Arsenic removal characteristics of natural Mn-Fe binary coating on waste filter sand from a water treatment facility
In this study, the arsenic (As) removal characteristics of a Mn–Fe binary coating formed on waste sand filter of an acid mine drainage treatment facility are investigated. Owing to the Mn–Fe binary coating forming on the surfaces of the sand grains, its potential for arsenic removal, particularly As...
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description | In this study, the arsenic (As) removal characteristics of a Mn–Fe binary coating formed on waste sand filter of an acid mine drainage treatment facility are investigated. Owing to the Mn–Fe binary coating forming on the surfaces of the sand grains, its potential for arsenic removal, particularly As(III), was evaluated and characterized through batch experiments and x-ray absorption spectroscopy. Sorption isotherms reveal that the Mn–Fe binary coating exhibits comparable removal efficiencies for As(III) and As(V) under low initial As concentrations. However, at higher initial As(III) and As(V) concentrations, the As(III) removal efficiency increases because of newly formed active adsorption sites from reductive dissolution of Mn. The oxidation of the As(III) and reduction of the Mn oxide phases are verified through As K-edge and Mn K-edge X-ray absorption near edge fine structure analysis. The outstanding As(III) removal efficiency of the Mn–Fe binary coating suggests synergy of Fe- and Mn-oxides, highlighting a potential application for this coating system. The natural formation of binary coating through acid mine drainage treatment reported in this study indicates that similar coating can form naturally in other environments, thus, providing plausible natural attenuation processes for arsenic immobilization. |
doi_str_mv | 10.1007/s11356-021-15580-0 |
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Owing to the Mn–Fe binary coating forming on the surfaces of the sand grains, its potential for arsenic removal, particularly As(III), was evaluated and characterized through batch experiments and x-ray absorption spectroscopy. Sorption isotherms reveal that the Mn–Fe binary coating exhibits comparable removal efficiencies for As(III) and As(V) under low initial As concentrations. However, at higher initial As(III) and As(V) concentrations, the As(III) removal efficiency increases because of newly formed active adsorption sites from reductive dissolution of Mn. The oxidation of the As(III) and reduction of the Mn oxide phases are verified through As K-edge and Mn K-edge X-ray absorption near edge fine structure analysis. The outstanding As(III) removal efficiency of the Mn–Fe binary coating suggests synergy of Fe- and Mn-oxides, highlighting a potential application for this coating system. The natural formation of binary coating through acid mine drainage treatment reported in this study indicates that similar coating can form naturally in other environments, thus, providing plausible natural attenuation processes for arsenic immobilization.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-021-15580-0</identifier><identifier>PMID: 34363167</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Absorption spectroscopy ; Acid mine drainage ; Adsorption ; Aquatic Pollution ; Arsenic ; Arsenic removal ; Atmospheric Protection/Air Quality Control/Air Pollution ; Attenuation ; Coating ; Coatings ; Drainage facilities ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Fine structure ; Immobilization ; Iron ; Manganese ; Mine drainage ; Natural attenuation ; Oxidation ; Oxidation-Reduction ; Oxides ; Pollutant removal ; Protective coatings ; Research Article ; Sand ; Sand filters ; Structural analysis ; Ultrastructure ; Waste Water Technology ; Water Management ; Water Pollutants, Chemical - analysis ; Water Pollution Control ; Water Purification ; Water treatment ; Water treatment plants ; X ray absorption ; X-ray absorption spectroscopy</subject><ispartof>Environmental science and pollution research international, 2022, Vol.29 (2), p.2136-2145</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021</rights><rights>2021. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c375t-fd845bec7e13ffb32f1ee876c9bfe2ca786404bc5f190619cb3440271842d1cc3</citedby><cites>FETCH-LOGICAL-c375t-fd845bec7e13ffb32f1ee876c9bfe2ca786404bc5f190619cb3440271842d1cc3</cites><orcidid>0000-0003-0071-2713</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-021-15580-0$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-021-15580-0$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/34363167$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Han, Young-Soo</creatorcontrib><creatorcontrib>Kim, Seol-Hee</creatorcontrib><creatorcontrib>Jang, Jeong-Yun</creatorcontrib><creatorcontrib>Ji, Sangwoo</creatorcontrib><title>Arsenic removal characteristics of natural Mn-Fe binary coating on waste filter sand from a water treatment facility</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>In this study, the arsenic (As) removal characteristics of a Mn–Fe binary coating formed on waste sand filter of an acid mine drainage treatment facility are investigated. Owing to the Mn–Fe binary coating forming on the surfaces of the sand grains, its potential for arsenic removal, particularly As(III), was evaluated and characterized through batch experiments and x-ray absorption spectroscopy. Sorption isotherms reveal that the Mn–Fe binary coating exhibits comparable removal efficiencies for As(III) and As(V) under low initial As concentrations. However, at higher initial As(III) and As(V) concentrations, the As(III) removal efficiency increases because of newly formed active adsorption sites from reductive dissolution of Mn. The oxidation of the As(III) and reduction of the Mn oxide phases are verified through As K-edge and Mn K-edge X-ray absorption near edge fine structure analysis. The outstanding As(III) removal efficiency of the Mn–Fe binary coating suggests synergy of Fe- and Mn-oxides, highlighting a potential application for this coating system. The natural formation of binary coating through acid mine drainage treatment reported in this study indicates that similar coating can form naturally in other environments, thus, providing plausible natural attenuation processes for arsenic immobilization.</description><subject>Absorption spectroscopy</subject><subject>Acid mine drainage</subject><subject>Adsorption</subject><subject>Aquatic Pollution</subject><subject>Arsenic</subject><subject>Arsenic removal</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Attenuation</subject><subject>Coating</subject><subject>Coatings</subject><subject>Drainage facilities</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Fine structure</subject><subject>Immobilization</subject><subject>Iron</subject><subject>Manganese</subject><subject>Mine drainage</subject><subject>Natural attenuation</subject><subject>Oxidation</subject><subject>Oxidation-Reduction</subject><subject>Oxides</subject><subject>Pollutant removal</subject><subject>Protective coatings</subject><subject>Research Article</subject><subject>Sand</subject><subject>Sand filters</subject><subject>Structural analysis</subject><subject>Ultrastructure</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollutants, Chemical - analysis</subject><subject>Water Pollution Control</subject><subject>Water Purification</subject><subject>Water treatment</subject><subject>Water treatment plants</subject><subject>X ray absorption</subject><subject>X-ray absorption spectroscopy</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp9kUFvFSEUhYmpsc_WP9CFIXHjBuUCM8wsm8Zqkxo3uiYM71JpZqAFxqb_Xl5faxMXXZFwvnMu3EPICfBPwLn-XABk1zMugEHXDZzxV2QDPSim1TgekA0flWIglTokb0u55lzwUeg35FAq2Uvo9YbU01wwBkczLumPnan7bbN1FXMoNbhCk6fR1jU36Xtk50inEG2-py7ZGuIVTZHe2VKR-jA3Fy02bqnPaaG2CbubmtHWBWOl3rowh3p_TF57Oxd893gekV_nX36efWOXP75enJ1eMid1V5nfDqqb0GkE6f0khQfEQfdunDwKZ_XQK64m13kYeQ-jm9pXudAwKLEF5-QR-bjPvcnpdsVSzRKKw3m2EdNajOi6UTUP8IZ--A-9TmuO7XVG9G1TbawWjRJ7yuVUSkZvbnJY2joMcLPrxOw7Ma0T89CJ2UW_f4xepwW3_yxPJTRA7oHSpHiF-Xn2C7F_AcRRl_w</recordid><startdate>2022</startdate><enddate>2022</enddate><creator>Han, Young-Soo</creator><creator>Kim, Seol-Hee</creator><creator>Jang, Jeong-Yun</creator><creator>Ji, Sangwoo</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QL</scope><scope>7SN</scope><scope>7T7</scope><scope>7TV</scope><scope>7U7</scope><scope>7WY</scope><scope>7WZ</scope><scope>7X7</scope><scope>7XB</scope><scope>87Z</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8FL</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BEZIV</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FRNLG</scope><scope>FYUFA</scope><scope>F~G</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K60</scope><scope>K6~</scope><scope>K9.</scope><scope>L.-</scope><scope>M0C</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7N</scope><scope>P64</scope><scope>PATMY</scope><scope>PQBIZ</scope><scope>PQBZA</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0003-0071-2713</orcidid></search><sort><creationdate>2022</creationdate><title>Arsenic removal characteristics of natural Mn-Fe binary coating on waste filter sand from a water treatment facility</title><author>Han, Young-Soo ; Kim, Seol-Hee ; Jang, Jeong-Yun ; Ji, Sangwoo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c375t-fd845bec7e13ffb32f1ee876c9bfe2ca786404bc5f190619cb3440271842d1cc3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Absorption spectroscopy</topic><topic>Acid mine drainage</topic><topic>Adsorption</topic><topic>Aquatic Pollution</topic><topic>Arsenic</topic><topic>Arsenic removal</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Attenuation</topic><topic>Coating</topic><topic>Coatings</topic><topic>Drainage facilities</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental science</topic><topic>Fine structure</topic><topic>Immobilization</topic><topic>Iron</topic><topic>Manganese</topic><topic>Mine drainage</topic><topic>Natural attenuation</topic><topic>Oxidation</topic><topic>Oxidation-Reduction</topic><topic>Oxides</topic><topic>Pollutant removal</topic><topic>Protective coatings</topic><topic>Research Article</topic><topic>Sand</topic><topic>Sand filters</topic><topic>Structural analysis</topic><topic>Ultrastructure</topic><topic>Waste Water Technology</topic><topic>Water Management</topic><topic>Water Pollutants, Chemical - analysis</topic><topic>Water Pollution Control</topic><topic>Water Purification</topic><topic>Water treatment</topic><topic>Water treatment plants</topic><topic>X ray absorption</topic><topic>X-ray absorption spectroscopy</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Han, Young-Soo</creatorcontrib><creatorcontrib>Kim, Seol-Hee</creatorcontrib><creatorcontrib>Jang, Jeong-Yun</creatorcontrib><creatorcontrib>Ji, Sangwoo</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Bacteriology Abstracts (Microbiology B)</collection><collection>Ecology Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>Access via ABI/INFORM (ProQuest)</collection><collection>ABI/INFORM Global (PDF only)</collection><collection>Health & Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>ABI/INFORM Global (Alumni Edition)</collection><collection>Medical Database (Alumni Edition)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest Pharma Collection</collection><collection>Public Health Database</collection><collection>Technology Research Database</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>ABI/INFORM Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>Agricultural & Environmental Science Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Business Premium Collection</collection><collection>Natural Science Collection</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>Engineering Research Database</collection><collection>Business Premium Collection (Alumni)</collection><collection>Health Research Premium Collection</collection><collection>ABI/INFORM Global (Corporate)</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Business Collection (Alumni Edition)</collection><collection>ProQuest Business Collection</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>ABI/INFORM Professional Advanced</collection><collection>ABI/INFORM Global</collection><collection>Health & Medical Collection (Alumni Edition)</collection><collection>Medical Database</collection><collection>Science Database</collection><collection>Algology Mycology and Protozoology Abstracts (Microbiology C)</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Environmental Science Database</collection><collection>ProQuest One Business</collection><collection>ProQuest One Business (Alumni)</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Environmental Science Collection</collection><collection>ProQuest Central Basic</collection><collection>MEDLINE - Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Han, Young-Soo</au><au>Kim, Seol-Hee</au><au>Jang, Jeong-Yun</au><au>Ji, Sangwoo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Arsenic removal characteristics of natural Mn-Fe binary coating on waste filter sand from a water treatment facility</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2022</date><risdate>2022</risdate><volume>29</volume><issue>2</issue><spage>2136</spage><epage>2145</epage><pages>2136-2145</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>In this study, the arsenic (As) removal characteristics of a Mn–Fe binary coating formed on waste sand filter of an acid mine drainage treatment facility are investigated. Owing to the Mn–Fe binary coating forming on the surfaces of the sand grains, its potential for arsenic removal, particularly As(III), was evaluated and characterized through batch experiments and x-ray absorption spectroscopy. Sorption isotherms reveal that the Mn–Fe binary coating exhibits comparable removal efficiencies for As(III) and As(V) under low initial As concentrations. However, at higher initial As(III) and As(V) concentrations, the As(III) removal efficiency increases because of newly formed active adsorption sites from reductive dissolution of Mn. The oxidation of the As(III) and reduction of the Mn oxide phases are verified through As K-edge and Mn K-edge X-ray absorption near edge fine structure analysis. The outstanding As(III) removal efficiency of the Mn–Fe binary coating suggests synergy of Fe- and Mn-oxides, highlighting a potential application for this coating system. The natural formation of binary coating through acid mine drainage treatment reported in this study indicates that similar coating can form naturally in other environments, thus, providing plausible natural attenuation processes for arsenic immobilization.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>34363167</pmid><doi>10.1007/s11356-021-15580-0</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0003-0071-2713</orcidid></addata></record> |
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subjects | Absorption spectroscopy Acid mine drainage Adsorption Aquatic Pollution Arsenic Arsenic removal Atmospheric Protection/Air Quality Control/Air Pollution Attenuation Coating Coatings Drainage facilities Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental science Fine structure Immobilization Iron Manganese Mine drainage Natural attenuation Oxidation Oxidation-Reduction Oxides Pollutant removal Protective coatings Research Article Sand Sand filters Structural analysis Ultrastructure Waste Water Technology Water Management Water Pollutants, Chemical - analysis Water Pollution Control Water Purification Water treatment Water treatment plants X ray absorption X-ray absorption spectroscopy |
title | Arsenic removal characteristics of natural Mn-Fe binary coating on waste filter sand from a water treatment facility |
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