Elucidation of adsorption mechanisms and mass transfer controlling resistances during single and binary adsorption of caffeic and chlorogenic acids
In this work, the potential of activated carbon to remove caffeic and chlorogenic acids in aqueous solution was investigated. The study focused on evaluating the single and binary adsorption equilibrium, as well as investigating the mass transfer resistances present during the process by applying di...
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| Veröffentlicht in: | Environmental science and pollution research international 2022-04, Vol.29 (18), p.26297-26311 |
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| creator | Hernández-Padilla, Eyden S. Zárate-Guzmán, Ana I. González-Ortega, Omar Padilla-Ortega, Erika Gómez-Durán, Azael Delgado-Sánchez, Pablo Aguilar-Aguilar, Angélica Cortés, Farid B. Ocampo-Pérez, Raúl |
| description | In this work, the potential of activated carbon to remove caffeic and chlorogenic acids in aqueous solution was investigated. The study focused on evaluating the single and binary adsorption equilibrium, as well as investigating the mass transfer resistances present during the process by applying diffusional models for a future scale-up of the process. For both compounds, the single adsorption equilibrium was studied at pH values of 3, 5, and 7. The experimental adsorption isotherms were interpreted using the Langmuir and Freundlich models, obtaining maximum adsorption capacities of 1.33 and 1.62 mmol/g for caffeic and chlorogenic acid, respectively. It was found that the adsorption mechanisms for both compounds were derived from π-π, electrostatic, and H-bonding interactions. Also, the binary adsorption equilibrium was performed, and the experimental data were interpreted using the extended multicomponent Langmuir model. The results evidenced that the binary adsorption of caffeic acid and chlorogenic acid is antagonistic in nature. Finally, the experimental adsorption rate data were interpreted by an external mass transport model and a diffusional model, finding that the overall adsorption rate is governed by intraparticle diffusion. Moreover, the surface and pore volume diffusion mechanisms were meaningful. |
| doi_str_mv | 10.1007/s11356-021-17737-3 |
| format | Article |
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The study focused on evaluating the single and binary adsorption equilibrium, as well as investigating the mass transfer resistances present during the process by applying diffusional models for a future scale-up of the process. For both compounds, the single adsorption equilibrium was studied at pH values of 3, 5, and 7. The experimental adsorption isotherms were interpreted using the Langmuir and Freundlich models, obtaining maximum adsorption capacities of 1.33 and 1.62 mmol/g for caffeic and chlorogenic acid, respectively. It was found that the adsorption mechanisms for both compounds were derived from π-π, electrostatic, and H-bonding interactions. Also, the binary adsorption equilibrium was performed, and the experimental data were interpreted using the extended multicomponent Langmuir model. The results evidenced that the binary adsorption of caffeic acid and chlorogenic acid is antagonistic in nature. Finally, the experimental adsorption rate data were interpreted by an external mass transport model and a diffusional model, finding that the overall adsorption rate is governed by intraparticle diffusion. Moreover, the surface and pore volume diffusion mechanisms were meaningful.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-021-17737-3</identifier><identifier>PMID: 34851488</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Activated carbon ; Adsorption ; Aquatic Pollution ; Aqueous solutions ; Atmospheric Protection/Air Quality Control/Air Pollution ; Caffeic acid ; Charcoal - chemistry ; Chlorogenic Acid ; Diffusion ; Diffusion rate ; Earth and Environmental Science ; Ecotoxicology ; Electrostatic properties ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Equilibrium ; Kinetics ; Mass transfer ; Mass transport ; Research Article ; Waste Water Technology ; Water Management ; Water Pollutants, Chemical - analysis ; Water Pollution Control ; Water Purification - methods</subject><ispartof>Environmental science and pollution research international, 2022-04, Vol.29 (18), p.26297-26311</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021</rights><rights>2021. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c419t-a19fc596152fd49098eb41a1622d0654025fa5e1a2d5b83ebb3625e94c5e42a83</citedby><cites>FETCH-LOGICAL-c419t-a19fc596152fd49098eb41a1622d0654025fa5e1a2d5b83ebb3625e94c5e42a83</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-021-17737-3$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-021-17737-3$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27923,27924,41487,42556,51318</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/34851488$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Hernández-Padilla, Eyden S.</creatorcontrib><creatorcontrib>Zárate-Guzmán, Ana I.</creatorcontrib><creatorcontrib>González-Ortega, Omar</creatorcontrib><creatorcontrib>Padilla-Ortega, Erika</creatorcontrib><creatorcontrib>Gómez-Durán, Azael</creatorcontrib><creatorcontrib>Delgado-Sánchez, Pablo</creatorcontrib><creatorcontrib>Aguilar-Aguilar, Angélica</creatorcontrib><creatorcontrib>Cortés, Farid B.</creatorcontrib><creatorcontrib>Ocampo-Pérez, Raúl</creatorcontrib><title>Elucidation of adsorption mechanisms and mass transfer controlling resistances during single and binary adsorption of caffeic and chlorogenic acids</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>In this work, the potential of activated carbon to remove caffeic and chlorogenic acids in aqueous solution was investigated. The study focused on evaluating the single and binary adsorption equilibrium, as well as investigating the mass transfer resistances present during the process by applying diffusional models for a future scale-up of the process. For both compounds, the single adsorption equilibrium was studied at pH values of 3, 5, and 7. The experimental adsorption isotherms were interpreted using the Langmuir and Freundlich models, obtaining maximum adsorption capacities of 1.33 and 1.62 mmol/g for caffeic and chlorogenic acid, respectively. It was found that the adsorption mechanisms for both compounds were derived from π-π, electrostatic, and H-bonding interactions. Also, the binary adsorption equilibrium was performed, and the experimental data were interpreted using the extended multicomponent Langmuir model. The results evidenced that the binary adsorption of caffeic acid and chlorogenic acid is antagonistic in nature. Finally, the experimental adsorption rate data were interpreted by an external mass transport model and a diffusional model, finding that the overall adsorption rate is governed by intraparticle diffusion. Moreover, the surface and pore volume diffusion mechanisms were meaningful.</description><subject>Activated carbon</subject><subject>Adsorption</subject><subject>Aquatic Pollution</subject><subject>Aqueous solutions</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Caffeic acid</subject><subject>Charcoal - chemistry</subject><subject>Chlorogenic Acid</subject><subject>Diffusion</subject><subject>Diffusion rate</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Electrostatic properties</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Equilibrium</subject><subject>Kinetics</subject><subject>Mass transfer</subject><subject>Mass transport</subject><subject>Research Article</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollutants, Chemical - 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Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Hernández-Padilla, Eyden S.</au><au>Zárate-Guzmán, Ana I.</au><au>González-Ortega, Omar</au><au>Padilla-Ortega, Erika</au><au>Gómez-Durán, Azael</au><au>Delgado-Sánchez, Pablo</au><au>Aguilar-Aguilar, Angélica</au><au>Cortés, Farid B.</au><au>Ocampo-Pérez, Raúl</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Elucidation of adsorption mechanisms and mass transfer controlling resistances during single and binary adsorption of caffeic and chlorogenic acids</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2022-04-01</date><risdate>2022</risdate><volume>29</volume><issue>18</issue><spage>26297</spage><epage>26311</epage><pages>26297-26311</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>In this work, the potential of activated carbon to remove caffeic and chlorogenic acids in aqueous solution was investigated. The study focused on evaluating the single and binary adsorption equilibrium, as well as investigating the mass transfer resistances present during the process by applying diffusional models for a future scale-up of the process. For both compounds, the single adsorption equilibrium was studied at pH values of 3, 5, and 7. The experimental adsorption isotherms were interpreted using the Langmuir and Freundlich models, obtaining maximum adsorption capacities of 1.33 and 1.62 mmol/g for caffeic and chlorogenic acid, respectively. It was found that the adsorption mechanisms for both compounds were derived from π-π, electrostatic, and H-bonding interactions. Also, the binary adsorption equilibrium was performed, and the experimental data were interpreted using the extended multicomponent Langmuir model. The results evidenced that the binary adsorption of caffeic acid and chlorogenic acid is antagonistic in nature. Finally, the experimental adsorption rate data were interpreted by an external mass transport model and a diffusional model, finding that the overall adsorption rate is governed by intraparticle diffusion. Moreover, the surface and pore volume diffusion mechanisms were meaningful.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>34851488</pmid><doi>10.1007/s11356-021-17737-3</doi><tpages>15</tpages><oa>free_for_read</oa></addata></record> |
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| ispartof | Environmental science and pollution research international, 2022-04, Vol.29 (18), p.26297-26311 |
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| subjects | Activated carbon Adsorption Aquatic Pollution Aqueous solutions Atmospheric Protection/Air Quality Control/Air Pollution Caffeic acid Charcoal - chemistry Chlorogenic Acid Diffusion Diffusion rate Earth and Environmental Science Ecotoxicology Electrostatic properties Environment Environmental Chemistry Environmental Health Environmental science Equilibrium Kinetics Mass transfer Mass transport Research Article Waste Water Technology Water Management Water Pollutants, Chemical - analysis Water Pollution Control Water Purification - methods |
| title | Elucidation of adsorption mechanisms and mass transfer controlling resistances during single and binary adsorption of caffeic and chlorogenic acids |
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