Upconversion under Photon Trapping in ZnO/BN Nanoarray: An Ultrahigh Responsivity Solar‐Blind Photodetecting Paper
Solar‐blind photodetectors (PDs) are widely applicable in special, military, medical, environmental, and commercial fields. However, high performance and flexible PD for deep ultraviolet (UV) range is still a challenge. Here, it is demonstrated that an upconversion of photon absorption beyond the en...
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| creator | Liu, Guozhen Chen, Han Lu, Shiqiang Liu, Lian Xu, Xiangyu Shi, Lan Chen, Binghuan Guo, Bin Shen, Peng Cai, Yehang Zhang, Hongye Tang, Yan Soomro, Abdul Majid Xu, Feiya Chen, Xiaohong Zheng, Tongchang Li, Jing Li, Shuping Cai, Duanjun Kang, Junyong |
| description | Solar‐blind photodetectors (PDs) are widely applicable in special, military, medical, environmental, and commercial fields. However, high performance and flexible PD for deep ultraviolet (UV) range is still a challenge. Here, it is demonstrated that an upconversion of photon absorption beyond the energy bandgap is achieved in the ZnO nanoarray/h‐BN heterostructure, which enables the ultrahigh responsivity of a solar‐blind photodetecting paper. The direct growth of ultralong ZnO nanoarray on polycrystalline copper paper induced by h‐BN 2D interlayer is obtained. Meanwhile, strong photon trapping takes place within the ZnO nanoarray forest through the cyclic state transition of surface oxygen ions, resulting in an extremely high absorption efficiency (> 99.5%). A flexible photodetecting paper is fabricated for switchable detections between near UV and deep UV signals by critical external bias. The device shows robust reliability, ultrahigh responsivity up to 700 A W−1 @ 265–276 nm, and high photoconductive gain of ≈2 × 103. A negative differential resistance effect is revealed for driving the rapid transfer of up‐converted electrons between adjacent energy valleys (Γ to A) above the critical bias (3.9 V). The discovered rationale and device structure are expected to bring high‐efficiency deep UV detecting and future wearable applications.
A solar‐blind photodetecting paper based on ZnO nanoarray and 2D h‐BN interlayer is developed with ultrahigh responsivity up to 700 A W−1 @ 265–276 nm and switchable detection bands between UVA (>315 nm) and UVC ( |
| doi_str_mv | 10.1002/smll.202200563 |
| format | Article |
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A solar‐blind photodetecting paper based on ZnO nanoarray and 2D h‐BN interlayer is developed with ultrahigh responsivity up to 700 A W−1 @ 265–276 nm and switchable detection bands between UVA (>315 nm) and UVC (<280 nm), through up‐conversion absorption and negative differential resistance effect.</description><identifier>ISSN: 1613-6810</identifier><identifier>EISSN: 1613-6829</identifier><identifier>DOI: 10.1002/smll.202200563</identifier><identifier>PMID: 35289505</identifier><language>eng</language><publisher>Germany: Wiley Subscription Services, Inc</publisher><subject>Bias ; Energy gap ; Extreme values ; Heterostructures ; hexagonal boron nitride ; high responsivity ; Interlayers ; Nanotechnology ; negative differential resistance ; Oxygen ions ; Photon absorption ; Photons ; Photovoltaic cells ; Reproducibility of Results ; solar‐blind ultraviolet photodetectors ; Sunlight ; Trapping ; Ultraviolet Rays ; Upconversion ; Zinc oxide ; Zinc Oxide - chemistry ; ZnO nanoarrays</subject><ispartof>Small (Weinheim an der Bergstrasse, Germany), 2022-06, Vol.18 (22), p.e2200563-n/a</ispartof><rights>2022 Wiley‐VCH GmbH</rights><rights>2022 Wiley-VCH GmbH.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c3733-273ef3e376f1601c49b552a10b1304570b1ee349d78a01cb9f5dce22712958823</citedby><cites>FETCH-LOGICAL-c3733-273ef3e376f1601c49b552a10b1304570b1ee349d78a01cb9f5dce22712958823</cites><orcidid>0000-0002-7094-7799</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fsmll.202200563$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fsmll.202200563$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,776,780,1411,27901,27902,45550,45551</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/35289505$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Liu, Guozhen</creatorcontrib><creatorcontrib>Chen, Han</creatorcontrib><creatorcontrib>Lu, Shiqiang</creatorcontrib><creatorcontrib>Liu, Lian</creatorcontrib><creatorcontrib>Xu, Xiangyu</creatorcontrib><creatorcontrib>Shi, Lan</creatorcontrib><creatorcontrib>Chen, Binghuan</creatorcontrib><creatorcontrib>Guo, Bin</creatorcontrib><creatorcontrib>Shen, Peng</creatorcontrib><creatorcontrib>Cai, Yehang</creatorcontrib><creatorcontrib>Zhang, Hongye</creatorcontrib><creatorcontrib>Tang, Yan</creatorcontrib><creatorcontrib>Soomro, Abdul Majid</creatorcontrib><creatorcontrib>Xu, Feiya</creatorcontrib><creatorcontrib>Chen, Xiaohong</creatorcontrib><creatorcontrib>Zheng, Tongchang</creatorcontrib><creatorcontrib>Li, Jing</creatorcontrib><creatorcontrib>Li, Shuping</creatorcontrib><creatorcontrib>Cai, Duanjun</creatorcontrib><creatorcontrib>Kang, Junyong</creatorcontrib><title>Upconversion under Photon Trapping in ZnO/BN Nanoarray: An Ultrahigh Responsivity Solar‐Blind Photodetecting Paper</title><title>Small (Weinheim an der Bergstrasse, Germany)</title><addtitle>Small</addtitle><description>Solar‐blind photodetectors (PDs) are widely applicable in special, military, medical, environmental, and commercial fields. However, high performance and flexible PD for deep ultraviolet (UV) range is still a challenge. Here, it is demonstrated that an upconversion of photon absorption beyond the energy bandgap is achieved in the ZnO nanoarray/h‐BN heterostructure, which enables the ultrahigh responsivity of a solar‐blind photodetecting paper. The direct growth of ultralong ZnO nanoarray on polycrystalline copper paper induced by h‐BN 2D interlayer is obtained. Meanwhile, strong photon trapping takes place within the ZnO nanoarray forest through the cyclic state transition of surface oxygen ions, resulting in an extremely high absorption efficiency (> 99.5%). A flexible photodetecting paper is fabricated for switchable detections between near UV and deep UV signals by critical external bias. The device shows robust reliability, ultrahigh responsivity up to 700 A W−1 @ 265–276 nm, and high photoconductive gain of ≈2 × 103. A negative differential resistance effect is revealed for driving the rapid transfer of up‐converted electrons between adjacent energy valleys (Γ to A) above the critical bias (3.9 V). The discovered rationale and device structure are expected to bring high‐efficiency deep UV detecting and future wearable applications.
A solar‐blind photodetecting paper based on ZnO nanoarray and 2D h‐BN interlayer is developed with ultrahigh responsivity up to 700 A W−1 @ 265–276 nm and switchable detection bands between UVA (>315 nm) and UVC (<280 nm), through up‐conversion absorption and negative differential resistance effect.</description><subject>Bias</subject><subject>Energy gap</subject><subject>Extreme values</subject><subject>Heterostructures</subject><subject>hexagonal boron nitride</subject><subject>high responsivity</subject><subject>Interlayers</subject><subject>Nanotechnology</subject><subject>negative differential resistance</subject><subject>Oxygen ions</subject><subject>Photon absorption</subject><subject>Photons</subject><subject>Photovoltaic cells</subject><subject>Reproducibility of Results</subject><subject>solar‐blind ultraviolet photodetectors</subject><subject>Sunlight</subject><subject>Trapping</subject><subject>Ultraviolet Rays</subject><subject>Upconversion</subject><subject>Zinc oxide</subject><subject>Zinc Oxide - chemistry</subject><subject>ZnO nanoarrays</subject><issn>1613-6810</issn><issn>1613-6829</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkU1vEzEQhi1ERT_gyhFZ4sIlqT1er9fc2opCpfRDtLlwWTm7s40rx17s3aLc-An8Rn4JjlJSiQunmdE882ikl5C3nE05Y3CcVs5NgQEwJkvxghzwkotJWYF-ues52yeHKT0wJjgU6hXZFxIqLZk8IMO8b4J_xJhs8HT0LUZ6swxDHu6i6Xvr76n19Ju_Pj69olfGBxOjWX-kJ57O3RDN0t4v6VdMffDJPtphTW-DM_H3z1-nzvp2K2txwGbYuG5Mj_E12euMS_jmqR6R-fmnu7Mvk9n154uzk9mkEUqICSiBnUChyo6XjDeFXkgJhrMFF6yQKldEUehWVSavF7qTbYMAioOWVQXiiHzYevsYvo-YhnplU4POGY9hTDWUQgNUXBcZff8P-hDG6PN3mVIAULJCZWq6pZoYUorY1X20KxPXNWf1Jo96k0e9yyMfvHvSjosVtjv8bwAZ0Fvgh3W4_o-uvr2czZ7lfwAFA5eb</recordid><startdate>20220601</startdate><enddate>20220601</enddate><creator>Liu, Guozhen</creator><creator>Chen, Han</creator><creator>Lu, Shiqiang</creator><creator>Liu, Lian</creator><creator>Xu, Xiangyu</creator><creator>Shi, Lan</creator><creator>Chen, Binghuan</creator><creator>Guo, Bin</creator><creator>Shen, Peng</creator><creator>Cai, Yehang</creator><creator>Zhang, Hongye</creator><creator>Tang, Yan</creator><creator>Soomro, Abdul Majid</creator><creator>Xu, Feiya</creator><creator>Chen, Xiaohong</creator><creator>Zheng, Tongchang</creator><creator>Li, Jing</creator><creator>Li, Shuping</creator><creator>Cai, Duanjun</creator><creator>Kang, Junyong</creator><general>Wiley Subscription Services, Inc</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-7094-7799</orcidid></search><sort><creationdate>20220601</creationdate><title>Upconversion under Photon Trapping in ZnO/BN Nanoarray: An Ultrahigh Responsivity Solar‐Blind Photodetecting Paper</title><author>Liu, Guozhen ; Chen, Han ; Lu, Shiqiang ; Liu, Lian ; Xu, Xiangyu ; Shi, Lan ; Chen, Binghuan ; Guo, Bin ; Shen, Peng ; Cai, Yehang ; Zhang, Hongye ; Tang, Yan ; Soomro, Abdul Majid ; Xu, Feiya ; Chen, Xiaohong ; Zheng, Tongchang ; Li, Jing ; Li, Shuping ; Cai, Duanjun ; Kang, Junyong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c3733-273ef3e376f1601c49b552a10b1304570b1ee349d78a01cb9f5dce22712958823</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Bias</topic><topic>Energy gap</topic><topic>Extreme values</topic><topic>Heterostructures</topic><topic>hexagonal boron nitride</topic><topic>high responsivity</topic><topic>Interlayers</topic><topic>Nanotechnology</topic><topic>negative differential resistance</topic><topic>Oxygen ions</topic><topic>Photon absorption</topic><topic>Photons</topic><topic>Photovoltaic cells</topic><topic>Reproducibility of Results</topic><topic>solar‐blind ultraviolet photodetectors</topic><topic>Sunlight</topic><topic>Trapping</topic><topic>Ultraviolet Rays</topic><topic>Upconversion</topic><topic>Zinc oxide</topic><topic>Zinc Oxide - chemistry</topic><topic>ZnO nanoarrays</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Liu, Guozhen</creatorcontrib><creatorcontrib>Chen, Han</creatorcontrib><creatorcontrib>Lu, Shiqiang</creatorcontrib><creatorcontrib>Liu, Lian</creatorcontrib><creatorcontrib>Xu, Xiangyu</creatorcontrib><creatorcontrib>Shi, Lan</creatorcontrib><creatorcontrib>Chen, Binghuan</creatorcontrib><creatorcontrib>Guo, Bin</creatorcontrib><creatorcontrib>Shen, Peng</creatorcontrib><creatorcontrib>Cai, Yehang</creatorcontrib><creatorcontrib>Zhang, Hongye</creatorcontrib><creatorcontrib>Tang, Yan</creatorcontrib><creatorcontrib>Soomro, Abdul Majid</creatorcontrib><creatorcontrib>Xu, Feiya</creatorcontrib><creatorcontrib>Chen, Xiaohong</creatorcontrib><creatorcontrib>Zheng, Tongchang</creatorcontrib><creatorcontrib>Li, Jing</creatorcontrib><creatorcontrib>Li, Shuping</creatorcontrib><creatorcontrib>Cai, Duanjun</creatorcontrib><creatorcontrib>Kang, Junyong</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Small (Weinheim an der Bergstrasse, Germany)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Liu, Guozhen</au><au>Chen, Han</au><au>Lu, Shiqiang</au><au>Liu, Lian</au><au>Xu, Xiangyu</au><au>Shi, Lan</au><au>Chen, Binghuan</au><au>Guo, Bin</au><au>Shen, Peng</au><au>Cai, Yehang</au><au>Zhang, Hongye</au><au>Tang, Yan</au><au>Soomro, Abdul Majid</au><au>Xu, Feiya</au><au>Chen, Xiaohong</au><au>Zheng, Tongchang</au><au>Li, Jing</au><au>Li, Shuping</au><au>Cai, Duanjun</au><au>Kang, Junyong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Upconversion under Photon Trapping in ZnO/BN Nanoarray: An Ultrahigh Responsivity Solar‐Blind Photodetecting Paper</atitle><jtitle>Small (Weinheim an der Bergstrasse, Germany)</jtitle><addtitle>Small</addtitle><date>2022-06-01</date><risdate>2022</risdate><volume>18</volume><issue>22</issue><spage>e2200563</spage><epage>n/a</epage><pages>e2200563-n/a</pages><issn>1613-6810</issn><eissn>1613-6829</eissn><abstract>Solar‐blind photodetectors (PDs) are widely applicable in special, military, medical, environmental, and commercial fields. However, high performance and flexible PD for deep ultraviolet (UV) range is still a challenge. Here, it is demonstrated that an upconversion of photon absorption beyond the energy bandgap is achieved in the ZnO nanoarray/h‐BN heterostructure, which enables the ultrahigh responsivity of a solar‐blind photodetecting paper. The direct growth of ultralong ZnO nanoarray on polycrystalline copper paper induced by h‐BN 2D interlayer is obtained. Meanwhile, strong photon trapping takes place within the ZnO nanoarray forest through the cyclic state transition of surface oxygen ions, resulting in an extremely high absorption efficiency (> 99.5%). A flexible photodetecting paper is fabricated for switchable detections between near UV and deep UV signals by critical external bias. The device shows robust reliability, ultrahigh responsivity up to 700 A W−1 @ 265–276 nm, and high photoconductive gain of ≈2 × 103. A negative differential resistance effect is revealed for driving the rapid transfer of up‐converted electrons between adjacent energy valleys (Γ to A) above the critical bias (3.9 V). The discovered rationale and device structure are expected to bring high‐efficiency deep UV detecting and future wearable applications.
A solar‐blind photodetecting paper based on ZnO nanoarray and 2D h‐BN interlayer is developed with ultrahigh responsivity up to 700 A W−1 @ 265–276 nm and switchable detection bands between UVA (>315 nm) and UVC (<280 nm), through up‐conversion absorption and negative differential resistance effect.</abstract><cop>Germany</cop><pub>Wiley Subscription Services, Inc</pub><pmid>35289505</pmid><doi>10.1002/smll.202200563</doi><tpages>14</tpages><orcidid>https://orcid.org/0000-0002-7094-7799</orcidid></addata></record> |
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| subjects | Bias Energy gap Extreme values Heterostructures hexagonal boron nitride high responsivity Interlayers Nanotechnology negative differential resistance Oxygen ions Photon absorption Photons Photovoltaic cells Reproducibility of Results solar‐blind ultraviolet photodetectors Sunlight Trapping Ultraviolet Rays Upconversion Zinc oxide Zinc Oxide - chemistry ZnO nanoarrays |
| title | Upconversion under Photon Trapping in ZnO/BN Nanoarray: An Ultrahigh Responsivity Solar‐Blind Photodetecting Paper |
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