Hydrophobic zeolite modification for in situ peroxide formation in methane oxidation to methanol

Selective partial oxidation of methane to methanol suffers from low efficiency. Here, we report a heterogeneous catalyst system for enhanced methanol productivity in methane oxidation by in situ generated hydrogen peroxide at mild temperature (70°C). The catalyst was synthesized by fixation of AuPd...

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Veröffentlicht in:	Science (American Association for the Advancement of Science) 2020-01, Vol.367 (6474), p.193-197
Hauptverfasser:	Jin, Zhu, Wang, Liang, Zuidema, Erik, Mondal, Kartick, Zhang, Ming, Zhang, Jian, Wang, Chengtao, Meng, Xiangju, Yang, Hengquan, Mesters, Carl, Xiao, Feng-Shou
Format:	Artikel
Sprache:	eng
Schlagworte:	Aluminosilicates Aluminum silicates Catalysts Chemical synthesis Confining Conversion Crystals Hydrogen Hydrogen peroxide Hydrophobicity Intermetallic compounds Methane Methanol Nanoalloys Nanoparticles Oxidants Oxidation Oxidizing agents Palladium Productivity Selectivity Silanes Zeolites
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