Evidence for laser-induced homogeneous oriented ice nucleation revealed via pulsed x-ray diffraction
The induction of homogeneous and oriented ice nucleation has to date not been achieved. Here, we report induced nucleation of ice from millimeter sized supercooled water drops illuminated by ns-optical laser pulses well below the ionization threshold making use of particular laser beam configuration...
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| Veröffentlicht in: | The Journal of chemical physics 2020-07, Vol.153 (2), p.024504-024504 |
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| container_end_page | 024504 |
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| container_issue | 2 |
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| container_title | The Journal of chemical physics |
| container_volume | 153 |
| creator | Nevo, Iftach Jahn, Sabrina Kretzschmar, Norman Levantino, Matteo Feldman, Yishay Naftali, Nir Wulff, Michael Oron, Dan Leiserowitz, Leslie |
| description | The induction of homogeneous and oriented ice nucleation has to date not been achieved. Here, we report induced nucleation of ice from millimeter sized supercooled water drops illuminated by ns-optical laser pulses well below the ionization threshold making use of particular laser beam configurations and polarizations. Employing a 100 ps synchrotron x-ray pulse 100 ns after each laser pulse, an unambiguous correlation was observed between the directions and the symmetry of the laser fields and that of the H-bonding arrays of the induced ice crystals. Moreover, an analysis of the x-ray diffraction data indicates that, in the main, the induced nucleation of ice is homogeneous at temperatures well above the observed and predicted values for supercooled water. |
| doi_str_mv | 10.1063/5.0006100 |
| format | Article |
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| ispartof | The Journal of chemical physics, 2020-07, Vol.153 (2), p.024504-024504 |
| issn | 0021-9606 1089-7690 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_2424441731 |
| source | AIP Journals Complete; Alma/SFX Local Collection |
| subjects | Ice crystals Laser beams Lasers Nucleation Physics Synchrotron radiation Synchrotrons Water drops X-ray diffraction |
| title | Evidence for laser-induced homogeneous oriented ice nucleation revealed via pulsed x-ray diffraction |
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