Enhanced ultraviolet-visible photocatalysis of RGO/equaixial geometry TiO2 composites on degradation of organic dyes in water
The reduced graphene oxide dopped equaixial geometry TiO 2 (rGO/egTiO 2 ) composite as photocatalyst was synthesized hydrothermally with various mass ratios of tetrabutyl titanate. The photocatalyst is considered to be rGO/equaixial geometry TiO 2 in terms of modifying the combined reduced graphene...
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| Veröffentlicht in: | Environmental science and pollution research international 2022-02, Vol.29 (8), p.12222-12236 |
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| creator | Hasan, Jaafar Wang, Jing Wang, Zhentao Idrees, Muhammad Batool, Saima Zhang, Caiwei Qin, Chuanguang |
| description | The reduced graphene oxide dopped equaixial geometry TiO
2
(rGO/egTiO
2
) composite as photocatalyst was synthesized hydrothermally with various mass ratios of tetrabutyl titanate. The photocatalyst is considered to be rGO/equaixial geometry TiO
2
in terms of modifying the combined reduced graphene Oxide and TiO
2
. The rGO plays a vital role in rGO/egTiO
2
composite as photocatalysts were analyzed in methylene blue (MB) and rhodamine B (RhB) photocatalytic degradation under UV and simulated solar light irradiation. This synthesized catalyst was characterized by various analytical techniques such as XPS, XRD, SEM, BET, and TEM. The rGO/egTiO
2
composite exhibits enhanced photocatalytic performance with degradation rates of 97.5 and 97% on RhB and MB for 60 min under UV radiation respectively, while the degradation rate of 94 and 92 % was observed on the same dyes for 6 h under the simulated sunlight radiation. The enhanced photocatalytic performance of the rGO/egTiO
2
composite under ultraviolet irradiation source was owing to a high separation efficiency of the photo-induced electron-hole pairs, while the photocatalytic performance under simulated sunlight radiation was due to the photosensitive and charge separator behavior of rGO. This offers us an excellent potential of significant photocatalytic activity for the removal of organic contaminants from wastewater.
Graphical abstract |
| doi_str_mv | 10.1007/s11356-021-16605-4 |
| format | Article |
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2
(rGO/egTiO
2
) composite as photocatalyst was synthesized hydrothermally with various mass ratios of tetrabutyl titanate. The photocatalyst is considered to be rGO/equaixial geometry TiO
2
in terms of modifying the combined reduced graphene Oxide and TiO
2
. The rGO plays a vital role in rGO/egTiO
2
composite as photocatalysts were analyzed in methylene blue (MB) and rhodamine B (RhB) photocatalytic degradation under UV and simulated solar light irradiation. This synthesized catalyst was characterized by various analytical techniques such as XPS, XRD, SEM, BET, and TEM. The rGO/egTiO
2
composite exhibits enhanced photocatalytic performance with degradation rates of 97.5 and 97% on RhB and MB for 60 min under UV radiation respectively, while the degradation rate of 94 and 92 % was observed on the same dyes for 6 h under the simulated sunlight radiation. The enhanced photocatalytic performance of the rGO/egTiO
2
composite under ultraviolet irradiation source was owing to a high separation efficiency of the photo-induced electron-hole pairs, while the photocatalytic performance under simulated sunlight radiation was due to the photosensitive and charge separator behavior of rGO. This offers us an excellent potential of significant photocatalytic activity for the removal of organic contaminants from wastewater.
Graphical abstract</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-021-16605-4</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Catalysts ; Catalytic activity ; Chemical synthesis ; Contaminants ; Dyes ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Geometry ; Graphene ; graphene oxide ; Holes (electron deficiencies) ; Irradiation ; Light irradiation ; lighting ; Mass ratios ; Methylene blue ; Organic contaminants ; Performance degradation ; Photocatalysis ; Photocatalysts ; Photodegradation ; Photosensitivity ; Radiation ; Research Article ; Rhodamine ; rhodamines ; Separators ; Simulation ; Sunlight ; Titanium dioxide ; Ultraviolet radiation ; Waste Water Technology ; Wastewater ; Water Management ; Water Pollution Control ; X ray photoelectron spectroscopy</subject><ispartof>Environmental science and pollution research international, 2022-02, Vol.29 (8), p.12222-12236</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c429t-3e9ecddb644d974a12fa73a96244adf22073ce9607a6fee9fc48bcada662c3453</citedby><cites>FETCH-LOGICAL-c429t-3e9ecddb644d974a12fa73a96244adf22073ce9607a6fee9fc48bcada662c3453</cites><orcidid>0000-0003-4849-0187</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-021-16605-4$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-021-16605-4$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Hasan, Jaafar</creatorcontrib><creatorcontrib>Wang, Jing</creatorcontrib><creatorcontrib>Wang, Zhentao</creatorcontrib><creatorcontrib>Idrees, Muhammad</creatorcontrib><creatorcontrib>Batool, Saima</creatorcontrib><creatorcontrib>Zhang, Caiwei</creatorcontrib><creatorcontrib>Qin, Chuanguang</creatorcontrib><title>Enhanced ultraviolet-visible photocatalysis of RGO/equaixial geometry TiO2 composites on degradation of organic dyes in water</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><description>The reduced graphene oxide dopped equaixial geometry TiO
2
(rGO/egTiO
2
) composite as photocatalyst was synthesized hydrothermally with various mass ratios of tetrabutyl titanate. The photocatalyst is considered to be rGO/equaixial geometry TiO
2
in terms of modifying the combined reduced graphene Oxide and TiO
2
. The rGO plays a vital role in rGO/egTiO
2
composite as photocatalysts were analyzed in methylene blue (MB) and rhodamine B (RhB) photocatalytic degradation under UV and simulated solar light irradiation. This synthesized catalyst was characterized by various analytical techniques such as XPS, XRD, SEM, BET, and TEM. The rGO/egTiO
2
composite exhibits enhanced photocatalytic performance with degradation rates of 97.5 and 97% on RhB and MB for 60 min under UV radiation respectively, while the degradation rate of 94 and 92 % was observed on the same dyes for 6 h under the simulated sunlight radiation. The enhanced photocatalytic performance of the rGO/egTiO
2
composite under ultraviolet irradiation source was owing to a high separation efficiency of the photo-induced electron-hole pairs, while the photocatalytic performance under simulated sunlight radiation was due to the photosensitive and charge separator behavior of rGO. This offers us an excellent potential of significant photocatalytic activity for the removal of organic contaminants from wastewater.
Graphical abstract</description><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Catalysts</subject><subject>Catalytic activity</subject><subject>Chemical synthesis</subject><subject>Contaminants</subject><subject>Dyes</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Geometry</subject><subject>Graphene</subject><subject>graphene oxide</subject><subject>Holes (electron deficiencies)</subject><subject>Irradiation</subject><subject>Light irradiation</subject><subject>lighting</subject><subject>Mass ratios</subject><subject>Methylene blue</subject><subject>Organic contaminants</subject><subject>Performance degradation</subject><subject>Photocatalysis</subject><subject>Photocatalysts</subject><subject>Photodegradation</subject><subject>Photosensitivity</subject><subject>Radiation</subject><subject>Research Article</subject><subject>Rhodamine</subject><subject>rhodamines</subject><subject>Separators</subject><subject>Simulation</subject><subject>Sunlight</subject><subject>Titanium dioxide</subject><subject>Ultraviolet radiation</subject><subject>Waste Water Technology</subject><subject>Wastewater</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><subject>X ray photoelectron spectroscopy</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNqFkU1rVDEUhoMoOFb_gKuAGzfX5uPcpFlKqVUoDEhdhzO5505T7txMk9zqLPrfTZ2C0IWuciDP-xwOL2PvpfgkhbCnRUrdm04o2UljRN_BC7aSRkJnwbmXbCUcQCc1wGv2ppRbIZRwyq7Yw8V8g3OggS9TzXgf00S1u48lbibi-5tUU8CK06HEwtPIv1-uT-luwfgr4sS3lHZU84Ffx7XiIe32qcRKjZz5QNuMA9bY5hZMeYtzDHw4tO84859YKb9lr0acCr17ek_Yjy8X1-dfu6v15bfzz1ddAOVqp8lRGIaNARicBZRqRKvRGQWAw6iUsDqQM8KiGYncGOBsE9pyY1TQ0OsT9vHo3ed0t1CpfhdLoGnCmdJSvDLagLLN8H-0t8b04PSj9cMz9DYteW6HNKHSSkgtzxqljlTIqZRMo9_nuMN88FL4x_L8sTzfyvN_yvPQQvoYKg2et5T_qv-R-g1kIp5g</recordid><startdate>20220201</startdate><enddate>20220201</enddate><creator>Hasan, Jaafar</creator><creator>Wang, Jing</creator><creator>Wang, Zhentao</creator><creator>Idrees, Muhammad</creator><creator>Batool, Saima</creator><creator>Zhang, Caiwei</creator><creator>Qin, 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ultraviolet-visible photocatalysis of RGO/equaixial geometry TiO2 composites on degradation of organic dyes in water</title><author>Hasan, Jaafar ; Wang, Jing ; Wang, Zhentao ; Idrees, Muhammad ; Batool, Saima ; Zhang, Caiwei ; Qin, Chuanguang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c429t-3e9ecddb644d974a12fa73a96244adf22073ce9607a6fee9fc48bcada662c3453</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Catalysts</topic><topic>Catalytic activity</topic><topic>Chemical synthesis</topic><topic>Contaminants</topic><topic>Dyes</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental 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Jaafar</creatorcontrib><creatorcontrib>Wang, Jing</creatorcontrib><creatorcontrib>Wang, Zhentao</creatorcontrib><creatorcontrib>Idrees, Muhammad</creatorcontrib><creatorcontrib>Batool, Saima</creatorcontrib><creatorcontrib>Zhang, Caiwei</creatorcontrib><creatorcontrib>Qin, Chuanguang</creatorcontrib><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Bacteriology Abstracts (Microbiology B)</collection><collection>Ecology Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>ABI/INFORM Collection</collection><collection>ABI/INFORM Global (PDF only)</collection><collection>Health & Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>ABI/INFORM Global (Alumni Edition)</collection><collection>Medical Database (Alumni 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Caiwei</au><au>Qin, Chuanguang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Enhanced ultraviolet-visible photocatalysis of RGO/equaixial geometry TiO2 composites on degradation of organic dyes in water</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><date>2022-02-01</date><risdate>2022</risdate><volume>29</volume><issue>8</issue><spage>12222</spage><epage>12236</epage><pages>12222-12236</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>The reduced graphene oxide dopped equaixial geometry TiO
2
(rGO/egTiO
2
) composite as photocatalyst was synthesized hydrothermally with various mass ratios of tetrabutyl titanate. The photocatalyst is considered to be rGO/equaixial geometry TiO
2
in terms of modifying the combined reduced graphene Oxide and TiO
2
. The rGO plays a vital role in rGO/egTiO
2
composite as photocatalysts were analyzed in methylene blue (MB) and rhodamine B (RhB) photocatalytic degradation under UV and simulated solar light irradiation. This synthesized catalyst was characterized by various analytical techniques such as XPS, XRD, SEM, BET, and TEM. The rGO/egTiO
2
composite exhibits enhanced photocatalytic performance with degradation rates of 97.5 and 97% on RhB and MB for 60 min under UV radiation respectively, while the degradation rate of 94 and 92 % was observed on the same dyes for 6 h under the simulated sunlight radiation. The enhanced photocatalytic performance of the rGO/egTiO
2
composite under ultraviolet irradiation source was owing to a high separation efficiency of the photo-induced electron-hole pairs, while the photocatalytic performance under simulated sunlight radiation was due to the photosensitive and charge separator behavior of rGO. This offers us an excellent potential of significant photocatalytic activity for the removal of organic contaminants from wastewater.
Graphical abstract</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s11356-021-16605-4</doi><tpages>15</tpages><orcidid>https://orcid.org/0000-0003-4849-0187</orcidid><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0944-1344 |
| ispartof | Environmental science and pollution research international, 2022-02, Vol.29 (8), p.12222-12236 |
| issn | 0944-1344 1614-7499 |
| language | eng |
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| source | Springer Nature - Complete Springer Journals |
| subjects | Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Catalysts Catalytic activity Chemical synthesis Contaminants Dyes Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental science Geometry Graphene graphene oxide Holes (electron deficiencies) Irradiation Light irradiation lighting Mass ratios Methylene blue Organic contaminants Performance degradation Photocatalysis Photocatalysts Photodegradation Photosensitivity Radiation Research Article Rhodamine rhodamines Separators Simulation Sunlight Titanium dioxide Ultraviolet radiation Waste Water Technology Wastewater Water Management Water Pollution Control X ray photoelectron spectroscopy |
| title | Enhanced ultraviolet-visible photocatalysis of RGO/equaixial geometry TiO2 composites on degradation of organic dyes in water |
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