Carbon nanotube-decorated hierarchical porous nickel/carbon hybrid derived from nickel-based metal-organic framework for enhanced methyl blue adsorption
[Display omitted] This work reports the incorporation of coordinated water into Ni-BTC nanorods (Ni-BTC-O) which induces their structural transformation to Ni-BTC nanofibres (Ni-BTC-F). The carbonization of the Ni-BTC nanofibres at 600 °C results in the formation of carbon nanotube (CNT)-decorated h...
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| Veröffentlicht in: | Journal of colloid and interface science 2023-05, Vol.638, p.220-230 |
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| creator | Cheng, Ping Wang, Xiaohan Markus, Josua Abdul Wahab, Md Chowdhury, Silvia Xin, Ruijing Alshehri, Saad M. Bando, Yoshio Yamauchi, Yusuke Kaneti, Yusuf Valentino |
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This work reports the incorporation of coordinated water into Ni-BTC nanorods (Ni-BTC-O) which induces their structural transformation to Ni-BTC nanofibres (Ni-BTC-F). The carbonization of the Ni-BTC nanofibres at 600 °C results in the formation of carbon nanotube (CNT)-decorated hierarchical porous nickel/carbon hybrid (labelled as Ni/C-600) with enlarged pores. In contrast, the Ni/C hybrid obtained from the carbonization of the original (unmodified) Ni-BTC nanorods (Ni-BTC-O) at 600 °C (labelled as Ni-BTC-O-600) exhibits smaller pore size and does not show the formation of CNTs. The Ni/C-600 hybrid derived from Ni-BTC-F shows a very high adsorption capacity of 686.8 mg g−1 toward methyl blue (MB) dye. This is approximately 4.8 times higher than the adsorption capacity of Ni-BTC-O-600 (144.1 mg g−1). The higher adsorption performance of Ni/C-600 relative to Ni-BTC-O-600 can be attributed to its larger pore volume, hierarchical porosity, and additional adsorption sites provided by the CNTs. In addition, the Ni/C-600 hybrid can maintain 90% of its adsorption capacity after 5 consecutive cycles, demonstrating its potential as an efficient and recyclable adsorbent for MB dye. |
| doi_str_mv | 10.1016/j.jcis.2023.01.075 |
| format | Article |
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This work reports the incorporation of coordinated water into Ni-BTC nanorods (Ni-BTC-O) which induces their structural transformation to Ni-BTC nanofibres (Ni-BTC-F). The carbonization of the Ni-BTC nanofibres at 600 °C results in the formation of carbon nanotube (CNT)-decorated hierarchical porous nickel/carbon hybrid (labelled as Ni/C-600) with enlarged pores. In contrast, the Ni/C hybrid obtained from the carbonization of the original (unmodified) Ni-BTC nanorods (Ni-BTC-O) at 600 °C (labelled as Ni-BTC-O-600) exhibits smaller pore size and does not show the formation of CNTs. The Ni/C-600 hybrid derived from Ni-BTC-F shows a very high adsorption capacity of 686.8 mg g−1 toward methyl blue (MB) dye. This is approximately 4.8 times higher than the adsorption capacity of Ni-BTC-O-600 (144.1 mg g−1). The higher adsorption performance of Ni/C-600 relative to Ni-BTC-O-600 can be attributed to its larger pore volume, hierarchical porosity, and additional adsorption sites provided by the CNTs. In addition, the Ni/C-600 hybrid can maintain 90% of its adsorption capacity after 5 consecutive cycles, demonstrating its potential as an efficient and recyclable adsorbent for MB dye.</description><identifier>ISSN: 0021-9797</identifier><identifier>EISSN: 1095-7103</identifier><identifier>DOI: 10.1016/j.jcis.2023.01.075</identifier><identifier>PMID: 36738545</identifier><language>eng</language><publisher>United States: Elsevier Inc</publisher><subject>adsorbents ; Adsorption ; carbon ; carbon nanotubes ; carbonization ; coordination polymers ; Dye removal ; dyes ; Hierarchical porous carbon ; Metal-organic frameworks ; nanofibers ; nanorods ; nickel ; porosity ; Wastewater treatment</subject><ispartof>Journal of colloid and interface science, 2023-05, Vol.638, p.220-230</ispartof><rights>2023 Elsevier Inc.</rights><rights>Copyright © 2023 Elsevier Inc. All rights reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c389t-f48000d0906f7c6f970517effbe7e617dcbdd11f26e99b010a3a7be58f322f603</citedby><cites>FETCH-LOGICAL-c389t-f48000d0906f7c6f970517effbe7e617dcbdd11f26e99b010a3a7be58f322f603</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0021979723000887$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3536,27903,27904,65309</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/36738545$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Cheng, Ping</creatorcontrib><creatorcontrib>Wang, Xiaohan</creatorcontrib><creatorcontrib>Markus, Josua</creatorcontrib><creatorcontrib>Abdul Wahab, Md</creatorcontrib><creatorcontrib>Chowdhury, Silvia</creatorcontrib><creatorcontrib>Xin, Ruijing</creatorcontrib><creatorcontrib>Alshehri, Saad M.</creatorcontrib><creatorcontrib>Bando, Yoshio</creatorcontrib><creatorcontrib>Yamauchi, Yusuke</creatorcontrib><creatorcontrib>Kaneti, Yusuf Valentino</creatorcontrib><title>Carbon nanotube-decorated hierarchical porous nickel/carbon hybrid derived from nickel-based metal-organic framework for enhanced methyl blue adsorption</title><title>Journal of colloid and interface science</title><addtitle>J Colloid Interface Sci</addtitle><description>[Display omitted]
This work reports the incorporation of coordinated water into Ni-BTC nanorods (Ni-BTC-O) which induces their structural transformation to Ni-BTC nanofibres (Ni-BTC-F). The carbonization of the Ni-BTC nanofibres at 600 °C results in the formation of carbon nanotube (CNT)-decorated hierarchical porous nickel/carbon hybrid (labelled as Ni/C-600) with enlarged pores. In contrast, the Ni/C hybrid obtained from the carbonization of the original (unmodified) Ni-BTC nanorods (Ni-BTC-O) at 600 °C (labelled as Ni-BTC-O-600) exhibits smaller pore size and does not show the formation of CNTs. The Ni/C-600 hybrid derived from Ni-BTC-F shows a very high adsorption capacity of 686.8 mg g−1 toward methyl blue (MB) dye. This is approximately 4.8 times higher than the adsorption capacity of Ni-BTC-O-600 (144.1 mg g−1). The higher adsorption performance of Ni/C-600 relative to Ni-BTC-O-600 can be attributed to its larger pore volume, hierarchical porosity, and additional adsorption sites provided by the CNTs. In addition, the Ni/C-600 hybrid can maintain 90% of its adsorption capacity after 5 consecutive cycles, demonstrating its potential as an efficient and recyclable adsorbent for MB dye.</description><subject>adsorbents</subject><subject>Adsorption</subject><subject>carbon</subject><subject>carbon nanotubes</subject><subject>carbonization</subject><subject>coordination polymers</subject><subject>Dye removal</subject><subject>dyes</subject><subject>Hierarchical porous carbon</subject><subject>Metal-organic frameworks</subject><subject>nanofibers</subject><subject>nanorods</subject><subject>nickel</subject><subject>porosity</subject><subject>Wastewater treatment</subject><issn>0021-9797</issn><issn>1095-7103</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNqFkcuO1DAQRS0EYnoGfoAFypJNMlVJJ25LbFBreEgjsYG15UeZuCeJGzuZUf8Jn4tbaVjCylL53CtVHcbeIFQI2N0eqoPxqaqhbirACnj7jG0QRFtyhOY52wDUWAou-BW7TukAgNi24iW7ajre7Nptu2G_9irqMBWTmsK8aCotmRDVTLboPUUVTe-NGopjiGFJxeTNAw23Zg31Jx29LSxF_5gDLobxQpRapTwZaVZDGeIPlcf5X430FOJD4UIsaOrVZFaoPw2FHhYqlE0hHmcfplfshVNDoteX94Z9_3j3bf-5vP_66cv-w31pmp2YS7fdAYAFAZ3jpnOCQ4ucnNPEqUNujbYW0dUdCaEBQTWKa2p3rqlr10Fzw96tvccYfi6UZjn6ZGgY1ER5Y1mLbQ1CAMf_o5w3iE2HbUbrFTUxpBTJyWP0o4oniSDP8uRBnuXJszwJKLO8HHp76V_0SPZv5I-tDLxfAcoHecx6ZDKezkf0kcwsbfD_6v8NTIWupw</recordid><startdate>20230515</startdate><enddate>20230515</enddate><creator>Cheng, Ping</creator><creator>Wang, Xiaohan</creator><creator>Markus, Josua</creator><creator>Abdul Wahab, Md</creator><creator>Chowdhury, Silvia</creator><creator>Xin, Ruijing</creator><creator>Alshehri, Saad M.</creator><creator>Bando, Yoshio</creator><creator>Yamauchi, Yusuke</creator><creator>Kaneti, Yusuf Valentino</creator><general>Elsevier Inc</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7S9</scope><scope>L.6</scope></search><sort><creationdate>20230515</creationdate><title>Carbon nanotube-decorated hierarchical porous nickel/carbon hybrid derived from nickel-based metal-organic framework for enhanced methyl blue adsorption</title><author>Cheng, Ping ; Wang, Xiaohan ; Markus, Josua ; Abdul Wahab, Md ; Chowdhury, Silvia ; Xin, Ruijing ; Alshehri, Saad M. ; Bando, Yoshio ; Yamauchi, Yusuke ; Kaneti, Yusuf Valentino</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c389t-f48000d0906f7c6f970517effbe7e617dcbdd11f26e99b010a3a7be58f322f603</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>adsorbents</topic><topic>Adsorption</topic><topic>carbon</topic><topic>carbon nanotubes</topic><topic>carbonization</topic><topic>coordination polymers</topic><topic>Dye removal</topic><topic>dyes</topic><topic>Hierarchical porous carbon</topic><topic>Metal-organic frameworks</topic><topic>nanofibers</topic><topic>nanorods</topic><topic>nickel</topic><topic>porosity</topic><topic>Wastewater treatment</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Cheng, Ping</creatorcontrib><creatorcontrib>Wang, Xiaohan</creatorcontrib><creatorcontrib>Markus, Josua</creatorcontrib><creatorcontrib>Abdul Wahab, Md</creatorcontrib><creatorcontrib>Chowdhury, Silvia</creatorcontrib><creatorcontrib>Xin, Ruijing</creatorcontrib><creatorcontrib>Alshehri, Saad M.</creatorcontrib><creatorcontrib>Bando, Yoshio</creatorcontrib><creatorcontrib>Yamauchi, Yusuke</creatorcontrib><creatorcontrib>Kaneti, Yusuf Valentino</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>AGRICOLA</collection><collection>AGRICOLA - Academic</collection><jtitle>Journal of colloid and interface science</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Cheng, Ping</au><au>Wang, Xiaohan</au><au>Markus, Josua</au><au>Abdul Wahab, Md</au><au>Chowdhury, Silvia</au><au>Xin, Ruijing</au><au>Alshehri, Saad M.</au><au>Bando, Yoshio</au><au>Yamauchi, Yusuke</au><au>Kaneti, Yusuf Valentino</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Carbon nanotube-decorated hierarchical porous nickel/carbon hybrid derived from nickel-based metal-organic framework for enhanced methyl blue adsorption</atitle><jtitle>Journal of colloid and interface science</jtitle><addtitle>J Colloid Interface Sci</addtitle><date>2023-05-15</date><risdate>2023</risdate><volume>638</volume><spage>220</spage><epage>230</epage><pages>220-230</pages><issn>0021-9797</issn><eissn>1095-7103</eissn><abstract>[Display omitted]
This work reports the incorporation of coordinated water into Ni-BTC nanorods (Ni-BTC-O) which induces their structural transformation to Ni-BTC nanofibres (Ni-BTC-F). The carbonization of the Ni-BTC nanofibres at 600 °C results in the formation of carbon nanotube (CNT)-decorated hierarchical porous nickel/carbon hybrid (labelled as Ni/C-600) with enlarged pores. In contrast, the Ni/C hybrid obtained from the carbonization of the original (unmodified) Ni-BTC nanorods (Ni-BTC-O) at 600 °C (labelled as Ni-BTC-O-600) exhibits smaller pore size and does not show the formation of CNTs. The Ni/C-600 hybrid derived from Ni-BTC-F shows a very high adsorption capacity of 686.8 mg g−1 toward methyl blue (MB) dye. This is approximately 4.8 times higher than the adsorption capacity of Ni-BTC-O-600 (144.1 mg g−1). The higher adsorption performance of Ni/C-600 relative to Ni-BTC-O-600 can be attributed to its larger pore volume, hierarchical porosity, and additional adsorption sites provided by the CNTs. In addition, the Ni/C-600 hybrid can maintain 90% of its adsorption capacity after 5 consecutive cycles, demonstrating its potential as an efficient and recyclable adsorbent for MB dye.</abstract><cop>United States</cop><pub>Elsevier Inc</pub><pmid>36738545</pmid><doi>10.1016/j.jcis.2023.01.075</doi><tpages>11</tpages></addata></record> |
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| subjects | adsorbents Adsorption carbon carbon nanotubes carbonization coordination polymers Dye removal dyes Hierarchical porous carbon Metal-organic frameworks nanofibers nanorods nickel porosity Wastewater treatment |
| title | Carbon nanotube-decorated hierarchical porous nickel/carbon hybrid derived from nickel-based metal-organic framework for enhanced methyl blue adsorption |
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