Synthesis of Pt-Loaded NiFe-LDH Nanosheets on Wood Veneer for Efficient Gaseous Formaldehyde Degradation

Traditional methods of removing gaseous formaldehyde are often associated with high energy consumption and secondary pollution. In this study, a new wood veneer-based composite decorated with Pt-loaded NiFe-LDH nanosheets is successfully developed by a hydrothermal reaction and impregnation-chemical...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:ACS applied materials & interfaces 2020-08, Vol.12 (33), p.37147-37154
Hauptverfasser: Cai, Tailong, Zhang, Ping, Shen, Xiaoyuan, Huang, Erzhuo, Shen, Xiaoping, Shi, Jiangtao, Wang, Zhe, Sun, Qingfeng
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 37154
container_issue 33
container_start_page 37147
container_title ACS applied materials & interfaces
container_volume 12
creator Cai, Tailong
Zhang, Ping
Shen, Xiaoyuan
Huang, Erzhuo
Shen, Xiaoping
Shi, Jiangtao
Wang, Zhe
Sun, Qingfeng
description Traditional methods of removing gaseous formaldehyde are often associated with high energy consumption and secondary pollution. In this study, a new wood veneer-based composite decorated with Pt-loaded NiFe-LDH nanosheets is successfully developed by a hydrothermal reaction and impregnation-chemical reduction. NiFe-LDH nanosheets as an adsorbent can capture formaldehyde molecules through their abundant hydroxyl groups. Pt nanoparticles as catalytic centers are evenly distributed on the surface of NiFe-LDH to excite the O atoms linked to NiFe-LDH and absorbed oxygen, which will further attack the absorbed formaldehyde molecules to generate CO2 and H2O. And the wood veneer not only increases the active area of the catalyst by endowing it with good dispersion but also provides convenient channels for reactants and products. In a simulated dark environment at room temperature, this synthetic wood veneer-based composite exhibits admirable catalytic activity, which can effectively degrade almost all gaseous formaldehyde with the initial concentration of 0.2 mg m–3 in 30 min and maintain a high catalytic activity of ≥97% after 10 cycles. This paper presents a feasible strategy for synthesizing an energy-efficient and ecofriendly wood veneer-based composite for efficient gaseous formaldehyde degradation at room temperature, which may play an important role in indoor air purification as a promising decorative material.
doi_str_mv 10.1021/acsami.0c09016
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_2425895860</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2425895860</sourcerecordid><originalsourceid>FETCH-LOGICAL-a307t-20d80ad61094d8d8b49e8e370bd3b215e11e2d1ea6e0f197db3434dbf9d27faf3</originalsourceid><addsrcrecordid>eNp1kD1PwzAQhi0EEqWwMntESCm243yNqKUtUlSQ-BotJz4TV4ld7HTovydVKjamO52e93T3IHRLyYwSRh9kHWRnZqQmBaHpGZrQgvMoZwk7_-s5v0RXIWwJSWNGkglq3g62byCYgJ3Gr31UOqlA4Y1ZQlQu1ngjrQsNQD8AFn85p_AnWACPtfP4SWtTG7A9XskAbh_w0vlOtgqagwK8gG8vleyNs9foQss2wM2pTtHH8ul9vo7Kl9Xz_LGMZEyyPmJE5USqlJKCq1zlFS8ghzgjlYorRhOgFJiiIFMgmhaZqmIec1XpQrFMSx1P0d24d-fdzx5CLzoTamhbaY_3CcZZkhdJnpIBnY1o7V0IHrTYedNJfxCUiKNSMSoVJ6VD4H4MDHOxdXtvh0_-g38BFEN5UQ</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2425895860</pqid></control><display><type>article</type><title>Synthesis of Pt-Loaded NiFe-LDH Nanosheets on Wood Veneer for Efficient Gaseous Formaldehyde Degradation</title><source>ACS Publications</source><creator>Cai, Tailong ; Zhang, Ping ; Shen, Xiaoyuan ; Huang, Erzhuo ; Shen, Xiaoping ; Shi, Jiangtao ; Wang, Zhe ; Sun, Qingfeng</creator><creatorcontrib>Cai, Tailong ; Zhang, Ping ; Shen, Xiaoyuan ; Huang, Erzhuo ; Shen, Xiaoping ; Shi, Jiangtao ; Wang, Zhe ; Sun, Qingfeng</creatorcontrib><description>Traditional methods of removing gaseous formaldehyde are often associated with high energy consumption and secondary pollution. In this study, a new wood veneer-based composite decorated with Pt-loaded NiFe-LDH nanosheets is successfully developed by a hydrothermal reaction and impregnation-chemical reduction. NiFe-LDH nanosheets as an adsorbent can capture formaldehyde molecules through their abundant hydroxyl groups. Pt nanoparticles as catalytic centers are evenly distributed on the surface of NiFe-LDH to excite the O atoms linked to NiFe-LDH and absorbed oxygen, which will further attack the absorbed formaldehyde molecules to generate CO2 and H2O. And the wood veneer not only increases the active area of the catalyst by endowing it with good dispersion but also provides convenient channels for reactants and products. In a simulated dark environment at room temperature, this synthetic wood veneer-based composite exhibits admirable catalytic activity, which can effectively degrade almost all gaseous formaldehyde with the initial concentration of 0.2 mg m–3 in 30 min and maintain a high catalytic activity of ≥97% after 10 cycles. This paper presents a feasible strategy for synthesizing an energy-efficient and ecofriendly wood veneer-based composite for efficient gaseous formaldehyde degradation at room temperature, which may play an important role in indoor air purification as a promising decorative material.</description><identifier>ISSN: 1944-8244</identifier><identifier>EISSN: 1944-8252</identifier><identifier>DOI: 10.1021/acsami.0c09016</identifier><language>eng</language><publisher>American Chemical Society</publisher><subject>Energy, Environmental, and Catalysis Applications</subject><ispartof>ACS applied materials &amp; interfaces, 2020-08, Vol.12 (33), p.37147-37154</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a307t-20d80ad61094d8d8b49e8e370bd3b215e11e2d1ea6e0f197db3434dbf9d27faf3</citedby><cites>FETCH-LOGICAL-a307t-20d80ad61094d8d8b49e8e370bd3b215e11e2d1ea6e0f197db3434dbf9d27faf3</cites><orcidid>0000-0003-3520-4970</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acsami.0c09016$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acsami.0c09016$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,776,780,2752,27053,27901,27902,56713,56763</link.rule.ids></links><search><creatorcontrib>Cai, Tailong</creatorcontrib><creatorcontrib>Zhang, Ping</creatorcontrib><creatorcontrib>Shen, Xiaoyuan</creatorcontrib><creatorcontrib>Huang, Erzhuo</creatorcontrib><creatorcontrib>Shen, Xiaoping</creatorcontrib><creatorcontrib>Shi, Jiangtao</creatorcontrib><creatorcontrib>Wang, Zhe</creatorcontrib><creatorcontrib>Sun, Qingfeng</creatorcontrib><title>Synthesis of Pt-Loaded NiFe-LDH Nanosheets on Wood Veneer for Efficient Gaseous Formaldehyde Degradation</title><title>ACS applied materials &amp; interfaces</title><addtitle>ACS Appl. Mater. Interfaces</addtitle><description>Traditional methods of removing gaseous formaldehyde are often associated with high energy consumption and secondary pollution. In this study, a new wood veneer-based composite decorated with Pt-loaded NiFe-LDH nanosheets is successfully developed by a hydrothermal reaction and impregnation-chemical reduction. NiFe-LDH nanosheets as an adsorbent can capture formaldehyde molecules through their abundant hydroxyl groups. Pt nanoparticles as catalytic centers are evenly distributed on the surface of NiFe-LDH to excite the O atoms linked to NiFe-LDH and absorbed oxygen, which will further attack the absorbed formaldehyde molecules to generate CO2 and H2O. And the wood veneer not only increases the active area of the catalyst by endowing it with good dispersion but also provides convenient channels for reactants and products. In a simulated dark environment at room temperature, this synthetic wood veneer-based composite exhibits admirable catalytic activity, which can effectively degrade almost all gaseous formaldehyde with the initial concentration of 0.2 mg m–3 in 30 min and maintain a high catalytic activity of ≥97% after 10 cycles. This paper presents a feasible strategy for synthesizing an energy-efficient and ecofriendly wood veneer-based composite for efficient gaseous formaldehyde degradation at room temperature, which may play an important role in indoor air purification as a promising decorative material.</description><subject>Energy, Environmental, and Catalysis Applications</subject><issn>1944-8244</issn><issn>1944-8252</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><recordid>eNp1kD1PwzAQhi0EEqWwMntESCm243yNqKUtUlSQ-BotJz4TV4ld7HTovydVKjamO52e93T3IHRLyYwSRh9kHWRnZqQmBaHpGZrQgvMoZwk7_-s5v0RXIWwJSWNGkglq3g62byCYgJ3Gr31UOqlA4Y1ZQlQu1ngjrQsNQD8AFn85p_AnWACPtfP4SWtTG7A9XskAbh_w0vlOtgqagwK8gG8vleyNs9foQss2wM2pTtHH8ul9vo7Kl9Xz_LGMZEyyPmJE5USqlJKCq1zlFS8ghzgjlYorRhOgFJiiIFMgmhaZqmIec1XpQrFMSx1P0d24d-fdzx5CLzoTamhbaY_3CcZZkhdJnpIBnY1o7V0IHrTYedNJfxCUiKNSMSoVJ6VD4H4MDHOxdXtvh0_-g38BFEN5UQ</recordid><startdate>20200819</startdate><enddate>20200819</enddate><creator>Cai, Tailong</creator><creator>Zhang, Ping</creator><creator>Shen, Xiaoyuan</creator><creator>Huang, Erzhuo</creator><creator>Shen, Xiaoping</creator><creator>Shi, Jiangtao</creator><creator>Wang, Zhe</creator><creator>Sun, Qingfeng</creator><general>American Chemical Society</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0003-3520-4970</orcidid></search><sort><creationdate>20200819</creationdate><title>Synthesis of Pt-Loaded NiFe-LDH Nanosheets on Wood Veneer for Efficient Gaseous Formaldehyde Degradation</title><author>Cai, Tailong ; Zhang, Ping ; Shen, Xiaoyuan ; Huang, Erzhuo ; Shen, Xiaoping ; Shi, Jiangtao ; Wang, Zhe ; Sun, Qingfeng</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a307t-20d80ad61094d8d8b49e8e370bd3b215e11e2d1ea6e0f197db3434dbf9d27faf3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Energy, Environmental, and Catalysis Applications</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Cai, Tailong</creatorcontrib><creatorcontrib>Zhang, Ping</creatorcontrib><creatorcontrib>Shen, Xiaoyuan</creatorcontrib><creatorcontrib>Huang, Erzhuo</creatorcontrib><creatorcontrib>Shen, Xiaoping</creatorcontrib><creatorcontrib>Shi, Jiangtao</creatorcontrib><creatorcontrib>Wang, Zhe</creatorcontrib><creatorcontrib>Sun, Qingfeng</creatorcontrib><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>ACS applied materials &amp; interfaces</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Cai, Tailong</au><au>Zhang, Ping</au><au>Shen, Xiaoyuan</au><au>Huang, Erzhuo</au><au>Shen, Xiaoping</au><au>Shi, Jiangtao</au><au>Wang, Zhe</au><au>Sun, Qingfeng</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Synthesis of Pt-Loaded NiFe-LDH Nanosheets on Wood Veneer for Efficient Gaseous Formaldehyde Degradation</atitle><jtitle>ACS applied materials &amp; interfaces</jtitle><addtitle>ACS Appl. Mater. Interfaces</addtitle><date>2020-08-19</date><risdate>2020</risdate><volume>12</volume><issue>33</issue><spage>37147</spage><epage>37154</epage><pages>37147-37154</pages><issn>1944-8244</issn><eissn>1944-8252</eissn><abstract>Traditional methods of removing gaseous formaldehyde are often associated with high energy consumption and secondary pollution. In this study, a new wood veneer-based composite decorated with Pt-loaded NiFe-LDH nanosheets is successfully developed by a hydrothermal reaction and impregnation-chemical reduction. NiFe-LDH nanosheets as an adsorbent can capture formaldehyde molecules through their abundant hydroxyl groups. Pt nanoparticles as catalytic centers are evenly distributed on the surface of NiFe-LDH to excite the O atoms linked to NiFe-LDH and absorbed oxygen, which will further attack the absorbed formaldehyde molecules to generate CO2 and H2O. And the wood veneer not only increases the active area of the catalyst by endowing it with good dispersion but also provides convenient channels for reactants and products. In a simulated dark environment at room temperature, this synthetic wood veneer-based composite exhibits admirable catalytic activity, which can effectively degrade almost all gaseous formaldehyde with the initial concentration of 0.2 mg m–3 in 30 min and maintain a high catalytic activity of ≥97% after 10 cycles. This paper presents a feasible strategy for synthesizing an energy-efficient and ecofriendly wood veneer-based composite for efficient gaseous formaldehyde degradation at room temperature, which may play an important role in indoor air purification as a promising decorative material.</abstract><pub>American Chemical Society</pub><doi>10.1021/acsami.0c09016</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0003-3520-4970</orcidid></addata></record>
fulltext fulltext
identifier ISSN: 1944-8244
ispartof ACS applied materials & interfaces, 2020-08, Vol.12 (33), p.37147-37154
issn 1944-8244
1944-8252
language eng
recordid cdi_proquest_miscellaneous_2425895860
source ACS Publications
subjects Energy, Environmental, and Catalysis Applications
title Synthesis of Pt-Loaded NiFe-LDH Nanosheets on Wood Veneer for Efficient Gaseous Formaldehyde Degradation
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-08T11%3A11%3A09IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Synthesis%20of%20Pt-Loaded%20NiFe-LDH%20Nanosheets%20on%20Wood%20Veneer%20for%20Efficient%20Gaseous%20Formaldehyde%20Degradation&rft.jtitle=ACS%20applied%20materials%20&%20interfaces&rft.au=Cai,%20Tailong&rft.date=2020-08-19&rft.volume=12&rft.issue=33&rft.spage=37147&rft.epage=37154&rft.pages=37147-37154&rft.issn=1944-8244&rft.eissn=1944-8252&rft_id=info:doi/10.1021/acsami.0c09016&rft_dat=%3Cproquest_cross%3E2425895860%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2425895860&rft_id=info:pmid/&rfr_iscdi=true