Fe‐O Clusters Anchored on Nodes of Metal–Organic Frameworks for Direct Methane Oxidation

Direct methane oxidation into value‐added organic oxygenates with high productivity under mild condition remains a great challenge. We show Fe‐O clusters on nodes of metal–organic frameworks (MOFs) with tunable electronic state for direct methane oxidation into C1 organic oxygenates at 50 °C. The Fe...

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Veröffentlicht in:	Angewandte Chemie International Edition 2021-03, Vol.60 (11), p.5811-5815
Hauptverfasser:	Zhao, Wenshi, Shi, Yanan, Jiang, Yuheng, Zhang, Xiaofei, Long, Chang, An, Pengfei, Zhu, Yanfei, Shao, Shengxian, Yan, Zhuang, Li, Guodong, Tang, Zhiyong
Format:	Artikel
Sprache:	eng
Schlagworte:	Acetic acid C1 oxygenates Clusters Electron states Hydrogen bonds Iron Metal-organic frameworks Methane Modulators Nodes Oxidation Selectivity Terephthalic acid Trifluoroacetic acid Valence
Online-Zugang:	Volltext
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