Niobium disulfide as a new saturable absorber for an ultrafast fiber laser

Group VB transition metal dichalcogenides (TMDCs) are emerging two-dimensional materials and have attracted significant interests in the fields of physics, chemistry, and material sciences. However, there are very few reports about the optical characteristics and ultrafast photonic applications base...

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Veröffentlicht in:Nanoscale 2020-02, Vol.12 (7), p.4537-4543
Hauptverfasser: Li, Lu, Pang, Lihui, Zhao, Qiyi, Wang, Yonggang, Liu, Wenjun
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creator Li, Lu
Pang, Lihui
Zhao, Qiyi
Wang, Yonggang
Liu, Wenjun
description Group VB transition metal dichalcogenides (TMDCs) are emerging two-dimensional materials and have attracted significant interests in the fields of physics, chemistry, and material sciences. However, there are very few reports about the optical characteristics and ultrafast photonic applications based on group VB TMDCs so far. In this work, we have calculated the niobium disulfide (NbS 2 ) band structure by the density functional theory (DFT), which has revealed that NbS 2 is a metallic TMDC. In addition, we have prepared an NbS 2 -microfiber device and the nonlinear optical characteristics have been investigated. The modulation depth, saturation intensity and non-saturable loss have been measured to be 13.7%, 59.93 MW cm −2 and 17.74%, respectively. Based on the nonlinear optical modulation effect, the Er-doped fiber (EDF) laser works in the soliton mode-locking state with the pump power of 94-413 mW. The pulse duration of 709 fs and the maximum average output power of 23.34 mW have been obtained at the pump power of 413 mW. The slope efficiency is as high as 6.79%. Compared to the recently reported studies based on TMDCs comprehensively, our experimental results are better. These experimental results demonstrate that NbS 2 with excellent nonlinear optical properties can be used as a promising candidate to advance the development of ultrafast photonics. Group VB transition metal dichalcogenides (TMDCs) are emerging two-dimensional materials and have attracted significant interests in the fields of physics, chemistry, and material sciences.
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However, there are very few reports about the optical characteristics and ultrafast photonic applications based on group VB TMDCs so far. In this work, we have calculated the niobium disulfide (NbS 2 ) band structure by the density functional theory (DFT), which has revealed that NbS 2 is a metallic TMDC. In addition, we have prepared an NbS 2 -microfiber device and the nonlinear optical characteristics have been investigated. The modulation depth, saturation intensity and non-saturable loss have been measured to be 13.7%, 59.93 MW cm −2 and 17.74%, respectively. Based on the nonlinear optical modulation effect, the Er-doped fiber (EDF) laser works in the soliton mode-locking state with the pump power of 94-413 mW. The pulse duration of 709 fs and the maximum average output power of 23.34 mW have been obtained at the pump power of 413 mW. The slope efficiency is as high as 6.79%. Compared to the recently reported studies based on TMDCs comprehensively, our experimental results are better. These experimental results demonstrate that NbS 2 with excellent nonlinear optical properties can be used as a promising candidate to advance the development of ultrafast photonics. 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However, there are very few reports about the optical characteristics and ultrafast photonic applications based on group VB TMDCs so far. In this work, we have calculated the niobium disulfide (NbS 2 ) band structure by the density functional theory (DFT), which has revealed that NbS 2 is a metallic TMDC. In addition, we have prepared an NbS 2 -microfiber device and the nonlinear optical characteristics have been investigated. The modulation depth, saturation intensity and non-saturable loss have been measured to be 13.7%, 59.93 MW cm −2 and 17.74%, respectively. Based on the nonlinear optical modulation effect, the Er-doped fiber (EDF) laser works in the soliton mode-locking state with the pump power of 94-413 mW. The pulse duration of 709 fs and the maximum average output power of 23.34 mW have been obtained at the pump power of 413 mW. The slope efficiency is as high as 6.79%. Compared to the recently reported studies based on TMDCs comprehensively, our experimental results are better. These experimental results demonstrate that NbS 2 with excellent nonlinear optical properties can be used as a promising candidate to advance the development of ultrafast photonics. 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However, there are very few reports about the optical characteristics and ultrafast photonic applications based on group VB TMDCs so far. In this work, we have calculated the niobium disulfide (NbS 2 ) band structure by the density functional theory (DFT), which has revealed that NbS 2 is a metallic TMDC. In addition, we have prepared an NbS 2 -microfiber device and the nonlinear optical characteristics have been investigated. The modulation depth, saturation intensity and non-saturable loss have been measured to be 13.7%, 59.93 MW cm −2 and 17.74%, respectively. Based on the nonlinear optical modulation effect, the Er-doped fiber (EDF) laser works in the soliton mode-locking state with the pump power of 94-413 mW. The pulse duration of 709 fs and the maximum average output power of 23.34 mW have been obtained at the pump power of 413 mW. The slope efficiency is as high as 6.79%. Compared to the recently reported studies based on TMDCs comprehensively, our experimental results are better. These experimental results demonstrate that NbS 2 with excellent nonlinear optical properties can be used as a promising candidate to advance the development of ultrafast photonics. Group VB transition metal dichalcogenides (TMDCs) are emerging two-dimensional materials and have attracted significant interests in the fields of physics, chemistry, and material sciences.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>32040131</pmid><doi>10.1039/c9nr10873d</doi><tpages>7</tpages><orcidid>https://orcid.org/0000-0002-3097-1954</orcidid><orcidid>https://orcid.org/0000-0001-9380-2990</orcidid></addata></record>
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source Royal Society Of Chemistry Journals 2008-
subjects Density functional theory
Doped fibers
Fiber lasers
Locking
Microfibers
Modulation
Niobium
Optical properties
Organic chemistry
Photonics
Power efficiency
Pulse duration
Solitary waves
Transition metal compounds
Two dimensional materials
title Niobium disulfide as a new saturable absorber for an ultrafast fiber laser
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