K-dependent exchange interaction of quadrupole excitons in Cu2O

The long‐ and short‐range exchange interaction for the quadrupole allowed transition to the yellow 1S orthoexciton in Cu2O is derived. While the three orthoexciton states still remain degenerate, when treating the exchange up to the order of K‐linear terms, a fine structure arises when K‐quadratic t...

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Veröffentlicht in:Phys. Status Solidi (b). Vol. 238, no. 3, pp. 541-547. 2003 no. 3, pp. 541-547. 2003, 2003-08, Vol.238 (3), p.541-547
Hauptverfasser: Dasbach, G., Fröhlich, D., Stolz, H., Klieber, R., Suter, D., Bayer, M.
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container_end_page 547
container_issue 3
container_start_page 541
container_title Phys. Status Solidi (b). Vol. 238, no. 3, pp. 541-547. 2003
container_volume 238
creator Dasbach, G.
Fröhlich, D.
Stolz, H.
Klieber, R.
Suter, D.
Bayer, M.
description The long‐ and short‐range exchange interaction for the quadrupole allowed transition to the yellow 1S orthoexciton in Cu2O is derived. While the three orthoexciton states still remain degenerate, when treating the exchange up to the order of K‐linear terms, a fine structure arises when K‐quadratic terms are included. This splitting is investigated experimentally by high resolution spectroscopy. Exchange contributions of few μeV are resolved and compared to theory. The impact of strain on the exciton fine structure is discussed and evaluated.
doi_str_mv 10.1002/pssb.200303186
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subjects 71.35.Cc
78.20.-e
78.40.Fy
Condensed matter: electronic structure, electrical, magnetic, and optical properties
Electron states
Exact sciences and technology
Excitons and related phenomena
Intrinsic properties of excitons
optical absorption spectra
Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation
Physics
Time-resolved optical spectroscopies and other ultrafast optical measurements in condensed matter
title K-dependent exchange interaction of quadrupole excitons in Cu2O
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