Enhanced Dielectric Energy Storage Performance of 0.45Na0.5Bi0.5TiO3‑0.55Sr0.7Bi0.2TiO3/AlN 0–3 Type Lead-Free Composite Ceramics
Na0.5Bi0.5TiO3 (NBT) ceramic is the promising dielectric material for energy storage devices due to its high maximum polarizability and temperature stability. However, its low breakdown strength limits its application. Here, we prepared 0–3 type composite 0.45Na0.5Bi0.5TiO3-0.55Sr0.7Bi0.2TiO3/x wt %...
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Veröffentlicht in: | ACS applied materials & interfaces 2022-04, Vol.14 (15), p.17652-17661 |
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creator | You, Di Tan, Hua Yan, Zilin Gao, Huayun Chen, Shenggui Ma, Weigang Fan, Pengyuan Tran, Nguyen-Minh-An Liu, Yang Salamon, David Zhang, Haibo |
description | Na0.5Bi0.5TiO3 (NBT) ceramic is the promising dielectric material for energy storage devices due to its high maximum polarizability and temperature stability. However, its low breakdown strength limits its application. Here, we prepared 0–3 type composite 0.45Na0.5Bi0.5TiO3-0.55Sr0.7Bi0.2TiO3/x wt % AlN (NBT-SBT/xAlN) to increase the breakdown strength. The effects of the various AlN contents on the phase composition, microstructures, dielectric, and energy storage properties of NBT-SBT were systematically discussed. The result showed that the enhanced energy storage properties were obtained by introducing AlN particles. The NBT-SBT/6AlN composite ceramics showed a high breakdown strength of 360 kV/cm, large energy density of 5.53 J/cm3, and energy efficiency of 90%. Meanwhile, the excellent frequency (10–500 Hz) and temperature stability (25–125 °C) were exhibited with the fluctuation of energy storage within 9% and energy efficiency more than 87%, suggesting that the 0–3 composite NBT-SBT/xAlN is a candidate dielectric material for the dielectric energy storage. |
doi_str_mv | 10.1021/acsami.2c01406 |
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However, its low breakdown strength limits its application. Here, we prepared 0–3 type composite 0.45Na0.5Bi0.5TiO3-0.55Sr0.7Bi0.2TiO3/x wt % AlN (NBT-SBT/xAlN) to increase the breakdown strength. The effects of the various AlN contents on the phase composition, microstructures, dielectric, and energy storage properties of NBT-SBT were systematically discussed. The result showed that the enhanced energy storage properties were obtained by introducing AlN particles. The NBT-SBT/6AlN composite ceramics showed a high breakdown strength of 360 kV/cm, large energy density of 5.53 J/cm3, and energy efficiency of 90%. Meanwhile, the excellent frequency (10–500 Hz) and temperature stability (25–125 °C) were exhibited with the fluctuation of energy storage within 9% and energy efficiency more than 87%, suggesting that the 0–3 composite NBT-SBT/xAlN is a candidate dielectric material for the dielectric energy storage.</description><identifier>ISSN: 1944-8244</identifier><identifier>EISSN: 1944-8252</identifier><identifier>DOI: 10.1021/acsami.2c01406</identifier><language>eng</language><publisher>American Chemical Society</publisher><subject>Functional Inorganic Materials and Devices</subject><ispartof>ACS applied materials & interfaces, 2022-04, Vol.14 (15), p.17652-17661</ispartof><rights>2022 American Chemical Society</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><orcidid>0000-0002-5544-531X</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acsami.2c01406$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acsami.2c01406$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,776,780,27055,27903,27904,56717,56767</link.rule.ids></links><search><creatorcontrib>You, Di</creatorcontrib><creatorcontrib>Tan, Hua</creatorcontrib><creatorcontrib>Yan, Zilin</creatorcontrib><creatorcontrib>Gao, Huayun</creatorcontrib><creatorcontrib>Chen, Shenggui</creatorcontrib><creatorcontrib>Ma, Weigang</creatorcontrib><creatorcontrib>Fan, Pengyuan</creatorcontrib><creatorcontrib>Tran, Nguyen-Minh-An</creatorcontrib><creatorcontrib>Liu, Yang</creatorcontrib><creatorcontrib>Salamon, David</creatorcontrib><creatorcontrib>Zhang, Haibo</creatorcontrib><title>Enhanced Dielectric Energy Storage Performance of 0.45Na0.5Bi0.5TiO3‑0.55Sr0.7Bi0.2TiO3/AlN 0–3 Type Lead-Free Composite Ceramics</title><title>ACS applied materials & interfaces</title><addtitle>ACS Appl. Mater. Interfaces</addtitle><description>Na0.5Bi0.5TiO3 (NBT) ceramic is the promising dielectric material for energy storage devices due to its high maximum polarizability and temperature stability. However, its low breakdown strength limits its application. Here, we prepared 0–3 type composite 0.45Na0.5Bi0.5TiO3-0.55Sr0.7Bi0.2TiO3/x wt % AlN (NBT-SBT/xAlN) to increase the breakdown strength. The effects of the various AlN contents on the phase composition, microstructures, dielectric, and energy storage properties of NBT-SBT were systematically discussed. The result showed that the enhanced energy storage properties were obtained by introducing AlN particles. The NBT-SBT/6AlN composite ceramics showed a high breakdown strength of 360 kV/cm, large energy density of 5.53 J/cm3, and energy efficiency of 90%. Meanwhile, the excellent frequency (10–500 Hz) and temperature stability (25–125 °C) were exhibited with the fluctuation of energy storage within 9% and energy efficiency more than 87%, suggesting that the 0–3 composite NBT-SBT/xAlN is a candidate dielectric material for the dielectric energy storage.</description><subject>Functional Inorganic Materials and Devices</subject><issn>1944-8244</issn><issn>1944-8252</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNo9kM1OwkAUhRujiYhuXc_SmLTMb9tZIoKaEDAB18105hZLSgdnyoIdGx_A-IY8iW0gbu45OTm5OfmC4J7giGBKBkp7tSkjqjHhOL4IekRyHqZU0Mt_z_l1cOP9GuOYUSx6wfe4_lS1BoOeS6hAN67UaFyDW-3RorFOrQC9gyus23Q1ZAuEIy5mCkfiqWzPspyz4-GndWLhcJR0Ie3CwbCaIXw8_DK03G8BTUGZcOIA0MhuttaXTevAtZO1vw2uClV5uDtrP_iYjJej13A6f3kbDaehopQ1oeEFNSmVihvAhVLaUJbzXHJqACTEmiQFEYRKkHlapFJCaqQ0QlOZQJ4b1g8eTn-3zn7twDfZpvQaqkrVYHc-ozFPYiGkYG318VRtsWZru3N1OywjOOtYZyfW2Zk1-wM2-HJR</recordid><startdate>20220420</startdate><enddate>20220420</enddate><creator>You, Di</creator><creator>Tan, Hua</creator><creator>Yan, Zilin</creator><creator>Gao, Huayun</creator><creator>Chen, Shenggui</creator><creator>Ma, Weigang</creator><creator>Fan, Pengyuan</creator><creator>Tran, Nguyen-Minh-An</creator><creator>Liu, Yang</creator><creator>Salamon, David</creator><creator>Zhang, Haibo</creator><general>American Chemical Society</general><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-5544-531X</orcidid></search><sort><creationdate>20220420</creationdate><title>Enhanced Dielectric Energy Storage Performance of 0.45Na0.5Bi0.5TiO3‑0.55Sr0.7Bi0.2TiO3/AlN 0–3 Type Lead-Free Composite Ceramics</title><author>You, Di ; Tan, Hua ; Yan, Zilin ; Gao, Huayun ; Chen, Shenggui ; Ma, Weigang ; Fan, Pengyuan ; Tran, Nguyen-Minh-An ; Liu, Yang ; Salamon, David ; Zhang, Haibo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a223t-d4f2d829a4de0faacd23b4b942dee9e6c17f15129e9b8f899e8d99d5c297ebbd3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Functional Inorganic Materials and Devices</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>You, Di</creatorcontrib><creatorcontrib>Tan, Hua</creatorcontrib><creatorcontrib>Yan, Zilin</creatorcontrib><creatorcontrib>Gao, Huayun</creatorcontrib><creatorcontrib>Chen, Shenggui</creatorcontrib><creatorcontrib>Ma, Weigang</creatorcontrib><creatorcontrib>Fan, Pengyuan</creatorcontrib><creatorcontrib>Tran, Nguyen-Minh-An</creatorcontrib><creatorcontrib>Liu, Yang</creatorcontrib><creatorcontrib>Salamon, David</creatorcontrib><creatorcontrib>Zhang, Haibo</creatorcontrib><collection>MEDLINE - Academic</collection><jtitle>ACS applied materials & interfaces</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>You, Di</au><au>Tan, Hua</au><au>Yan, Zilin</au><au>Gao, Huayun</au><au>Chen, Shenggui</au><au>Ma, Weigang</au><au>Fan, Pengyuan</au><au>Tran, Nguyen-Minh-An</au><au>Liu, Yang</au><au>Salamon, David</au><au>Zhang, Haibo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Enhanced Dielectric Energy Storage Performance of 0.45Na0.5Bi0.5TiO3‑0.55Sr0.7Bi0.2TiO3/AlN 0–3 Type Lead-Free Composite Ceramics</atitle><jtitle>ACS applied materials & interfaces</jtitle><addtitle>ACS Appl. Mater. Interfaces</addtitle><date>2022-04-20</date><risdate>2022</risdate><volume>14</volume><issue>15</issue><spage>17652</spage><epage>17661</epage><pages>17652-17661</pages><issn>1944-8244</issn><eissn>1944-8252</eissn><abstract>Na0.5Bi0.5TiO3 (NBT) ceramic is the promising dielectric material for energy storage devices due to its high maximum polarizability and temperature stability. However, its low breakdown strength limits its application. Here, we prepared 0–3 type composite 0.45Na0.5Bi0.5TiO3-0.55Sr0.7Bi0.2TiO3/x wt % AlN (NBT-SBT/xAlN) to increase the breakdown strength. The effects of the various AlN contents on the phase composition, microstructures, dielectric, and energy storage properties of NBT-SBT were systematically discussed. The result showed that the enhanced energy storage properties were obtained by introducing AlN particles. The NBT-SBT/6AlN composite ceramics showed a high breakdown strength of 360 kV/cm, large energy density of 5.53 J/cm3, and energy efficiency of 90%. Meanwhile, the excellent frequency (10–500 Hz) and temperature stability (25–125 °C) were exhibited with the fluctuation of energy storage within 9% and energy efficiency more than 87%, suggesting that the 0–3 composite NBT-SBT/xAlN is a candidate dielectric material for the dielectric energy storage.</abstract><pub>American Chemical Society</pub><doi>10.1021/acsami.2c01406</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0002-5544-531X</orcidid></addata></record> |
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title | Enhanced Dielectric Energy Storage Performance of 0.45Na0.5Bi0.5TiO3‑0.55Sr0.7Bi0.2TiO3/AlN 0–3 Type Lead-Free Composite Ceramics |
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