Occurrence, distribution and risk assessment of organophosphate ester flame retardants and plasticizers in surface seawater of the West Pacific
Twenty-eight samples of surface seawater were collected from the West Pacific Ocean during 2019 using a high-volume solid-phase extraction with high-throughput organic analysis (Hi-throat/Hi-volume SPE) method, and concentrations of 10 organophosphate ester flame retardants and plasticizers (OPEs) w...
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| Veröffentlicht in: | Marine pollution bulletin 2021-09, Vol.170, p.112691-112691, Article 112691 |
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| container_title | Marine pollution bulletin |
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| creator | Xiao, Kaiyan Lu, Zhibo Yang, Chao Zhao, Song Zheng, Hongyuan Gao, Yuan Kaluwin, Chalapan Liu, Yanguang Cai, Minghong |
| description | Twenty-eight samples of surface seawater were collected from the West Pacific Ocean during 2019 using a high-volume solid-phase extraction with high-throughput organic analysis (Hi-throat/Hi-volume SPE) method, and concentrations of 10 organophosphate ester flame retardants and plasticizers (OPEs) were determined. The total OPE concentration in the samples was 3.02–48.4 ng L−1 (mean 25.0 ± 10.5 ng L−1), with tris(2-chloroethyl) phosphate (TCEP) being the largest contributor. Cluster analysis results showed off-shore input from the coast of East and Southeast Asia was an important source of these chemicals. Tri-p-tolyl phosphate (TpTP) should also be considered for long-term monitoring, because of its high detection frequency. Results of a risk assessment indicated low ecological risk to species in the West Pacific Ocean for TPhP and ΣOPEs. Hazard quotients (HQs) were all |
| doi_str_mv | 10.1016/j.marpolbul.2021.112691 |
| format | Article |
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[Display omitted]
•Hi-throat/Hi-volume SPE was applied to analyse 10 OPEs in seawater.•Distribution of OPEs in the West Pacific Ocean was investigated.•Off-shore input was a major source for OPEs in the West Pacific Ocean.•Ecological risk of OPEs in the West Pacific Ocean was evaluated at a low level.</description><identifier>ISSN: 0025-326X</identifier><identifier>EISSN: 1879-3363</identifier><identifier>DOI: 10.1016/j.marpolbul.2021.112691</identifier><language>eng</language><publisher>Oxford: Elsevier Ltd</publisher><subject>Chemical analysis ; Chemicals ; Cluster analysis ; Ecological effects ; Ecological risk assessment ; Environmental risk ; Flame retardants ; Health risks ; High-volume solid-phase extraction with high-throughput organic analysis method ; Organophosphate ester flame retardants and plasticizers ; Organophosphates ; Phosphates ; Plasticizers ; Quotients ; Risk ; Risk assessment ; Seawater ; Solid phases ; The West Pacific Ocean ; Water analysis</subject><ispartof>Marine pollution bulletin, 2021-09, Vol.170, p.112691-112691, Article 112691</ispartof><rights>2021 Elsevier Ltd</rights><rights>Copyright Elsevier BV Sep 2021</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c376t-434b6ab8e9dcb80d53d37f273cf45ca194e80fff549c42bb3ccb4d5f246e4e073</citedby><cites>FETCH-LOGICAL-c376t-434b6ab8e9dcb80d53d37f273cf45ca194e80fff549c42bb3ccb4d5f246e4e073</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.marpolbul.2021.112691$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,777,781,3537,27905,27906,45976</link.rule.ids></links><search><creatorcontrib>Xiao, Kaiyan</creatorcontrib><creatorcontrib>Lu, Zhibo</creatorcontrib><creatorcontrib>Yang, Chao</creatorcontrib><creatorcontrib>Zhao, Song</creatorcontrib><creatorcontrib>Zheng, Hongyuan</creatorcontrib><creatorcontrib>Gao, Yuan</creatorcontrib><creatorcontrib>Kaluwin, Chalapan</creatorcontrib><creatorcontrib>Liu, Yanguang</creatorcontrib><creatorcontrib>Cai, Minghong</creatorcontrib><title>Occurrence, distribution and risk assessment of organophosphate ester flame retardants and plasticizers in surface seawater of the West Pacific</title><title>Marine pollution bulletin</title><description>Twenty-eight samples of surface seawater were collected from the West Pacific Ocean during 2019 using a high-volume solid-phase extraction with high-throughput organic analysis (Hi-throat/Hi-volume SPE) method, and concentrations of 10 organophosphate ester flame retardants and plasticizers (OPEs) were determined. The total OPE concentration in the samples was 3.02–48.4 ng L−1 (mean 25.0 ± 10.5 ng L−1), with tris(2-chloroethyl) phosphate (TCEP) being the largest contributor. Cluster analysis results showed off-shore input from the coast of East and Southeast Asia was an important source of these chemicals. Tri-p-tolyl phosphate (TpTP) should also be considered for long-term monitoring, because of its high detection frequency. Results of a risk assessment indicated low ecological risk to species in the West Pacific Ocean for TPhP and ΣOPEs. Hazard quotients (HQs) were all <1, indicating that the health risk to humans from these chemicals was at acceptable levels.
[Display omitted]
•Hi-throat/Hi-volume SPE was applied to analyse 10 OPEs in seawater.•Distribution of OPEs in the West Pacific Ocean was investigated.•Off-shore input was a major source for OPEs in the West Pacific Ocean.•Ecological risk of OPEs in the West Pacific Ocean was evaluated at a low level.</description><subject>Chemical analysis</subject><subject>Chemicals</subject><subject>Cluster analysis</subject><subject>Ecological effects</subject><subject>Ecological risk assessment</subject><subject>Environmental risk</subject><subject>Flame retardants</subject><subject>Health risks</subject><subject>High-volume solid-phase extraction with high-throughput organic analysis method</subject><subject>Organophosphate ester flame retardants and plasticizers</subject><subject>Organophosphates</subject><subject>Phosphates</subject><subject>Plasticizers</subject><subject>Quotients</subject><subject>Risk</subject><subject>Risk assessment</subject><subject>Seawater</subject><subject>Solid phases</subject><subject>The West Pacific Ocean</subject><subject>Water analysis</subject><issn>0025-326X</issn><issn>1879-3363</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNqFkU1v1DAQhiMEEkvhN2CJCwey-CtxfKwqvqRK5dCq3CzHHrNesnHwOCD4E_xlvN2KA5ee5vK8r2bmaZqXjG4ZZf3b_fZg85KmcZ22nHK2ZYz3mj1qNmxQuhWiF4-bDaW8awXvvzxtniHuKaWKK7Zp_lw5t-YMs4M3xEcsOY5riWkmdvYkR_xGLCIgHmAuJAWS8lc7p2WXcNnZAgSwQCZhsgcgGYrN3s4F79LLZLFEF39DRhJngmsO1gFBsD_tMVXryg7Ibe0gn62LIbrnzZNgJ4QX9_OsuXn_7vriY3t59eHTxfll64TqSyuFHHs7DqC9GwfqO-GFClwJF2TnLNMSBhpC6KR2ko-jcG6Uvgtc9iCBKnHWvD71Ljl9X-sC5hDRwTTZGdKKhndy0EyKQVf01X_oPq15rttVqtf110r3lVInyuWEmCGYJcdq5pdh1BxFmb35J8ocRZmTqJo8PyWh3vsjQjbo4lGIjxlcMT7FBzv-ArIVpHc</recordid><startdate>202109</startdate><enddate>202109</enddate><creator>Xiao, Kaiyan</creator><creator>Lu, Zhibo</creator><creator>Yang, Chao</creator><creator>Zhao, Song</creator><creator>Zheng, Hongyuan</creator><creator>Gao, Yuan</creator><creator>Kaluwin, Chalapan</creator><creator>Liu, Yanguang</creator><creator>Cai, Minghong</creator><general>Elsevier Ltd</general><general>Elsevier BV</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7ST</scope><scope>7T7</scope><scope>7TN</scope><scope>7TV</scope><scope>7U7</scope><scope>8FD</scope><scope>C1K</scope><scope>F1W</scope><scope>FR3</scope><scope>M7N</scope><scope>P64</scope><scope>SOI</scope><scope>7X8</scope></search><sort><creationdate>202109</creationdate><title>Occurrence, distribution and risk assessment of organophosphate ester flame retardants and plasticizers in surface seawater of the West Pacific</title><author>Xiao, Kaiyan ; Lu, Zhibo ; Yang, Chao ; Zhao, Song ; Zheng, Hongyuan ; Gao, Yuan ; Kaluwin, Chalapan ; Liu, Yanguang ; Cai, Minghong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c376t-434b6ab8e9dcb80d53d37f273cf45ca194e80fff549c42bb3ccb4d5f246e4e073</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Chemical analysis</topic><topic>Chemicals</topic><topic>Cluster analysis</topic><topic>Ecological effects</topic><topic>Ecological risk assessment</topic><topic>Environmental risk</topic><topic>Flame retardants</topic><topic>Health risks</topic><topic>High-volume solid-phase extraction with high-throughput organic analysis method</topic><topic>Organophosphate ester flame retardants and plasticizers</topic><topic>Organophosphates</topic><topic>Phosphates</topic><topic>Plasticizers</topic><topic>Quotients</topic><topic>Risk</topic><topic>Risk assessment</topic><topic>Seawater</topic><topic>Solid phases</topic><topic>The West Pacific Ocean</topic><topic>Water analysis</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Xiao, Kaiyan</creatorcontrib><creatorcontrib>Lu, Zhibo</creatorcontrib><creatorcontrib>Yang, Chao</creatorcontrib><creatorcontrib>Zhao, Song</creatorcontrib><creatorcontrib>Zheng, Hongyuan</creatorcontrib><creatorcontrib>Gao, Yuan</creatorcontrib><creatorcontrib>Kaluwin, Chalapan</creatorcontrib><creatorcontrib>Liu, Yanguang</creatorcontrib><creatorcontrib>Cai, Minghong</creatorcontrib><collection>CrossRef</collection><collection>Environment Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Oceanic Abstracts</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Engineering Research Database</collection><collection>Algology Mycology and Protozoology Abstracts (Microbiology C)</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Environment Abstracts</collection><collection>MEDLINE - Academic</collection><jtitle>Marine pollution bulletin</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Xiao, Kaiyan</au><au>Lu, Zhibo</au><au>Yang, Chao</au><au>Zhao, Song</au><au>Zheng, Hongyuan</au><au>Gao, Yuan</au><au>Kaluwin, Chalapan</au><au>Liu, Yanguang</au><au>Cai, Minghong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Occurrence, distribution and risk assessment of organophosphate ester flame retardants and plasticizers in surface seawater of the West Pacific</atitle><jtitle>Marine pollution bulletin</jtitle><date>2021-09</date><risdate>2021</risdate><volume>170</volume><spage>112691</spage><epage>112691</epage><pages>112691-112691</pages><artnum>112691</artnum><issn>0025-326X</issn><eissn>1879-3363</eissn><abstract>Twenty-eight samples of surface seawater were collected from the West Pacific Ocean during 2019 using a high-volume solid-phase extraction with high-throughput organic analysis (Hi-throat/Hi-volume SPE) method, and concentrations of 10 organophosphate ester flame retardants and plasticizers (OPEs) were determined. The total OPE concentration in the samples was 3.02–48.4 ng L−1 (mean 25.0 ± 10.5 ng L−1), with tris(2-chloroethyl) phosphate (TCEP) being the largest contributor. Cluster analysis results showed off-shore input from the coast of East and Southeast Asia was an important source of these chemicals. Tri-p-tolyl phosphate (TpTP) should also be considered for long-term monitoring, because of its high detection frequency. Results of a risk assessment indicated low ecological risk to species in the West Pacific Ocean for TPhP and ΣOPEs. Hazard quotients (HQs) were all <1, indicating that the health risk to humans from these chemicals was at acceptable levels.
[Display omitted]
•Hi-throat/Hi-volume SPE was applied to analyse 10 OPEs in seawater.•Distribution of OPEs in the West Pacific Ocean was investigated.•Off-shore input was a major source for OPEs in the West Pacific Ocean.•Ecological risk of OPEs in the West Pacific Ocean was evaluated at a low level.</abstract><cop>Oxford</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.marpolbul.2021.112691</doi><tpages>1</tpages></addata></record> |
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| subjects | Chemical analysis Chemicals Cluster analysis Ecological effects Ecological risk assessment Environmental risk Flame retardants Health risks High-volume solid-phase extraction with high-throughput organic analysis method Organophosphate ester flame retardants and plasticizers Organophosphates Phosphates Plasticizers Quotients Risk Risk assessment Seawater Solid phases The West Pacific Ocean Water analysis |
| title | Occurrence, distribution and risk assessment of organophosphate ester flame retardants and plasticizers in surface seawater of the West Pacific |
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