Programmable Self‐Regulation with Wrinkled Hydrogels and Plasmonic Nanoparticle Lattices
This paper describes a self‐regulating system that combines wrinkle‐patterned hydrogels with plasmonic nanoparticle (NP) lattices. In the feedback loop, the wrinkle patterns flatten in response to moisture, which then allows light to reach the NP lattice on the bottom layer. Upon light absorption, t...
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| Veröffentlicht in: | Small (Weinheim an der Bergstrasse, Germany) Germany), 2022-01, Vol.18 (1), p.e2103865-n/a |
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| creator | Lee, Young‐Ah Lucy Mousavikhamene, Zeynab Amrithanath, Abhishek Kottaram Neidhart, Suzanne M. Krishnaswamy, Sridhar Schatz, George C. Odom, Teri W. |
| description | This paper describes a self‐regulating system that combines wrinkle‐patterned hydrogels with plasmonic nanoparticle (NP) lattices. In the feedback loop, the wrinkle patterns flatten in response to moisture, which then allows light to reach the NP lattice on the bottom layer. Upon light absorption, the NP lattice produces a photothermal effect that dries the hydrogel, and the system then returns to the initial wrinkled configuration. The timescale of this regulatory cycle can be programmed by tuning the degree of photothermal heating by NP size and substrate material. Time‐dependent finite element analysis reveals the thermal and mechanical mechanisms of wrinkle formation. This self‐regulating system couples morphological, optical, and thermo‐mechanical properties of different materials components and offers promising design principles for future smart systems.
A self‐regulating platform combining hydrogel microwrinkles and plasmonic nanoparticle lattices can demonstrate programmable regulation with tunable timescales. The system couples the dynamic optical properties of the wrinkle patterns with moisture‐responsive mechanical actuation that can be controlled by the photothermal effect of the plasmonic lattices. |
| doi_str_mv | 10.1002/smll.202103865 |
| format | Article |
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A self‐regulating platform combining hydrogel microwrinkles and plasmonic nanoparticle lattices can demonstrate programmable regulation with tunable timescales. The system couples the dynamic optical properties of the wrinkle patterns with moisture‐responsive mechanical actuation that can be controlled by the photothermal effect of the plasmonic lattices.</description><identifier>ISSN: 1613-6810</identifier><identifier>EISSN: 1613-6829</identifier><identifier>DOI: 10.1002/smll.202103865</identifier><identifier>PMID: 34755454</identifier><language>eng</language><publisher>Germany: Wiley Subscription Services, Inc</publisher><subject>Electromagnetic absorption ; Feedback loops ; Finite element method ; Hydrogels ; Lattices ; Mechanical properties ; Nanoparticles ; Nanotechnology ; Optical properties ; Plasmonics ; Self-Control ; self‐regulation ; Skin Aging ; smart systems ; Substrates ; wrinkles</subject><ispartof>Small (Weinheim an der Bergstrasse, Germany), 2022-01, Vol.18 (1), p.e2103865-n/a</ispartof><rights>2021 Wiley‐VCH GmbH</rights><rights>2021 Wiley-VCH GmbH.</rights><rights>2022 Wiley‐VCH GmbH</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c3735-9bd6ce4f3f17836d08dd78ae39913c13937ef372a904fe04e542a2a563d334b03</citedby><cites>FETCH-LOGICAL-c3735-9bd6ce4f3f17836d08dd78ae39913c13937ef372a904fe04e542a2a563d334b03</cites><orcidid>0000-0002-3015-9149 ; 0000-0002-2167-3939 ; 0000-0002-8490-292X ; 0000-0001-5837-4740 ; 0000-0002-2125-2501</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fsmll.202103865$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fsmll.202103865$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>315,782,786,1419,27931,27932,45581,45582</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/34755454$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Lee, Young‐Ah Lucy</creatorcontrib><creatorcontrib>Mousavikhamene, Zeynab</creatorcontrib><creatorcontrib>Amrithanath, Abhishek Kottaram</creatorcontrib><creatorcontrib>Neidhart, Suzanne M.</creatorcontrib><creatorcontrib>Krishnaswamy, Sridhar</creatorcontrib><creatorcontrib>Schatz, George C.</creatorcontrib><creatorcontrib>Odom, Teri W.</creatorcontrib><title>Programmable Self‐Regulation with Wrinkled Hydrogels and Plasmonic Nanoparticle Lattices</title><title>Small (Weinheim an der Bergstrasse, Germany)</title><addtitle>Small</addtitle><description>This paper describes a self‐regulating system that combines wrinkle‐patterned hydrogels with plasmonic nanoparticle (NP) lattices. In the feedback loop, the wrinkle patterns flatten in response to moisture, which then allows light to reach the NP lattice on the bottom layer. Upon light absorption, the NP lattice produces a photothermal effect that dries the hydrogel, and the system then returns to the initial wrinkled configuration. The timescale of this regulatory cycle can be programmed by tuning the degree of photothermal heating by NP size and substrate material. Time‐dependent finite element analysis reveals the thermal and mechanical mechanisms of wrinkle formation. This self‐regulating system couples morphological, optical, and thermo‐mechanical properties of different materials components and offers promising design principles for future smart systems.
A self‐regulating platform combining hydrogel microwrinkles and plasmonic nanoparticle lattices can demonstrate programmable regulation with tunable timescales. The system couples the dynamic optical properties of the wrinkle patterns with moisture‐responsive mechanical actuation that can be controlled by the photothermal effect of the plasmonic lattices.</description><subject>Electromagnetic absorption</subject><subject>Feedback loops</subject><subject>Finite element method</subject><subject>Hydrogels</subject><subject>Lattices</subject><subject>Mechanical properties</subject><subject>Nanoparticles</subject><subject>Nanotechnology</subject><subject>Optical properties</subject><subject>Plasmonics</subject><subject>Self-Control</subject><subject>self‐regulation</subject><subject>Skin Aging</subject><subject>smart systems</subject><subject>Substrates</subject><subject>wrinkles</subject><issn>1613-6810</issn><issn>1613-6829</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkEFP2zAUgK2JaZSy644oEhcu7Ww_24mPEwKKFBgaTJN2sdz4BdI5SbETVb3xE_Yb-SWkKisSl53eO3zv09NHyBdGp4xS_jXW3k855YxCpuQHMmKKwURlXO_tdkb3yUGMC0qBcZF-IvsgUimFFCPy-ya098HWtZ17TG7Rl89Pf3_gfe9tV7VNsqq6h-RXqJo_Hl0yW7sBRx8T27jkxttYt01VJNe2aZc2dFUxSHLbDQvGQ_KxtD7i59c5Jj_Pz-5OZ5P8-8Xl6bd8UkAKcqLnThUoSihZmoFyNHMuzSyC1gwKBhpSLCHlVlNRIhUoBbfcSgUOQMwpjMnJ1rsM7WOPsTN1FQv03jbY9tFwqRVloPQGPX6HLto-NMN3hiumhiQS2EBNt1QR2hgDlmYZqtqGtWHUbKqbTXWzqz4cHL1q-3mNbof_yzwAegusKo_r_-jM7VWev8lfACfcj0g</recordid><startdate>20220101</startdate><enddate>20220101</enddate><creator>Lee, Young‐Ah Lucy</creator><creator>Mousavikhamene, Zeynab</creator><creator>Amrithanath, Abhishek Kottaram</creator><creator>Neidhart, Suzanne M.</creator><creator>Krishnaswamy, Sridhar</creator><creator>Schatz, George C.</creator><creator>Odom, Teri W.</creator><general>Wiley Subscription Services, Inc</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-3015-9149</orcidid><orcidid>https://orcid.org/0000-0002-2167-3939</orcidid><orcidid>https://orcid.org/0000-0002-8490-292X</orcidid><orcidid>https://orcid.org/0000-0001-5837-4740</orcidid><orcidid>https://orcid.org/0000-0002-2125-2501</orcidid></search><sort><creationdate>20220101</creationdate><title>Programmable Self‐Regulation with Wrinkled Hydrogels and Plasmonic Nanoparticle Lattices</title><author>Lee, Young‐Ah Lucy ; Mousavikhamene, Zeynab ; Amrithanath, Abhishek Kottaram ; Neidhart, Suzanne M. ; Krishnaswamy, Sridhar ; Schatz, George C. ; Odom, Teri W.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c3735-9bd6ce4f3f17836d08dd78ae39913c13937ef372a904fe04e542a2a563d334b03</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Electromagnetic absorption</topic><topic>Feedback loops</topic><topic>Finite element method</topic><topic>Hydrogels</topic><topic>Lattices</topic><topic>Mechanical properties</topic><topic>Nanoparticles</topic><topic>Nanotechnology</topic><topic>Optical properties</topic><topic>Plasmonics</topic><topic>Self-Control</topic><topic>self‐regulation</topic><topic>Skin Aging</topic><topic>smart systems</topic><topic>Substrates</topic><topic>wrinkles</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Lee, Young‐Ah Lucy</creatorcontrib><creatorcontrib>Mousavikhamene, Zeynab</creatorcontrib><creatorcontrib>Amrithanath, Abhishek Kottaram</creatorcontrib><creatorcontrib>Neidhart, Suzanne M.</creatorcontrib><creatorcontrib>Krishnaswamy, Sridhar</creatorcontrib><creatorcontrib>Schatz, George C.</creatorcontrib><creatorcontrib>Odom, Teri W.</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Small (Weinheim an der Bergstrasse, Germany)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lee, Young‐Ah Lucy</au><au>Mousavikhamene, Zeynab</au><au>Amrithanath, Abhishek Kottaram</au><au>Neidhart, Suzanne M.</au><au>Krishnaswamy, Sridhar</au><au>Schatz, George C.</au><au>Odom, Teri W.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Programmable Self‐Regulation with Wrinkled Hydrogels and Plasmonic Nanoparticle Lattices</atitle><jtitle>Small (Weinheim an der Bergstrasse, Germany)</jtitle><addtitle>Small</addtitle><date>2022-01-01</date><risdate>2022</risdate><volume>18</volume><issue>1</issue><spage>e2103865</spage><epage>n/a</epage><pages>e2103865-n/a</pages><issn>1613-6810</issn><eissn>1613-6829</eissn><abstract>This paper describes a self‐regulating system that combines wrinkle‐patterned hydrogels with plasmonic nanoparticle (NP) lattices. In the feedback loop, the wrinkle patterns flatten in response to moisture, which then allows light to reach the NP lattice on the bottom layer. Upon light absorption, the NP lattice produces a photothermal effect that dries the hydrogel, and the system then returns to the initial wrinkled configuration. The timescale of this regulatory cycle can be programmed by tuning the degree of photothermal heating by NP size and substrate material. Time‐dependent finite element analysis reveals the thermal and mechanical mechanisms of wrinkle formation. This self‐regulating system couples morphological, optical, and thermo‐mechanical properties of different materials components and offers promising design principles for future smart systems.
A self‐regulating platform combining hydrogel microwrinkles and plasmonic nanoparticle lattices can demonstrate programmable regulation with tunable timescales. The system couples the dynamic optical properties of the wrinkle patterns with moisture‐responsive mechanical actuation that can be controlled by the photothermal effect of the plasmonic lattices.</abstract><cop>Germany</cop><pub>Wiley Subscription Services, Inc</pub><pmid>34755454</pmid><doi>10.1002/smll.202103865</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0002-3015-9149</orcidid><orcidid>https://orcid.org/0000-0002-2167-3939</orcidid><orcidid>https://orcid.org/0000-0002-8490-292X</orcidid><orcidid>https://orcid.org/0000-0001-5837-4740</orcidid><orcidid>https://orcid.org/0000-0002-2125-2501</orcidid></addata></record> |
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| subjects | Electromagnetic absorption Feedback loops Finite element method Hydrogels Lattices Mechanical properties Nanoparticles Nanotechnology Optical properties Plasmonics Self-Control self‐regulation Skin Aging smart systems Substrates wrinkles |
| title | Programmable Self‐Regulation with Wrinkled Hydrogels and Plasmonic Nanoparticle Lattices |
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