Enhanced Dielectric Energy Storage Performance of 0.45Na0.5Bi0.5TiO3‑0.55Sr0.7Bi0.2TiO3/AlN 0–3 Type Lead-Free Composite Ceramics

Na0.5Bi0.5TiO3 (NBT) ceramic is the promising dielectric material for energy storage devices due to its high maximum polarizability and temperature stability. However, its low breakdown strength limits its application. Here, we prepared 0–3 type composite 0.45Na0.5Bi0.5TiO3-0.55Sr0.7Bi0.2TiO3/x wt %...

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Veröffentlicht in:ACS applied materials & interfaces 2022-04, Vol.14 (15), p.17652-17661
Hauptverfasser: You, Di, Tan, Hua, Yan, Zilin, Gao, Huayun, Chen, Shenggui, Ma, Weigang, Fan, Pengyuan, Tran, Nguyen-Minh-An, Liu, Yang, Salamon, David, Zhang, Haibo
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container_end_page 17661
container_issue 15
container_start_page 17652
container_title ACS applied materials & interfaces
container_volume 14
creator You, Di
Tan, Hua
Yan, Zilin
Gao, Huayun
Chen, Shenggui
Ma, Weigang
Fan, Pengyuan
Tran, Nguyen-Minh-An
Liu, Yang
Salamon, David
Zhang, Haibo
description Na0.5Bi0.5TiO3 (NBT) ceramic is the promising dielectric material for energy storage devices due to its high maximum polarizability and temperature stability. However, its low breakdown strength limits its application. Here, we prepared 0–3 type composite 0.45Na0.5Bi0.5TiO3-0.55Sr0.7Bi0.2TiO3/x wt % AlN (NBT-SBT/xAlN) to increase the breakdown strength. The effects of the various AlN contents on the phase composition, microstructures, dielectric, and energy storage properties of NBT-SBT were systematically discussed. The result showed that the enhanced energy storage properties were obtained by introducing AlN particles. The NBT-SBT/6AlN composite ceramics showed a high breakdown strength of 360 kV/cm, large energy density of 5.53 J/cm3, and energy efficiency of 90%. Meanwhile, the excellent frequency (10–500 Hz) and temperature stability (25–125 °C) were exhibited with the fluctuation of energy storage within 9% and energy efficiency more than 87%, suggesting that the 0–3 composite NBT-SBT/xAlN is a candidate dielectric material for the dielectric energy storage.
doi_str_mv 10.1021/acsami.2c01406
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title Enhanced Dielectric Energy Storage Performance of 0.45Na0.5Bi0.5TiO3‑0.55Sr0.7Bi0.2TiO3/AlN 0–3 Type Lead-Free Composite Ceramics
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