Investigation of two new low-cost adsorbents functionalized with magnetic nanoparticles for the efficient removal of triclosan and a synthetic mixture
Triclosan (TCS) is widely used in the production of antibacterial products, being often found in wastewater. Therefore, this study developed new materials via soybean hulls (SBH F ) and açaí seeds (AÇS F ) functionalization with iron oxide nanoparticles to be applied in the TCS adsorption. The chara...
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| Veröffentlicht in: | Environmental science and pollution research international 2022-07, Vol.29 (31), p.46813-46829 |
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| creator | Vidovix, Taynara Basso Januário, Eduarda Freitas Diogo Araújo, Micael Furioso Bergamasco, Rosângela Vieira, Angélica Marquetotti Salcedo |
| description | Triclosan (TCS) is widely used in the production of antibacterial products, being often found in wastewater. Therefore, this study developed new materials via soybean hulls (SBH
F
) and açaí seeds (AÇS
F
) functionalization with iron oxide nanoparticles to be applied in the TCS adsorption. The characterization confirmed the functionalization of the materials. The adsorption results indicated that the equilibrium of the process occurred after 480 and 960 min for SBH
F
and AÇS
F
, respectively. The maximum adsorptive capacity values were 158.35 and 155.09 mg g
−1
for SBH
F
and AÇS
F
, respectively, at 318 K. The kinetic and isothermal data better fitted to the pseudo-second-order and Langmuir models. Thermodynamics indicated that the processes had an endothermic, spontaneous, and reversible character. The main adsorption mechanisms were H-bond and π-interactions. The pH and ionic strength studies indicated that the adsorption efficiency has not been reduced pronouncedly. The biosorbents reuse was effective for five cycles. In the synthetic mixture, the removal rate was satisfactory (92.53% and 57.02%, respectively for SBH
F
and AÇS
F
)
.
These results demonstrate the biosorbents high potential for large-scale application. |
| doi_str_mv | 10.1007/s11356-022-19187-x |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_2629384598</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2629384598</sourcerecordid><originalsourceid>FETCH-LOGICAL-c375t-c5a3689f8bba21dd8a8b90e0f144e8055af9e06990fe92b566f1cf7aad65ad913</originalsourceid><addsrcrecordid>eNp9kc1u1DAURi1ERYfCC7BAltiwCbUTO7GXqOKnUiU2ZW3dJNdTV4k92E5nyoPwvDidAhKLrnwln--70j2EvOHsA2esO0-cN7KtWF1XXHPVVYdnZMNbLqpOaP2cbJgWouKNEKfkZUq3jNVM190LctpI3nHB5Yb8uvR3mLLbQnbB02Bp3gfqcU-nsK-GkDKFMYXYo8-J2sUPKweT-4kj3bt8Q2fYesxuoB582EEs44QFDZHmG6RorRtcSdOIc7iD6WFHLFBI4Cn4kQJN976wa8nsDnmJ-IqcWJgSvn58z8j3z5-uL75WV9--XF58vKqGppO5GiQ0rdJW9T3UfBwVqF4zZJYLgYpJCVYja7VmFnXdy7a1fLAdwNhKGDVvzsj7Y-8uhh9LOYSZXRpwmsBjWJKp21o3SkitCvruP_Q2LLGcYqUUE6LlbKXqIzXEkFJEa3bRzRDvDWdmtWaO1kyxZh6smUMJvX2sXvoZx7-RP5oK0ByBVL78FuO_3U_U_gaN1qdE</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2680446108</pqid></control><display><type>article</type><title>Investigation of two new low-cost adsorbents functionalized with magnetic nanoparticles for the efficient removal of triclosan and a synthetic mixture</title><source>SpringerLink Journals - AutoHoldings</source><creator>Vidovix, Taynara Basso ; Januário, Eduarda Freitas Diogo ; Araújo, Micael Furioso ; Bergamasco, Rosângela ; Vieira, Angélica Marquetotti Salcedo</creator><creatorcontrib>Vidovix, Taynara Basso ; Januário, Eduarda Freitas Diogo ; Araújo, Micael Furioso ; Bergamasco, Rosângela ; Vieira, Angélica Marquetotti Salcedo</creatorcontrib><description>Triclosan (TCS) is widely used in the production of antibacterial products, being often found in wastewater. Therefore, this study developed new materials via soybean hulls (SBH
F
) and açaí seeds (AÇS
F
) functionalization with iron oxide nanoparticles to be applied in the TCS adsorption. The characterization confirmed the functionalization of the materials. The adsorption results indicated that the equilibrium of the process occurred after 480 and 960 min for SBH
F
and AÇS
F
, respectively. The maximum adsorptive capacity values were 158.35 and 155.09 mg g
−1
for SBH
F
and AÇS
F
, respectively, at 318 K. The kinetic and isothermal data better fitted to the pseudo-second-order and Langmuir models. Thermodynamics indicated that the processes had an endothermic, spontaneous, and reversible character. The main adsorption mechanisms were H-bond and π-interactions. The pH and ionic strength studies indicated that the adsorption efficiency has not been reduced pronouncedly. The biosorbents reuse was effective for five cycles. In the synthetic mixture, the removal rate was satisfactory (92.53% and 57.02%, respectively for SBH
F
and AÇS
F
)
.
These results demonstrate the biosorbents high potential for large-scale application.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-022-19187-x</identifier><identifier>PMID: 35171415</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorption ; Adsorptivity ; Antiinfectives and antibacterials ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Earth and Environmental Science ; Ecotoxicology ; Endothermic reactions ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Ionic strength ; Iron oxides ; Mixtures ; Nanoparticles ; Research Article ; Seeds ; Soybeans ; Triclosan ; Waste Water Technology ; Wastewater ; Water Management ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2022-07, Vol.29 (31), p.46813-46829</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022</rights><rights>2022. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c375t-c5a3689f8bba21dd8a8b90e0f144e8055af9e06990fe92b566f1cf7aad65ad913</citedby><cites>FETCH-LOGICAL-c375t-c5a3689f8bba21dd8a8b90e0f144e8055af9e06990fe92b566f1cf7aad65ad913</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-022-19187-x$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-022-19187-x$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27923,27924,41487,42556,51318</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/35171415$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Vidovix, Taynara Basso</creatorcontrib><creatorcontrib>Januário, Eduarda Freitas Diogo</creatorcontrib><creatorcontrib>Araújo, Micael Furioso</creatorcontrib><creatorcontrib>Bergamasco, Rosângela</creatorcontrib><creatorcontrib>Vieira, Angélica Marquetotti Salcedo</creatorcontrib><title>Investigation of two new low-cost adsorbents functionalized with magnetic nanoparticles for the efficient removal of triclosan and a synthetic mixture</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Triclosan (TCS) is widely used in the production of antibacterial products, being often found in wastewater. Therefore, this study developed new materials via soybean hulls (SBH
F
) and açaí seeds (AÇS
F
) functionalization with iron oxide nanoparticles to be applied in the TCS adsorption. The characterization confirmed the functionalization of the materials. The adsorption results indicated that the equilibrium of the process occurred after 480 and 960 min for SBH
F
and AÇS
F
, respectively. The maximum adsorptive capacity values were 158.35 and 155.09 mg g
−1
for SBH
F
and AÇS
F
, respectively, at 318 K. The kinetic and isothermal data better fitted to the pseudo-second-order and Langmuir models. Thermodynamics indicated that the processes had an endothermic, spontaneous, and reversible character. The main adsorption mechanisms were H-bond and π-interactions. The pH and ionic strength studies indicated that the adsorption efficiency has not been reduced pronouncedly. The biosorbents reuse was effective for five cycles. In the synthetic mixture, the removal rate was satisfactory (92.53% and 57.02%, respectively for SBH
F
and AÇS
F
)
.
These results demonstrate the biosorbents high potential for large-scale application.</description><subject>Adsorption</subject><subject>Adsorptivity</subject><subject>Antiinfectives and antibacterials</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Endothermic reactions</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Ionic strength</subject><subject>Iron oxides</subject><subject>Mixtures</subject><subject>Nanoparticles</subject><subject>Research Article</subject><subject>Seeds</subject><subject>Soybeans</subject><subject>Triclosan</subject><subject>Waste Water Technology</subject><subject>Wastewater</subject><subject>Water Management</subject><subject>Water Pollution 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Basic</collection><collection>MEDLINE - Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Vidovix, Taynara Basso</au><au>Januário, Eduarda Freitas Diogo</au><au>Araújo, Micael Furioso</au><au>Bergamasco, Rosângela</au><au>Vieira, Angélica Marquetotti Salcedo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Investigation of two new low-cost adsorbents functionalized with magnetic nanoparticles for the efficient removal of triclosan and a synthetic mixture</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2022-07-01</date><risdate>2022</risdate><volume>29</volume><issue>31</issue><spage>46813</spage><epage>46829</epage><pages>46813-46829</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Triclosan (TCS) is widely used in the production of antibacterial products, being often found in wastewater. Therefore, this study developed new materials via soybean hulls (SBH
F
) and açaí seeds (AÇS
F
) functionalization with iron oxide nanoparticles to be applied in the TCS adsorption. The characterization confirmed the functionalization of the materials. The adsorption results indicated that the equilibrium of the process occurred after 480 and 960 min for SBH
F
and AÇS
F
, respectively. The maximum adsorptive capacity values were 158.35 and 155.09 mg g
−1
for SBH
F
and AÇS
F
, respectively, at 318 K. The kinetic and isothermal data better fitted to the pseudo-second-order and Langmuir models. Thermodynamics indicated that the processes had an endothermic, spontaneous, and reversible character. The main adsorption mechanisms were H-bond and π-interactions. The pH and ionic strength studies indicated that the adsorption efficiency has not been reduced pronouncedly. The biosorbents reuse was effective for five cycles. In the synthetic mixture, the removal rate was satisfactory (92.53% and 57.02%, respectively for SBH
F
and AÇS
F
)
.
These results demonstrate the biosorbents high potential for large-scale application.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>35171415</pmid><doi>10.1007/s11356-022-19187-x</doi><tpages>17</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0944-1344 |
| ispartof | Environmental science and pollution research international, 2022-07, Vol.29 (31), p.46813-46829 |
| issn | 0944-1344 1614-7499 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_2629384598 |
| source | SpringerLink Journals - AutoHoldings |
| subjects | Adsorption Adsorptivity Antiinfectives and antibacterials Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Earth and Environmental Science Ecotoxicology Endothermic reactions Environment Environmental Chemistry Environmental Health Environmental science Ionic strength Iron oxides Mixtures Nanoparticles Research Article Seeds Soybeans Triclosan Waste Water Technology Wastewater Water Management Water Pollution Control |
| title | Investigation of two new low-cost adsorbents functionalized with magnetic nanoparticles for the efficient removal of triclosan and a synthetic mixture |
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