Local correlation during Ostwald ripening of two-dimensional islands on Ag(111)

Using two-dimensional Ag adatom islands on Ag(111) as a model system, we study the importance of local correlations in diffusion-limited Ostwald ripening. For the coverages studied (0.08, 0.21, and 0.3ML), we find that the ripening can be surprisingly well described in a nearest neighbour model base...

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Veröffentlicht in:Surface science 1999-11, Vol.441 (2-3), p.289-300
Hauptverfasser: Morgenstern, Karina, Rosenfeld, Georg, Comsa, George
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Rosenfeld, Georg
Comsa, George
description Using two-dimensional Ag adatom islands on Ag(111) as a model system, we study the importance of local correlations in diffusion-limited Ostwald ripening. For the coverages studied (0.08, 0.21, and 0.3ML), we find that the ripening can be surprisingly well described in a nearest neighbour model based on pairwise atom exchange between neighbouring islands. The results reveal the local nature of diffusion-limited Ostwald ripening and demonstrate the limits of the mean-field theories in describing experimental data.
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subjects Applied sciences
Condensed matter: structure, mechanical and thermal properties
Diffusion
interface formation
Exact sciences and technology
Metals. Metallurgy
Physics
Scanning tunneling microscopy
Silver
Solid surfaces and solid-solid interfaces
Surface diffusion
Surfaces and interfaces
thin films and whiskers (structure and nonelectronic properties)
title Local correlation during Ostwald ripening of two-dimensional islands on Ag(111)
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