Identifying the Active Site on Graphene Oxide Nanosheets for Ambient Electrocatalytic Nitrogen Reduction
Identifying the active sites on graphene oxide (GO) nanosheets is of great importance. In situ electroreduction at different potentials is applied to control the oxygenated groups on GO surfaces. Both experiments and theoretical calculations suggest the CO group is critical for N2 adsorption and ac...
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| Veröffentlicht in: | Inorganic chemistry 2020-08, Vol.59 (15), p.11108-11112 |
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| container_end_page | 11112 |
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| container_issue | 15 |
| container_start_page | 11108 |
| container_title | Inorganic chemistry |
| container_volume | 59 |
| creator | Wang, Sini Zhu, Jingjing Zhang, Yicheng Liu, Qiangchun Chen, Guilin Kong, Xiangkai |
| description | Identifying the active sites on graphene oxide (GO) nanosheets is of great importance. In situ electroreduction at different potentials is applied to control the oxygenated groups on GO surfaces. Both experiments and theoretical calculations suggest the CO group is critical for N2 adsorption and activation, guaranteeing the ambient electrocatalytic N2 reduction. |
| doi_str_mv | 10.1021/acs.inorgchem.0c01596 |
| format | Article |
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| title | Identifying the Active Site on Graphene Oxide Nanosheets for Ambient Electrocatalytic Nitrogen Reduction |
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