High-harmonic-driven inverse Raman scattering
Spectral analysis of high-order harmonics generated by ultrashort mid-infrared pulses in molecular nitrogen reveals well-resolved signatures of inverse Raman scattering, showing up near the frequencies of prominent vibrational transitions of nitrogen molecules. When tuned on a resonance with the v ′...
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| Veröffentlicht in: | Optics letters 2021-07, Vol.46 (13), p.3219-3222 |
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| container_title | Optics letters |
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| creator | Mitrofanov, A. V. Rozhko, M. V. Voronin, A. A. Sidorov-Biryukov, D. A. Fedotov, A. B. Zheltikov, A. M. |
| description | Spectral analysis of high-order harmonics generated by ultrashort mid-infrared pulses in molecular nitrogen reveals well-resolved signatures of inverse Raman scattering, showing up near the frequencies of prominent vibrational transitions of nitrogen molecules. When tuned on a resonance with the v ′ = 0 → v ′ ′ = 0 pathway within the B 3 Π g → C 3 Π u second positive system of molecular nitrogen, the eleventh harmonic of a 3.9 µm, 80 fs driver is shown to acquire a distinctive antisymmetric spectral profile with red-shifted bright and blue-shifted dark features as indicators of stimulated Raman gain and loss. This high-harmonic setting extends the inverse Raman effect to a vast class of strong-field light–matter interaction scenarios. |
| doi_str_mv | 10.1364/OL.419790 |
| format | Article |
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This high-harmonic setting extends the inverse Raman effect to a vast class of strong-field light–matter interaction scenarios.</description><subject>Blue shift</subject><subject>Higher harmonics</subject><subject>Infrared analysis</subject><subject>Infrared signatures</subject><subject>Nitrogen</subject><subject>Raman spectra</subject><subject>Spectrum analysis</subject><issn>0146-9592</issn><issn>1539-4794</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><recordid>eNpd0M1KAzEUBeAgCtbqwjcouNFFav4zWUpRKwwURNfhzsydNqWTqcm04Ns7Uleuzubj3Msh5JazOZdGPa7KueLOOnZGJlxLR5V16pxMGFeGOu3EJbnKecsYM1bKCaHLsN7QDaSuj6GmTQpHjLMQj5gyzt6hgzjLNQwDphDX1-SihV3Gm7-cks-X54_Fkpar17fFU0lr4dhAG8vHAyCgqoWQrFDCOFRKyEKgEljZCoBVDUiEFpAZ2VjROtUwWxRCSiun5P7Uu0_91wHz4LuQa9ztIGJ_yF5oVSgujNYjvftHt_0hxfG7UWmpjS14MaqHk6pTn3PC1u9T6CB9e87873B-VfrTcPIHzNldrg</recordid><startdate>20210701</startdate><enddate>20210701</enddate><creator>Mitrofanov, A. 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| ispartof | Optics letters, 2021-07, Vol.46 (13), p.3219-3222 |
| issn | 0146-9592 1539-4794 |
| language | eng |
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| source | Optica Publishing Group Journals |
| subjects | Blue shift Higher harmonics Infrared analysis Infrared signatures Nitrogen Raman spectra Spectrum analysis |
| title | High-harmonic-driven inverse Raman scattering |
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