Laser-Driven Growth of Semiconductor Nanowires from Colloidal Nanocrystals
Semiconductor nanowire production through vapor- and solution-based processes has propelled nanowire systems toward a wide range of technological applications. Although vapor-based nanowire syntheses enable precise control over nanowire composition and phase, they typically employ batch processes wi...
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Veröffentlicht in: | ACS nano 2021-05, Vol.15 (5), p.8653-8662 |
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creator | Pandres, Elena P Crane, Matthew J Davis, E. James Pauzauskie, Peter J Holmberg, Vincent C |
description | Semiconductor nanowire production through vapor- and solution-based processes has propelled nanowire systems toward a wide range of technological applications. Although vapor-based nanowire syntheses enable precise control over nanowire composition and phase, they typically employ batch processes with specialized pressure management systems, limiting throughput. Solution-based nanowire growth processes have improved scalability but can require even more extensive pressure and temperature management systems. Here, we demonstrate a solution-based nanowire growth process that utilizes the large Young–Laplace interfacial surface pressures and collective heating effects of colloidal metal nanocrystals under irradiation to drive nanowire growth photothermally. Laser irradiation of a solution containing metal nanocrystals and semiconductor precursors facilitates rapid heating, precursor decomposition, and nanowire growth on a benchtop in simple glassware under standard conditions, potentially enabling a range of solution-based experiments including in-line combinatorial identification of optimized reaction parameters, in situ measurements, and the production of nanowires with complex compositions. |
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Here, we demonstrate a solution-based nanowire growth process that utilizes the large Young–Laplace interfacial surface pressures and collective heating effects of colloidal metal nanocrystals under irradiation to drive nanowire growth photothermally. Laser irradiation of a solution containing metal nanocrystals and semiconductor precursors facilitates rapid heating, precursor decomposition, and nanowire growth on a benchtop in simple glassware under standard conditions, potentially enabling a range of solution-based experiments including in-line combinatorial identification of optimized reaction parameters, in situ measurements, and the production of nanowires with complex compositions.</abstract><cop>United States</cop><pub>American Chemical Society</pub><pmid>33950682</pmid><doi>10.1021/acsnano.1c00683</doi><tpages>10</tpages><orcidid>https://orcid.org/0000-0001-8461-4808</orcidid><orcidid>https://orcid.org/0000-0003-1435-5614</orcidid><orcidid>https://orcid.org/0000-0002-9591-8951</orcidid><orcidid>https://orcid.org/0000-0002-1554-5949</orcidid></addata></record> |
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title | Laser-Driven Growth of Semiconductor Nanowires from Colloidal Nanocrystals |
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