Hyperbolic whispering-gallery phonon polaritons in boron nitride nanotubes
Light confinement in nanostructures produces an enhanced light–matter interaction that enables a vast range of applications including single-photon sources, nanolasers and nanosensors. In particular, nanocavity-confined polaritons display a strongly enhanced light–matter interaction in the infrared...
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| Veröffentlicht in: | Nature nanotechnology 2023-05, Vol.18 (5), p.529-534 |
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| creator | Guo, Xiangdong Li, Ning Yang, Xiaoxia Qi, Ruishi Wu, Chenchen Shi, Ruochen Li, Yuehui Huang, Yang García de Abajo, F. Javier Wang, En-Ge Gao, Peng Dai, Qing |
| description | Light confinement in nanostructures produces an enhanced light–matter interaction that enables a vast range of applications including single-photon sources, nanolasers and nanosensors. In particular, nanocavity-confined polaritons display a strongly enhanced light–matter interaction in the infrared regime. This interaction could be further boosted if polaritonic modes were moulded to form whispering-gallery modes; but scattering losses within nanocavities have so far prevented their observation. Here, we show that hexagonal BN nanotubes act as an atomically smooth nanocavity that can sustain phonon-polariton whispering-gallery modes, owing to their intrinsic hyperbolic dispersion and low scattering losses. Hyperbolic whispering-gallery phonon polaritons on BN nanotubes of ～4 nm radius (sidewall of six atomic layers) are characterized by an ultrasmall nanocavity mode volume (
V
m
≈ 10
–10
λ
0
3
at an optical wavelength
λ
0
≈ 6.4 μm) and a Purcell factor (
Q
/
V
m
) as high as 10
12
. We posit that BN nanotubes could become an important material platform for the realization of one-dimensional, ultrastrong light–matter interactions, with exciting implications for compact photonic devices.
A Purcell factor as high as 10
12
is measured in atomically smooth nanocavities of hexagonal boron nitride nanotubes. |
| doi_str_mv | 10.1038/s41565-023-01324-3 |
| format | Article |
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V
m
≈ 10
–10
λ
0
3
at an optical wavelength
λ
0
≈ 6.4 μm) and a Purcell factor (
Q
/
V
m
) as high as 10
12
. We posit that BN nanotubes could become an important material platform for the realization of one-dimensional, ultrastrong light–matter interactions, with exciting implications for compact photonic devices.
A Purcell factor as high as 10
12
is measured in atomically smooth nanocavities of hexagonal boron nitride nanotubes.</description><identifier>ISSN: 1748-3387</identifier><identifier>EISSN: 1748-3395</identifier><identifier>DOI: 10.1038/s41565-023-01324-3</identifier><identifier>PMID: 36823369</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/301/930/12 ; 639/624/399/1098 ; 639/624/400/2797 ; 639/925/357/1018 ; Atomic radius ; Boron ; Boron nitride ; Chemistry and Materials Science ; Interdisciplinary aspects ; Laboratories ; Light ; Materials Science ; Microscopy ; Nanosensors ; Nanotechnology ; Nanotechnology and Microengineering ; Nanotubes ; Phonons ; Physics ; Polaritons ; Scattering ; Spectrum analysis</subject><ispartof>Nature nanotechnology, 2023-05, Vol.18 (5), p.529-534</ispartof><rights>The Author(s), under exclusive licence to Springer Nature Limited 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><rights>2023. The Author(s), under exclusive licence to Springer Nature Limited.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c375t-7688cd9186fca25ed388c899093af61df7051cb01882366879fa92486da042673</citedby><cites>FETCH-LOGICAL-c375t-7688cd9186fca25ed388c899093af61df7051cb01882366879fa92486da042673</cites><orcidid>0000-0001-9868-2115 ; 0000-0002-1750-0867 ; 0000-0002-0670-053X ; 0000-0001-5624-5320 ; 0000-0002-4970-4565</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1038/s41565-023-01324-3$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1038/s41565-023-01324-3$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/36823369$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Guo, Xiangdong</creatorcontrib><creatorcontrib>Li, Ning</creatorcontrib><creatorcontrib>Yang, Xiaoxia</creatorcontrib><creatorcontrib>Qi, Ruishi</creatorcontrib><creatorcontrib>Wu, Chenchen</creatorcontrib><creatorcontrib>Shi, Ruochen</creatorcontrib><creatorcontrib>Li, Yuehui</creatorcontrib><creatorcontrib>Huang, Yang</creatorcontrib><creatorcontrib>García de Abajo, F. Javier</creatorcontrib><creatorcontrib>Wang, En-Ge</creatorcontrib><creatorcontrib>Gao, Peng</creatorcontrib><creatorcontrib>Dai, Qing</creatorcontrib><title>Hyperbolic whispering-gallery phonon polaritons in boron nitride nanotubes</title><title>Nature nanotechnology</title><addtitle>Nat. Nanotechnol</addtitle><addtitle>Nat Nanotechnol</addtitle><description>Light confinement in nanostructures produces an enhanced light–matter interaction that enables a vast range of applications including single-photon sources, nanolasers and nanosensors. In particular, nanocavity-confined polaritons display a strongly enhanced light–matter interaction in the infrared regime. This interaction could be further boosted if polaritonic modes were moulded to form whispering-gallery modes; but scattering losses within nanocavities have so far prevented their observation. Here, we show that hexagonal BN nanotubes act as an atomically smooth nanocavity that can sustain phonon-polariton whispering-gallery modes, owing to their intrinsic hyperbolic dispersion and low scattering losses. Hyperbolic whispering-gallery phonon polaritons on BN nanotubes of ～4 nm radius (sidewall of six atomic layers) are characterized by an ultrasmall nanocavity mode volume (
V
m
≈ 10
–10
λ
0
3
at an optical wavelength
λ
0
≈ 6.4 μm) and a Purcell factor (
Q
/
V
m
) as high as 10
12
. We posit that BN nanotubes could become an important material platform for the realization of one-dimensional, ultrastrong light–matter interactions, with exciting implications for compact photonic devices.
A Purcell factor as high as 10
12
is measured in atomically smooth nanocavities of hexagonal boron nitride nanotubes.</description><subject>639/301/930/12</subject><subject>639/624/399/1098</subject><subject>639/624/400/2797</subject><subject>639/925/357/1018</subject><subject>Atomic radius</subject><subject>Boron</subject><subject>Boron nitride</subject><subject>Chemistry and Materials Science</subject><subject>Interdisciplinary aspects</subject><subject>Laboratories</subject><subject>Light</subject><subject>Materials Science</subject><subject>Microscopy</subject><subject>Nanosensors</subject><subject>Nanotechnology</subject><subject>Nanotechnology and Microengineering</subject><subject>Nanotubes</subject><subject>Phonons</subject><subject>Physics</subject><subject>Polaritons</subject><subject>Scattering</subject><subject>Spectrum analysis</subject><issn>1748-3387</issn><issn>1748-3395</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp9kE9PwyAYh4nRuDn9Ah5MEy9eUP4UCkezqNMs8aJnQlu6sXRQoY3Zt5e5ORMPnuAlz_vjlweAS4xuMaLiLuaYcQYRoRBhSnJIj8AYF7mAlEp2fLiLYgTOYlwhxIgk-SkYUS4IpVyOwcts05lQ-tZW2efSxjRYt4AL3bYmbLJu6Z13WedbHWzvXcysy0of0puzfbC1yZx2vh9KE8_BSaPbaC725wS8Pz68TWdw_vr0PL2fw4oWrIcFF6KqJRa8qTRhpqZpFlIiSXXDcd0UiOGqRFikjpyLQjY6tRa81ignvKATcLPL7YL_GEzs1drGyrStdsYPUZFCIMTzFJDQ6z_oyg_BpXaKCMwET7ksUWRHVcHHGEyjumDXOmwURmprWu1Mq2RafZtWNC1d7aOHcm3qw8qP2gTQHRC7rVITfv_-J_YLB1CINQ</recordid><startdate>20230501</startdate><enddate>20230501</enddate><creator>Guo, Xiangdong</creator><creator>Li, Ning</creator><creator>Yang, Xiaoxia</creator><creator>Qi, Ruishi</creator><creator>Wu, Chenchen</creator><creator>Shi, Ruochen</creator><creator>Li, Yuehui</creator><creator>Huang, Yang</creator><creator>García de Abajo, F. 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Javier</au><au>Wang, En-Ge</au><au>Gao, Peng</au><au>Dai, Qing</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Hyperbolic whispering-gallery phonon polaritons in boron nitride nanotubes</atitle><jtitle>Nature nanotechnology</jtitle><stitle>Nat. Nanotechnol</stitle><addtitle>Nat Nanotechnol</addtitle><date>2023-05-01</date><risdate>2023</risdate><volume>18</volume><issue>5</issue><spage>529</spage><epage>534</epage><pages>529-534</pages><issn>1748-3387</issn><eissn>1748-3395</eissn><abstract>Light confinement in nanostructures produces an enhanced light–matter interaction that enables a vast range of applications including single-photon sources, nanolasers and nanosensors. In particular, nanocavity-confined polaritons display a strongly enhanced light–matter interaction in the infrared regime. This interaction could be further boosted if polaritonic modes were moulded to form whispering-gallery modes; but scattering losses within nanocavities have so far prevented their observation. Here, we show that hexagonal BN nanotubes act as an atomically smooth nanocavity that can sustain phonon-polariton whispering-gallery modes, owing to their intrinsic hyperbolic dispersion and low scattering losses. Hyperbolic whispering-gallery phonon polaritons on BN nanotubes of ～4 nm radius (sidewall of six atomic layers) are characterized by an ultrasmall nanocavity mode volume (
V
m
≈ 10
–10
λ
0
3
at an optical wavelength
λ
0
≈ 6.4 μm) and a Purcell factor (
Q
/
V
m
) as high as 10
12
. We posit that BN nanotubes could become an important material platform for the realization of one-dimensional, ultrastrong light–matter interactions, with exciting implications for compact photonic devices.
A Purcell factor as high as 10
12
is measured in atomically smooth nanocavities of hexagonal boron nitride nanotubes.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>36823369</pmid><doi>10.1038/s41565-023-01324-3</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0001-9868-2115</orcidid><orcidid>https://orcid.org/0000-0002-1750-0867</orcidid><orcidid>https://orcid.org/0000-0002-0670-053X</orcidid><orcidid>https://orcid.org/0000-0001-5624-5320</orcidid><orcidid>https://orcid.org/0000-0002-4970-4565</orcidid></addata></record> |
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| subjects | 639/301/930/12 639/624/399/1098 639/624/400/2797 639/925/357/1018 Atomic radius Boron Boron nitride Chemistry and Materials Science Interdisciplinary aspects Laboratories Light Materials Science Microscopy Nanosensors Nanotechnology Nanotechnology and Microengineering Nanotubes Phonons Physics Polaritons Scattering Spectrum analysis |
| title | Hyperbolic whispering-gallery phonon polaritons in boron nitride nanotubes |
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