Environmental application of engineering magnesite slag for phosphate adsorption from wastewater
Herein, magnesite slags (MS), which remain after sulfuric acid extraction from light burnt magnesite in the magnesite industry, were used as phosphate adsorbents in wastewater. The MS were calcined under 700 °C to enhance phosphate adsorption. The calcined magnesite slags (CMS) were characterized by...
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| Veröffentlicht in: | Environmental science and pollution research international 2022-08, Vol.29 (39), p.59502-59512 |
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| description | Herein, magnesite slags (MS), which remain after sulfuric acid extraction from light burnt magnesite in the magnesite industry, were used as phosphate adsorbents in wastewater. The MS were calcined under 700 °C to enhance phosphate adsorption. The calcined magnesite slags (CMS) were characterized by nitrogen adsorption–desorption isotherm, X-ray diffraction, and scanning electron microscopy. A series of batch adsorption experiments were carried out to test the phosphate adsorption capacity of CMS. The results showed that the calcific treatment promoted the conversion from Mg, Ca, Fe, etc. compound to metal oxide of the MS. The generated metal oxide particles resulted in 237.4 mg/g increase in the phosphate adsorption capacity. The phosphate adsorption isotherm of CMS fitted the Langmuir model better, and the maximum adsorption capacity of CMS was 526 mg/g. The adsorption kinetics of phosphate on CMS can be described by the pseudo-second-order model. The phosphate removal efficiency was greater than 98% in 300 mg/L phosphate solution. Mechanism investigation results indicated that phosphate was adsorbed by CMS through MgO protonation, electrostatic attraction, Mg-P complexation, and ligand exchange. The results obtained in this work demonstrate that the CMS is a potential effective adsorbent for removal and reutilization phosphate from P-contaminated water, due to it can be employed as a fertilizer after phosphate adsorption.
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| doi_str_mv | 10.1007/s11356-022-20029-z |
| format | Article |
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Graphical abstract</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-022-20029-z</identifier><identifier>PMID: 35381926</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorbents ; Adsorption ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Calcium ; Earth and Environmental Science ; Ecotoxicology ; electron microscopy ; electrostatic interactions ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; fertilizers ; industry ; Iron ; Isotherms ; ligands ; Magnesite ; Magnesium carbonate ; Metal oxides ; nitrogen ; Phosphate ; Phosphates ; Phosphorus removal ; Protonation ; Research Article ; Roasting ; Scanning electron microscopy ; Slag ; slags ; sorption isotherms ; Sulfuric acid ; Waste Water Technology ; Wastewater ; Water Management ; Water pollution ; Water Pollution Control ; X-ray diffraction</subject><ispartof>Environmental science and pollution research international, 2022-08, Vol.29 (39), p.59502-59512</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022</rights><rights>2022. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c452t-5a0064d5da2a935b149af3d6b26f7fd8e144745f8dca42d09711342650ba5f9b3</citedby><cites>FETCH-LOGICAL-c452t-5a0064d5da2a935b149af3d6b26f7fd8e144745f8dca42d09711342650ba5f9b3</cites><orcidid>0000-0001-6983-7165</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-022-20029-z$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-022-20029-z$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/35381926$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Liang, Hai</creatorcontrib><creatorcontrib>Guo, Panliang</creatorcontrib><creatorcontrib>Yang, Yunhong</creatorcontrib><creatorcontrib>Wang, Wanting</creatorcontrib><creatorcontrib>Sun, Zhaonan</creatorcontrib><title>Environmental application of engineering magnesite slag for phosphate adsorption from wastewater</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Herein, magnesite slags (MS), which remain after sulfuric acid extraction from light burnt magnesite in the magnesite industry, were used as phosphate adsorbents in wastewater. The MS were calcined under 700 °C to enhance phosphate adsorption. The calcined magnesite slags (CMS) were characterized by nitrogen adsorption–desorption isotherm, X-ray diffraction, and scanning electron microscopy. A series of batch adsorption experiments were carried out to test the phosphate adsorption capacity of CMS. The results showed that the calcific treatment promoted the conversion from Mg, Ca, Fe, etc. compound to metal oxide of the MS. The generated metal oxide particles resulted in 237.4 mg/g increase in the phosphate adsorption capacity. The phosphate adsorption isotherm of CMS fitted the Langmuir model better, and the maximum adsorption capacity of CMS was 526 mg/g. The adsorption kinetics of phosphate on CMS can be described by the pseudo-second-order model. The phosphate removal efficiency was greater than 98% in 300 mg/L phosphate solution. Mechanism investigation results indicated that phosphate was adsorbed by CMS through MgO protonation, electrostatic attraction, Mg-P complexation, and ligand exchange. The results obtained in this work demonstrate that the CMS is a potential effective adsorbent for removal and reutilization phosphate from P-contaminated water, due to it can be employed as a fertilizer after phosphate adsorption.
Graphical abstract</description><subject>Adsorbents</subject><subject>Adsorption</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Calcium</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>electron microscopy</subject><subject>electrostatic interactions</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>fertilizers</subject><subject>industry</subject><subject>Iron</subject><subject>Isotherms</subject><subject>ligands</subject><subject>Magnesite</subject><subject>Magnesium carbonate</subject><subject>Metal oxides</subject><subject>nitrogen</subject><subject>Phosphate</subject><subject>Phosphates</subject><subject>Phosphorus removal</subject><subject>Protonation</subject><subject>Research Article</subject><subject>Roasting</subject><subject>Scanning electron microscopy</subject><subject>Slag</subject><subject>slags</subject><subject>sorption isotherms</subject><subject>Sulfuric acid</subject><subject>Waste Water Technology</subject><subject>Wastewater</subject><subject>Water Management</subject><subject>Water pollution</subject><subject>Water Pollution Control</subject><subject>X-ray 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pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2022-08-01</date><risdate>2022</risdate><volume>29</volume><issue>39</issue><spage>59502</spage><epage>59512</epage><pages>59502-59512</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Herein, magnesite slags (MS), which remain after sulfuric acid extraction from light burnt magnesite in the magnesite industry, were used as phosphate adsorbents in wastewater. The MS were calcined under 700 °C to enhance phosphate adsorption. The calcined magnesite slags (CMS) were characterized by nitrogen adsorption–desorption isotherm, X-ray diffraction, and scanning electron microscopy. A series of batch adsorption experiments were carried out to test the phosphate adsorption capacity of CMS. The results showed that the calcific treatment promoted the conversion from Mg, Ca, Fe, etc. compound to metal oxide of the MS. The generated metal oxide particles resulted in 237.4 mg/g increase in the phosphate adsorption capacity. The phosphate adsorption isotherm of CMS fitted the Langmuir model better, and the maximum adsorption capacity of CMS was 526 mg/g. The adsorption kinetics of phosphate on CMS can be described by the pseudo-second-order model. The phosphate removal efficiency was greater than 98% in 300 mg/L phosphate solution. Mechanism investigation results indicated that phosphate was adsorbed by CMS through MgO protonation, electrostatic attraction, Mg-P complexation, and ligand exchange. The results obtained in this work demonstrate that the CMS is a potential effective adsorbent for removal and reutilization phosphate from P-contaminated water, due to it can be employed as a fertilizer after phosphate adsorption.
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| subjects | Adsorbents Adsorption Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Calcium Earth and Environmental Science Ecotoxicology electron microscopy electrostatic interactions Environment Environmental Chemistry Environmental Health Environmental science fertilizers industry Iron Isotherms ligands Magnesite Magnesium carbonate Metal oxides nitrogen Phosphate Phosphates Phosphorus removal Protonation Research Article Roasting Scanning electron microscopy Slag slags sorption isotherms Sulfuric acid Waste Water Technology Wastewater Water Management Water pollution Water Pollution Control X-ray diffraction |
| title | Environmental application of engineering magnesite slag for phosphate adsorption from wastewater |
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