Engineered Pyrogenic Materials as Tools to Affect Arsenic Mobility in Old Mine Site Soil of Mediterranean Region
The application of pyrogenic materials in immobilization processes of metalloids represents a burning issue in environmental and waste applications and management. The main objective of this study was to characterize the effect of biomass pretreatment by Cu, Fe and Mg blending and pyrolysis temperat...
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| Veröffentlicht in: | Bulletin of environmental contamination and toxicology 2020-02, Vol.104 (2), p.265-272 |
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| creator | Frišták, Vladimír Moreno-Jiménez, Eduardo Bucheli, Thomas D. Fančovičová, Jana Soja, Gerhard Schmidt, Hans-Peter |
| description | The application of pyrogenic materials in immobilization processes of metalloids represents a burning issue in environmental and waste applications and management. The main objective of this study was to characterize the effect of biomass pretreatment by Cu, Fe and Mg blending and pyrolysis temperature on As sorption efficiency as a model of anionic metalloids from model solutions and As immobilization in old mine soil by pyrogenic materials. The physico-chemical characterization of engineered materials produced in slow pyrolysis process at 400 and 700°C from metal-blended hard wood chips (30% w/w) showed increasing of surface areas (1.4–1.8-fold), changes in pH, and more than 50% decrease in total C content. The batch sorption processes of As ions by Cu-modified pyrogenic materials (CuPM), Fe-modified pyrogenic materials (FePM), and Mg-modified pyrogenic materials (MgPM) showed increasing uptake in order CuPM700 (
Q
max
2.56 mg g
−1
) |
| doi_str_mv | 10.1007/s00128-019-02778-9 |
| format | Article |
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Q
max
2.56 mg g
−1
) < CuPM400 (
Q
max
3.88 mg g
−1
) < FePM700 (
Q
max
5.90 mg g
−1
) < MgPM700 (
Q
max
7.42 mg g
−1
) < MgPM400 (
Q
max
9.59 mg g
−1
) < FePM400 (
Q
max
10.55 mg g
−1
). Engineered pyrogenic materials produced at 400°C showed higher immobilization effect on soluble As in soil pore water of old mine site soil from Mediterranean area. FePM400 reduced mobility of arsenic > 3.2 times and MgPM400 > 5 times compared to control. Promising pyrogenic material MgPM400 showed immobilization effect also on additional heavy metals (Cd, Cu, Fe, Mn, Pb, Sr, Zn) present in studied soil.</description><identifier>ISSN: 0007-4861</identifier><identifier>EISSN: 1432-0800</identifier><identifier>DOI: 10.1007/s00128-019-02778-9</identifier><identifier>PMID: 31894372</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Adsorption ; Aquatic Pollution ; Arsenic ; Arsenic - chemistry ; Biomass ; Blending effects ; Burning ; Cadmium ; Copper ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental Restoration and Remediation - methods ; Heavy metals ; Immobilization ; Iron ; Lead ; Magnesium ; Manganese ; Mediterranean Region ; Metalloids ; Metals, Heavy - chemistry ; Mining ; Mobility ; Organic chemistry ; Pollution ; Pore water ; Pretreatment ; Pyrogens - chemical synthesis ; Pyrogens - chemistry ; Pyrolysis ; Soil Pollutants - chemistry ; Soil Science & Conservation ; Soil water ; Soils ; Sorption ; Waste Water Technology ; Water Management ; Water Pollution Control ; Wood chips ; Zinc</subject><ispartof>Bulletin of environmental contamination and toxicology, 2020-02, Vol.104 (2), p.265-272</ispartof><rights>Springer Science+Business Media, LLC, part of Springer Nature 2020</rights><rights>Bulletin of Environmental Contamination and Toxicology is a copyright of Springer, (2020). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a398t-1d084d1bb6a315dd1182606d90fbc3368b3107ced39b17e31047791aa413c6ec3</citedby><cites>FETCH-LOGICAL-a398t-1d084d1bb6a315dd1182606d90fbc3368b3107ced39b17e31047791aa413c6ec3</cites><orcidid>0000-0002-1912-3823</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s00128-019-02778-9$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s00128-019-02778-9$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/31894372$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Frišták, Vladimír</creatorcontrib><creatorcontrib>Moreno-Jiménez, Eduardo</creatorcontrib><creatorcontrib>Bucheli, Thomas D.</creatorcontrib><creatorcontrib>Fančovičová, Jana</creatorcontrib><creatorcontrib>Soja, Gerhard</creatorcontrib><creatorcontrib>Schmidt, Hans-Peter</creatorcontrib><title>Engineered Pyrogenic Materials as Tools to Affect Arsenic Mobility in Old Mine Site Soil of Mediterranean Region</title><title>Bulletin of environmental contamination and toxicology</title><addtitle>Bull Environ Contam Toxicol</addtitle><addtitle>Bull Environ Contam Toxicol</addtitle><description>The application of pyrogenic materials in immobilization processes of metalloids represents a burning issue in environmental and waste applications and management. The main objective of this study was to characterize the effect of biomass pretreatment by Cu, Fe and Mg blending and pyrolysis temperature on As sorption efficiency as a model of anionic metalloids from model solutions and As immobilization in old mine soil by pyrogenic materials. The physico-chemical characterization of engineered materials produced in slow pyrolysis process at 400 and 700°C from metal-blended hard wood chips (30% w/w) showed increasing of surface areas (1.4–1.8-fold), changes in pH, and more than 50% decrease in total C content. The batch sorption processes of As ions by Cu-modified pyrogenic materials (CuPM), Fe-modified pyrogenic materials (FePM), and Mg-modified pyrogenic materials (MgPM) showed increasing uptake in order CuPM700 (
Q
max
2.56 mg g
−1
) < CuPM400 (
Q
max
3.88 mg g
−1
) < FePM700 (
Q
max
5.90 mg g
−1
) < MgPM700 (
Q
max
7.42 mg g
−1
) < MgPM400 (
Q
max
9.59 mg g
−1
) < FePM400 (
Q
max
10.55 mg g
−1
). Engineered pyrogenic materials produced at 400°C showed higher immobilization effect on soluble As in soil pore water of old mine site soil from Mediterranean area. FePM400 reduced mobility of arsenic > 3.2 times and MgPM400 > 5 times compared to control. Promising pyrogenic material MgPM400 showed immobilization effect also on additional heavy metals (Cd, Cu, Fe, Mn, Pb, Sr, Zn) present in studied soil.</description><subject>Adsorption</subject><subject>Aquatic Pollution</subject><subject>Arsenic</subject><subject>Arsenic - chemistry</subject><subject>Biomass</subject><subject>Blending effects</subject><subject>Burning</subject><subject>Cadmium</subject><subject>Copper</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental Restoration and Remediation - methods</subject><subject>Heavy metals</subject><subject>Immobilization</subject><subject>Iron</subject><subject>Lead</subject><subject>Magnesium</subject><subject>Manganese</subject><subject>Mediterranean Region</subject><subject>Metalloids</subject><subject>Metals, Heavy - chemistry</subject><subject>Mining</subject><subject>Mobility</subject><subject>Organic chemistry</subject><subject>Pollution</subject><subject>Pore water</subject><subject>Pretreatment</subject><subject>Pyrogens - chemical synthesis</subject><subject>Pyrogens - chemistry</subject><subject>Pyrolysis</subject><subject>Soil Pollutants - chemistry</subject><subject>Soil Science & Conservation</subject><subject>Soil water</subject><subject>Soils</subject><subject>Sorption</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><subject>Wood chips</subject><subject>Zinc</subject><issn>0007-4861</issn><issn>1432-0800</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2020</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>BENPR</sourceid><recordid>eNp9kc9vFCEUx4nR2LX6D3gwJF68jPJgdoDjpqk_km5qaj0TZnizoZmFFWYP-9_32amaeOgFeOHzvrzwYewtiI8ghP5UhQBpGgG2EVJr09hnbAWtko0wQjxnK0FU05oOztirWu8IXxspX7IzBca2SssVO1ymXUyIBQP_fip5hykOfOtnLNFPlfvKb3Omw5z5ZhxxmPmm1AXKfZzifOIx8esp8C3l8B9xpiXHieeRbzFQWYpP6BO_wV3M6TV7MVIwvnncz9nPz5e3F1-bq-sv3y42V41X1swNBGHaAH3feQXrEACM7EQXrBj7QanO9AqEHjAo24NGKlqtLXjfgho6HNQ5-7DkHkr-dcQ6u32sA04TDZOP1UmlJH2T7VpC3_-H3uVjSTQdUa1SxKw1UXKhhpJrLTi6Q4l7X04OhPvtwy0-HPlwDz6cpaZ3j9HHfo_hb8sfAQSoBah0lXZY_r39ROw9GAiUaw</recordid><startdate>20200201</startdate><enddate>20200201</enddate><creator>Frišták, Vladimír</creator><creator>Moreno-Jiménez, Eduardo</creator><creator>Bucheli, Thomas D.</creator><creator>Fančovičová, Jana</creator><creator>Soja, Gerhard</creator><creator>Schmidt, Hans-Peter</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7T7</scope><scope>7TK</scope><scope>7TV</scope><scope>7U7</scope><scope>7X7</scope><scope>7XB</scope><scope>88E</scope><scope>88I</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FYUFA</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K9.</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>P64</scope><scope>PATMY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-1912-3823</orcidid></search><sort><creationdate>20200201</creationdate><title>Engineered Pyrogenic Materials as Tools to Affect Arsenic Mobility in Old Mine Site Soil of Mediterranean Region</title><author>Frišták, Vladimír ; Moreno-Jiménez, Eduardo ; Bucheli, Thomas D. ; Fančovičová, Jana ; Soja, Gerhard ; Schmidt, Hans-Peter</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a398t-1d084d1bb6a315dd1182606d90fbc3368b3107ced39b17e31047791aa413c6ec3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2020</creationdate><topic>Adsorption</topic><topic>Aquatic Pollution</topic><topic>Arsenic</topic><topic>Arsenic - chemistry</topic><topic>Biomass</topic><topic>Blending effects</topic><topic>Burning</topic><topic>Cadmium</topic><topic>Copper</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental Restoration and Remediation - methods</topic><topic>Heavy metals</topic><topic>Immobilization</topic><topic>Iron</topic><topic>Lead</topic><topic>Magnesium</topic><topic>Manganese</topic><topic>Mediterranean Region</topic><topic>Metalloids</topic><topic>Metals, Heavy - chemistry</topic><topic>Mining</topic><topic>Mobility</topic><topic>Organic chemistry</topic><topic>Pollution</topic><topic>Pore water</topic><topic>Pretreatment</topic><topic>Pyrogens - chemical synthesis</topic><topic>Pyrogens - chemistry</topic><topic>Pyrolysis</topic><topic>Soil Pollutants - chemistry</topic><topic>Soil Science & Conservation</topic><topic>Soil water</topic><topic>Soils</topic><topic>Sorption</topic><topic>Waste Water Technology</topic><topic>Water Management</topic><topic>Water Pollution Control</topic><topic>Wood chips</topic><topic>Zinc</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Frišták, Vladimír</creatorcontrib><creatorcontrib>Moreno-Jiménez, Eduardo</creatorcontrib><creatorcontrib>Bucheli, Thomas D.</creatorcontrib><creatorcontrib>Fančovičová, Jana</creatorcontrib><creatorcontrib>Soja, Gerhard</creatorcontrib><creatorcontrib>Schmidt, Hans-Peter</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Neurosciences Abstracts</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>Health & Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Medical Database (Alumni Edition)</collection><collection>Science Database (Alumni Edition)</collection><collection>Public Health Database</collection><collection>Technology Research Database</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>ProQuest Central (Alumni)</collection><collection>ProQuest One Sustainability</collection><collection>ProQuest Central</collection><collection>Agricultural & Environmental Science Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Natural Science Collection</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central</collection><collection>Engineering Research Database</collection><collection>Health Research Premium Collection</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>Health & Medical Collection (Alumni Edition)</collection><collection>Medical Database</collection><collection>Science Database</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Environmental Science Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Environmental Science Collection</collection><collection>ProQuest Central Basic</collection><collection>MEDLINE - Academic</collection><jtitle>Bulletin of environmental contamination and toxicology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Frišták, Vladimír</au><au>Moreno-Jiménez, Eduardo</au><au>Bucheli, Thomas D.</au><au>Fančovičová, Jana</au><au>Soja, Gerhard</au><au>Schmidt, Hans-Peter</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Engineered Pyrogenic Materials as Tools to Affect Arsenic Mobility in Old Mine Site Soil of Mediterranean Region</atitle><jtitle>Bulletin of environmental contamination and toxicology</jtitle><stitle>Bull Environ Contam Toxicol</stitle><addtitle>Bull Environ Contam Toxicol</addtitle><date>2020-02-01</date><risdate>2020</risdate><volume>104</volume><issue>2</issue><spage>265</spage><epage>272</epage><pages>265-272</pages><issn>0007-4861</issn><eissn>1432-0800</eissn><abstract>The application of pyrogenic materials in immobilization processes of metalloids represents a burning issue in environmental and waste applications and management. The main objective of this study was to characterize the effect of biomass pretreatment by Cu, Fe and Mg blending and pyrolysis temperature on As sorption efficiency as a model of anionic metalloids from model solutions and As immobilization in old mine soil by pyrogenic materials. The physico-chemical characterization of engineered materials produced in slow pyrolysis process at 400 and 700°C from metal-blended hard wood chips (30% w/w) showed increasing of surface areas (1.4–1.8-fold), changes in pH, and more than 50% decrease in total C content. The batch sorption processes of As ions by Cu-modified pyrogenic materials (CuPM), Fe-modified pyrogenic materials (FePM), and Mg-modified pyrogenic materials (MgPM) showed increasing uptake in order CuPM700 (
Q
max
2.56 mg g
−1
) < CuPM400 (
Q
max
3.88 mg g
−1
) < FePM700 (
Q
max
5.90 mg g
−1
) < MgPM700 (
Q
max
7.42 mg g
−1
) < MgPM400 (
Q
max
9.59 mg g
−1
) < FePM400 (
Q
max
10.55 mg g
−1
). Engineered pyrogenic materials produced at 400°C showed higher immobilization effect on soluble As in soil pore water of old mine site soil from Mediterranean area. FePM400 reduced mobility of arsenic > 3.2 times and MgPM400 > 5 times compared to control. Promising pyrogenic material MgPM400 showed immobilization effect also on additional heavy metals (Cd, Cu, Fe, Mn, Pb, Sr, Zn) present in studied soil.</abstract><cop>New York</cop><pub>Springer US</pub><pmid>31894372</pmid><doi>10.1007/s00128-019-02778-9</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0002-1912-3823</orcidid></addata></record> |
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| ispartof | Bulletin of environmental contamination and toxicology, 2020-02, Vol.104 (2), p.265-272 |
| issn | 0007-4861 1432-0800 |
| language | eng |
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| source | MEDLINE; Springer Online Journals |
| subjects | Adsorption Aquatic Pollution Arsenic Arsenic - chemistry Biomass Blending effects Burning Cadmium Copper Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental Restoration and Remediation - methods Heavy metals Immobilization Iron Lead Magnesium Manganese Mediterranean Region Metalloids Metals, Heavy - chemistry Mining Mobility Organic chemistry Pollution Pore water Pretreatment Pyrogens - chemical synthesis Pyrogens - chemistry Pyrolysis Soil Pollutants - chemistry Soil Science & Conservation Soil water Soils Sorption Waste Water Technology Water Management Water Pollution Control Wood chips Zinc |
| title | Engineered Pyrogenic Materials as Tools to Affect Arsenic Mobility in Old Mine Site Soil of Mediterranean Region |
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