uy2hN48qOd2wO535FdTBZALkMvV-B3T49v_0N4B8u2imA</recordid><startdate>20230501</startdate><enddate>20230501</enddate><creator>Zhang, Nizi</creator><creator>Tang, Chenliu</creator><creator>Bi, Weixia</creator><creator>Sun, Zhirong</creator><creator>Hu, Xiang</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QL</scope><scope>7SN</scope><scope>7T7</scope><scope>7TV</scope><scope>7U7</scope><scope>7WY</scope><scope>7WZ</scope><scope>7X7</scope><scope>7XB</scope><scope>87Z</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8FL</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BEZIV</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FRNLG</scope><scope>FYUFA</scope><scope>F~G</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K60</scope><scope>K6~</scope><scope>K9.</scope><scope>L.-</scope><scope>M0C</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7N</scope><scope>P64</scope><scope>PATMY</scope><scope>PQBIZ</scope><scope>PQBZA</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>7X8</scope><scope>7S9</scope><scope>L.6</scope><orcidid>https://orcid.org/0000-0003-4699-7136</orcidid></search><sort><creationdate>20230501</creationdate><title>Effective adsorptive removal of sulfamethoxazole (SMX) from aqueous solution by ZIF-8 derived adsorbent ZC-0.5</title><author>Zhang, Nizi ; Tang, Chenliu ; Bi, Weixia ; Sun, Zhirong ; Hu, Xiang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c408t-5fda78d5b25ce83f25e56f18e9a0f15d5252dbe6c0e35e739b831c80307c2c363</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Adsorbents</topic><topic>Adsorption</topic><topic>Adsorptivity</topic><topic>Ammonium</topic><topic>Anti-Bacterial Agents - 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Academic</collection><collection>AGRICOLA</collection><collection>AGRICOLA - Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhang, Nizi</au><au>Tang, Chenliu</au><au>Bi, Weixia</au><au>Sun, Zhirong</au><au>Hu, Xiang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effective adsorptive removal of sulfamethoxazole (SMX) from aqueous solution by ZIF-8 derived adsorbent ZC-0.5</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2023-05-01</date><risdate>2023</risdate><volume>30</volume><issue>21</issue><spage>60704</spage><epage>60716</epage><pages>60704-60716</pages><issn>1614-7499</issn><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Efficient removal of antibiotics from the aquatic environment is urgently needed due to their obstinate accumulation and non-biodegradability. In this study, a mesoporous carbon material (ZC-0.5) was successfully synthesized for the adsorption of sulfamethoxazole (SMX), one of the major antibiotics for the treatment of human and animal infections. ZIF-8 as the precursor of ZC-0.5, specifically, using cetyl trimethyl ammonium bromide (CTAB) and sodium laurate (SL) as dual templates and carbonizing at 800 ℃. This novel adsorbent exhibited a high proportion of mesopore (75.64%) and a large specific surface area (1459.73 m
2
·g
−1
). The adsorption experiment examined the reusability of ZC-0.5 and that it could retain superior maximum adsorption capacities (167.45 mg∙L
−1
) after five cycles of adsorption and desorption. The adsorption process satisfied the pseudo-second-order kinetic (PSO) and mixed first- and second-order kinetic (MOE). It also satisfied the Freundlich and Sips isotherm models. Moreover, thermodynamic calculation indicated the adsorption process was spontaneous, endothermal, and entropy-increasing. Furthermore, plausible adsorption mechanisms were explained through van der Waals force, electrostatic interaction, hydrophobic force, π-π interaction, and hydrogen bond. This work offers a new efficient adsorbent for antibiotic elimination.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>37041353</pmid><doi>10.1007/s11356-023-26588-z</doi><tpages>13</tpages><orcidid>https://orcid.org/0000-0003-4699-7136</orcidid></addata></record> |
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| ispartof | Environmental science and pollution research international, 2023-05, Vol.30 (21), p.60704-60716 |
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| subjects | Adsorbents Adsorption Adsorptivity Ammonium Anti-Bacterial Agents - chemistry Antibiotics Aquatic environment Aquatic Pollution Aqueous solutions Atmospheric Protection/Air Quality Control/Air Pollution Biodegradability Biodegradation carbon Cetyltrimethylammonium bromide desorption Earth and Environmental Science Ecotoxicology Electrostatic properties Entropy Environment Environmental Chemistry Environmental Health Environmental science Humans hydrogen bonding Hydrogen bonds Hydrogen-Ion Concentration Hydrophobicity Kinetics Lauric acid porous media Research Article sodium Sulfamethoxazole Sulfamethoxazole - chemistry surface area Thermodynamics Van der Waals forces Waste Water Technology Water Water Management Water Pollutants, Chemical - analysis Water Pollution Control |
| title | Effective adsorptive removal of sulfamethoxazole (SMX) from aqueous solution by ZIF-8 derived adsorbent ZC-0.5 |
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