Particle-bound organic and elemental carbons for source identification of PM < 0.1 µm from biomass combustion
•PM
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| Veröffentlicht in: | Journal of environmental sciences (China) 2022-03, Vol.113, p.385-393 |
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| container_title | Journal of environmental sciences (China) |
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| creator | Samae, Hisam Tekasakul, Surajit Tekasakul, Perapong Phairuang, Worradorn Furuuchi, Masami Hongtieab, Surapa |
| description | •PM |
| doi_str_mv | 10.1016/j.jes.2021.06.015 |
| format | Article |
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Atmospheric nanoparticles (PM < 0.1 µm) are a major cause of environmental problems and also affect health risk. To control and reduce these problems, sources identification of atmospheric particulates is necessary. Combustion of bituminous coal and biomass including rubber wood, palm kernel, palm fiber, rice stubble, rice straw, maize residue, sugarcane leaves and sugarcane bagasse, which are considered as sources of air quality problems in many countries, was performed. Emissions of particle-bound chemical components including organic carbon (OC), elemental carbon (EC), water-soluble ions (NH4+, Cl−, NO3−, SO42−), elements (Ca, K, Mg, Na) and heavy metals (Cd, Cr, Ni, Pb) were investigated. The results revealed that PM < 0.1 µm from all samples was dominated by the OC component (>50%) with minor contribution from EC (3%-12%). The higher fraction of carbonaceous components was found in the particulates with smaller sizes, and lignin content may relate to concentration of pyrolyzed organic carbon (PyOC) resulting in the differences of OC/EC values. PM emitted from burning palm fiber and rice stubble showed high values of OC/EC and also high PyOC. Non-carbonaceous components such as Cl−, Cr, Ca, Cd, Ni, Na and Mg may be useful as source indicators, but they did not show any correlation with the size of PM.
[Display omitted]</description><identifier>ISSN: 1001-0742</identifier><identifier>EISSN: 1878-7320</identifier><identifier>DOI: 10.1016/j.jes.2021.06.015</identifier><identifier>PMID: 34963546</identifier><language>eng</language><publisher>Netherlands: Elsevier B.V</publisher><subject>Aerosols ; Air Pollutants - analysis ; Biomass ; Carbon - analysis ; China ; Elemental carbon ; Emission factors ; Environmental Monitoring ; Organic carbon ; Particle Size ; Particulate Matter - analysis ; PM<0.1 µm ; Source identification</subject><ispartof>Journal of environmental sciences (China), 2022-03, Vol.113, p.385-393</ispartof><rights>2021</rights><rights>Copyright © 2021. Published by Elsevier B.V.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c334t-b86948cdbf57ebd37b40c638291a2ed1df3496be0ea37c5c3242fe49169be6713</citedby><cites>FETCH-LOGICAL-c334t-b86948cdbf57ebd37b40c638291a2ed1df3496be0ea37c5c3242fe49169be6713</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.jes.2021.06.015$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/34963546$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Samae, Hisam</creatorcontrib><creatorcontrib>Tekasakul, Surajit</creatorcontrib><creatorcontrib>Tekasakul, Perapong</creatorcontrib><creatorcontrib>Phairuang, Worradorn</creatorcontrib><creatorcontrib>Furuuchi, Masami</creatorcontrib><creatorcontrib>Hongtieab, Surapa</creatorcontrib><title>Particle-bound organic and elemental carbons for source identification of PM < 0.1 µm from biomass combustion</title><title>Journal of environmental sciences (China)</title><addtitle>J Environ Sci (China)</addtitle><description>•PM<0.1 µm contained more than 50% of OC, EC fractions.•Emissions of PM<0.1 µm were dominated by OC2.•OC2 was expected to be a marker of biomass combustion.•High lignin content in biomass might be responsible for high OC/EC and PyOC values.•Cl−, Cr, Ca, Cd, Ni, Na and Mg have potential as source indicators.
Atmospheric nanoparticles (PM < 0.1 µm) are a major cause of environmental problems and also affect health risk. To control and reduce these problems, sources identification of atmospheric particulates is necessary. Combustion of bituminous coal and biomass including rubber wood, palm kernel, palm fiber, rice stubble, rice straw, maize residue, sugarcane leaves and sugarcane bagasse, which are considered as sources of air quality problems in many countries, was performed. Emissions of particle-bound chemical components including organic carbon (OC), elemental carbon (EC), water-soluble ions (NH4+, Cl−, NO3−, SO42−), elements (Ca, K, Mg, Na) and heavy metals (Cd, Cr, Ni, Pb) were investigated. The results revealed that PM < 0.1 µm from all samples was dominated by the OC component (>50%) with minor contribution from EC (3%-12%). The higher fraction of carbonaceous components was found in the particulates with smaller sizes, and lignin content may relate to concentration of pyrolyzed organic carbon (PyOC) resulting in the differences of OC/EC values. PM emitted from burning palm fiber and rice stubble showed high values of OC/EC and also high PyOC. Non-carbonaceous components such as Cl−, Cr, Ca, Cd, Ni, Na and Mg may be useful as source indicators, but they did not show any correlation with the size of PM.
[Display omitted]</description><subject>Aerosols</subject><subject>Air Pollutants - analysis</subject><subject>Biomass</subject><subject>Carbon - analysis</subject><subject>China</subject><subject>Elemental carbon</subject><subject>Emission factors</subject><subject>Environmental Monitoring</subject><subject>Organic carbon</subject><subject>Particle Size</subject><subject>Particulate Matter - analysis</subject><subject>PM<0.1 µm</subject><subject>Source identification</subject><issn>1001-0742</issn><issn>1878-7320</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNp9kMtu1TAQhi1UREvhAdggL7tJGF_iJCqbqioXqYguYG35MkY-SuLWTpD6NrxEX6BPho9O6ZLVjDTf_Jr5CHnHoGXA1Iddu8PScuCsBdUC616QEzb0Q9MLDke1B2AN9JIfk9el7ABAdtC9IsdCjkp0Up2QdGPyGt2EjU3b4mnKv8wSHTW1xwlnXFYzUWeyTUuhIWVa0pYd0ujrKIbozBrTQlOgN9_oR1ove_zz-DDTkNNMbUyzKYW6NNut7ME35GUwU8G3T_WU_Px09ePyS3P9_fPXy4vrxgkh18YOapSD8zZ0PVoveivBKTHwkRmOnvmwf8EioBG965zgkgeUI1OjRdUzcUrODrm3Od1tWFY9x-JwmsyCaSuaK9YJEGzgFWUH1OVUSsagb3OcTb7XDPTes97p6lnvPWtQunquO--f4jc7o3_e-Ce2AucHAOuTvyNmXVzExaGPGd2qfYr_if8L5_yPsw</recordid><startdate>202203</startdate><enddate>202203</enddate><creator>Samae, Hisam</creator><creator>Tekasakul, Surajit</creator><creator>Tekasakul, Perapong</creator><creator>Phairuang, Worradorn</creator><creator>Furuuchi, Masami</creator><creator>Hongtieab, Surapa</creator><general>Elsevier B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope></search><sort><creationdate>202203</creationdate><title>Particle-bound organic and elemental carbons for source identification of PM < 0.1 µm from biomass combustion</title><author>Samae, Hisam ; Tekasakul, Surajit ; Tekasakul, Perapong ; Phairuang, Worradorn ; Furuuchi, Masami ; Hongtieab, Surapa</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c334t-b86948cdbf57ebd37b40c638291a2ed1df3496be0ea37c5c3242fe49169be6713</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Aerosols</topic><topic>Air Pollutants - analysis</topic><topic>Biomass</topic><topic>Carbon - analysis</topic><topic>China</topic><topic>Elemental carbon</topic><topic>Emission factors</topic><topic>Environmental Monitoring</topic><topic>Organic carbon</topic><topic>Particle Size</topic><topic>Particulate Matter - analysis</topic><topic>PM<0.1 µm</topic><topic>Source identification</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Samae, Hisam</creatorcontrib><creatorcontrib>Tekasakul, Surajit</creatorcontrib><creatorcontrib>Tekasakul, Perapong</creatorcontrib><creatorcontrib>Phairuang, Worradorn</creatorcontrib><creatorcontrib>Furuuchi, Masami</creatorcontrib><creatorcontrib>Hongtieab, Surapa</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Journal of environmental sciences (China)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Samae, Hisam</au><au>Tekasakul, Surajit</au><au>Tekasakul, Perapong</au><au>Phairuang, Worradorn</au><au>Furuuchi, Masami</au><au>Hongtieab, Surapa</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Particle-bound organic and elemental carbons for source identification of PM < 0.1 µm from biomass combustion</atitle><jtitle>Journal of environmental sciences (China)</jtitle><addtitle>J Environ Sci (China)</addtitle><date>2022-03</date><risdate>2022</risdate><volume>113</volume><spage>385</spage><epage>393</epage><pages>385-393</pages><issn>1001-0742</issn><eissn>1878-7320</eissn><abstract>•PM<0.1 µm contained more than 50% of OC, EC fractions.•Emissions of PM<0.1 µm were dominated by OC2.•OC2 was expected to be a marker of biomass combustion.•High lignin content in biomass might be responsible for high OC/EC and PyOC values.•Cl−, Cr, Ca, Cd, Ni, Na and Mg have potential as source indicators.
Atmospheric nanoparticles (PM < 0.1 µm) are a major cause of environmental problems and also affect health risk. To control and reduce these problems, sources identification of atmospheric particulates is necessary. Combustion of bituminous coal and biomass including rubber wood, palm kernel, palm fiber, rice stubble, rice straw, maize residue, sugarcane leaves and sugarcane bagasse, which are considered as sources of air quality problems in many countries, was performed. Emissions of particle-bound chemical components including organic carbon (OC), elemental carbon (EC), water-soluble ions (NH4+, Cl−, NO3−, SO42−), elements (Ca, K, Mg, Na) and heavy metals (Cd, Cr, Ni, Pb) were investigated. The results revealed that PM < 0.1 µm from all samples was dominated by the OC component (>50%) with minor contribution from EC (3%-12%). The higher fraction of carbonaceous components was found in the particulates with smaller sizes, and lignin content may relate to concentration of pyrolyzed organic carbon (PyOC) resulting in the differences of OC/EC values. PM emitted from burning palm fiber and rice stubble showed high values of OC/EC and also high PyOC. Non-carbonaceous components such as Cl−, Cr, Ca, Cd, Ni, Na and Mg may be useful as source indicators, but they did not show any correlation with the size of PM.
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| ispartof | Journal of environmental sciences (China), 2022-03, Vol.113, p.385-393 |
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| source | MEDLINE; ScienceDirect Journals (5 years ago - present); Alma/SFX Local Collection |
| subjects | Aerosols Air Pollutants - analysis Biomass Carbon - analysis China Elemental carbon Emission factors Environmental Monitoring Organic carbon Particle Size Particulate Matter - analysis PM<0.1 µm Source identification |
| title | Particle-bound organic and elemental carbons for source identification of PM < 0.1 µm from biomass combustion |
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