Light Scattering from Solid-State Quantum Emitters: Beyond the Atomic Picture
Coherent scattering of light by a single quantum emitter is a fundamental process at the heart of many proposed quantum technologies. Unlike atomic systems, solid-state emitters couple to their host lattice by phonons. Using a quantum dot in an optical nanocavity, we resolve these interactions in bo...
Gespeichert in:
| Veröffentlicht in: | Physical review letters 2019-10, Vol.123 (16), p.1-167403, Article 167403 |
|---|---|
| Hauptverfasser: | , , , , , , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 167403 |
|---|---|
| container_issue | 16 |
| container_start_page | 1 |
| container_title | Physical review letters |
| container_volume | 123 |
| creator | Brash, Alistair J. Iles-Smith, Jake Phillips, Catherine L. McCutcheon, Dara P. S. O’Hara, John Clarke, Edmund Royall, Benjamin Wilson, Luke R. Mørk, Jesper Skolnick, Maurice S. Fox, A. Mark Nazir, Ahsan |
| description | Coherent scattering of light by a single quantum emitter is a fundamental process at the heart of many proposed quantum technologies. Unlike atomic systems, solid-state emitters couple to their host lattice by phonons. Using a quantum dot in an optical nanocavity, we resolve these interactions in both time and frequency domains, going beyond the atomic picture to develop a comprehensive model of light scattering from solid-state emitters. We find that even in the presence of a low-Q cavity with high Purcell enhancement, phonon coupling leads to a sideband that is completely insensitive to excitation conditions and to a nonmonotonic relationship between laser detuning and coherent fraction, both of which are major deviations from atomlike behavior. |
| doi_str_mv | 10.1103/PhysRevLett.123.167403 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_2313376631</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2313376631</sourcerecordid><originalsourceid>FETCH-LOGICAL-c369t-cf74158ae575ad728ec6266bc0b276b9c88b28a640e6d45377ef85e8641bc8033</originalsourceid><addsrcrecordid>eNpd0EtLAzEUhuEgCtbqX5CAGzdTc5lJMu6q1AtUrFbXIZM506bMpSYZof_eKXUhrr7Nw-HwInRJyYRSwm8W6114h-85xDihjE-okCnhR2hEicwTSWl6jEaEcJrkhMhTdBbChhBCmVAj9DJ3q3XES2tiBO_aFa581-BlV7syWUYTAb_1po19g2eN25twi-9g17UljmvA09g1zuKFs7H3cI5OKlMHuPjdMfp8mH3cPyXz18fn--k8sVzkMbGVTGmmDGQyM6VkCqxgQhSWFEyKIrdKFUwZkRIQZZpxKaFSGSiR0sIqwvkYXR_ubn331UOIunHBQl2bFro-aMYp51KIYcbo6h_ddL1vh-8GRZTKUsXUoMRBWd-F4KHSW-8a43eaEr2vrP9U1kNlfajMfwBDQ3It</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2308854828</pqid></control><display><type>article</type><title>Light Scattering from Solid-State Quantum Emitters: Beyond the Atomic Picture</title><source>American Physical Society Journals</source><source>Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals</source><creator>Brash, Alistair J. ; Iles-Smith, Jake ; Phillips, Catherine L. ; McCutcheon, Dara P. S. ; O’Hara, John ; Clarke, Edmund ; Royall, Benjamin ; Wilson, Luke R. ; Mørk, Jesper ; Skolnick, Maurice S. ; Fox, A. Mark ; Nazir, Ahsan</creator><creatorcontrib>Brash, Alistair J. ; Iles-Smith, Jake ; Phillips, Catherine L. ; McCutcheon, Dara P. S. ; O’Hara, John ; Clarke, Edmund ; Royall, Benjamin ; Wilson, Luke R. ; Mørk, Jesper ; Skolnick, Maurice S. ; Fox, A. Mark ; Nazir, Ahsan</creatorcontrib><description>Coherent scattering of light by a single quantum emitter is a fundamental process at the heart of many proposed quantum technologies. Unlike atomic systems, solid-state emitters couple to their host lattice by phonons. Using a quantum dot in an optical nanocavity, we resolve these interactions in both time and frequency domains, going beyond the atomic picture to develop a comprehensive model of light scattering from solid-state emitters. We find that even in the presence of a low-Q cavity with high Purcell enhancement, phonon coupling leads to a sideband that is completely insensitive to excitation conditions and to a nonmonotonic relationship between laser detuning and coherent fraction, both of which are major deviations from atomlike behavior.</description><identifier>ISSN: 0031-9007</identifier><identifier>EISSN: 1079-7114</identifier><identifier>DOI: 10.1103/PhysRevLett.123.167403</identifier><language>eng</language><publisher>College Park: American Physical Society</publisher><subject>Coherent scattering ; Emitters ; Light scattering ; Phonons ; Quantum dots ; Solid state</subject><ispartof>Physical review letters, 2019-10, Vol.123 (16), p.1-167403, Article 167403</ispartof><rights>Copyright American Physical Society Oct 16, 2019</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c369t-cf74158ae575ad728ec6266bc0b276b9c88b28a640e6d45377ef85e8641bc8033</citedby><cites>FETCH-LOGICAL-c369t-cf74158ae575ad728ec6266bc0b276b9c88b28a640e6d45377ef85e8641bc8033</cites><orcidid>0000-0001-5717-6793</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,2863,2864,27901,27902</link.rule.ids></links><search><creatorcontrib>Brash, Alistair J.</creatorcontrib><creatorcontrib>Iles-Smith, Jake</creatorcontrib><creatorcontrib>Phillips, Catherine L.</creatorcontrib><creatorcontrib>McCutcheon, Dara P. S.</creatorcontrib><creatorcontrib>O’Hara, John</creatorcontrib><creatorcontrib>Clarke, Edmund</creatorcontrib><creatorcontrib>Royall, Benjamin</creatorcontrib><creatorcontrib>Wilson, Luke R.</creatorcontrib><creatorcontrib>Mørk, Jesper</creatorcontrib><creatorcontrib>Skolnick, Maurice S.</creatorcontrib><creatorcontrib>Fox, A. Mark</creatorcontrib><creatorcontrib>Nazir, Ahsan</creatorcontrib><title>Light Scattering from Solid-State Quantum Emitters: Beyond the Atomic Picture</title><title>Physical review letters</title><description>Coherent scattering of light by a single quantum emitter is a fundamental process at the heart of many proposed quantum technologies. Unlike atomic systems, solid-state emitters couple to their host lattice by phonons. Using a quantum dot in an optical nanocavity, we resolve these interactions in both time and frequency domains, going beyond the atomic picture to develop a comprehensive model of light scattering from solid-state emitters. We find that even in the presence of a low-Q cavity with high Purcell enhancement, phonon coupling leads to a sideband that is completely insensitive to excitation conditions and to a nonmonotonic relationship between laser detuning and coherent fraction, both of which are major deviations from atomlike behavior.</description><subject>Coherent scattering</subject><subject>Emitters</subject><subject>Light scattering</subject><subject>Phonons</subject><subject>Quantum dots</subject><subject>Solid state</subject><issn>0031-9007</issn><issn>1079-7114</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNpd0EtLAzEUhuEgCtbqX5CAGzdTc5lJMu6q1AtUrFbXIZM506bMpSYZof_eKXUhrr7Nw-HwInRJyYRSwm8W6114h-85xDihjE-okCnhR2hEicwTSWl6jEaEcJrkhMhTdBbChhBCmVAj9DJ3q3XES2tiBO_aFa581-BlV7syWUYTAb_1po19g2eN25twi-9g17UljmvA09g1zuKFs7H3cI5OKlMHuPjdMfp8mH3cPyXz18fn--k8sVzkMbGVTGmmDGQyM6VkCqxgQhSWFEyKIrdKFUwZkRIQZZpxKaFSGSiR0sIqwvkYXR_ubn331UOIunHBQl2bFro-aMYp51KIYcbo6h_ddL1vh-8GRZTKUsXUoMRBWd-F4KHSW-8a43eaEr2vrP9U1kNlfajMfwBDQ3It</recordid><startdate>20191016</startdate><enddate>20191016</enddate><creator>Brash, Alistair J.</creator><creator>Iles-Smith, Jake</creator><creator>Phillips, Catherine L.</creator><creator>McCutcheon, Dara P. S.</creator><creator>O’Hara, John</creator><creator>Clarke, Edmund</creator><creator>Royall, Benjamin</creator><creator>Wilson, Luke R.</creator><creator>Mørk, Jesper</creator><creator>Skolnick, Maurice S.</creator><creator>Fox, A. Mark</creator><creator>Nazir, Ahsan</creator><general>American Physical Society</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0001-5717-6793</orcidid></search><sort><creationdate>20191016</creationdate><title>Light Scattering from Solid-State Quantum Emitters: Beyond the Atomic Picture</title><author>Brash, Alistair J. ; Iles-Smith, Jake ; Phillips, Catherine L. ; McCutcheon, Dara P. S. ; O’Hara, John ; Clarke, Edmund ; Royall, Benjamin ; Wilson, Luke R. ; Mørk, Jesper ; Skolnick, Maurice S. ; Fox, A. Mark ; Nazir, Ahsan</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c369t-cf74158ae575ad728ec6266bc0b276b9c88b28a640e6d45377ef85e8641bc8033</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Coherent scattering</topic><topic>Emitters</topic><topic>Light scattering</topic><topic>Phonons</topic><topic>Quantum dots</topic><topic>Solid state</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Brash, Alistair J.</creatorcontrib><creatorcontrib>Iles-Smith, Jake</creatorcontrib><creatorcontrib>Phillips, Catherine L.</creatorcontrib><creatorcontrib>McCutcheon, Dara P. S.</creatorcontrib><creatorcontrib>O’Hara, John</creatorcontrib><creatorcontrib>Clarke, Edmund</creatorcontrib><creatorcontrib>Royall, Benjamin</creatorcontrib><creatorcontrib>Wilson, Luke R.</creatorcontrib><creatorcontrib>Mørk, Jesper</creatorcontrib><creatorcontrib>Skolnick, Maurice S.</creatorcontrib><creatorcontrib>Fox, A. Mark</creatorcontrib><creatorcontrib>Nazir, Ahsan</creatorcontrib><collection>CrossRef</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Physical review letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Brash, Alistair J.</au><au>Iles-Smith, Jake</au><au>Phillips, Catherine L.</au><au>McCutcheon, Dara P. S.</au><au>O’Hara, John</au><au>Clarke, Edmund</au><au>Royall, Benjamin</au><au>Wilson, Luke R.</au><au>Mørk, Jesper</au><au>Skolnick, Maurice S.</au><au>Fox, A. Mark</au><au>Nazir, Ahsan</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Light Scattering from Solid-State Quantum Emitters: Beyond the Atomic Picture</atitle><jtitle>Physical review letters</jtitle><date>2019-10-16</date><risdate>2019</risdate><volume>123</volume><issue>16</issue><spage>1</spage><epage>167403</epage><pages>1-167403</pages><artnum>167403</artnum><issn>0031-9007</issn><eissn>1079-7114</eissn><abstract>Coherent scattering of light by a single quantum emitter is a fundamental process at the heart of many proposed quantum technologies. Unlike atomic systems, solid-state emitters couple to their host lattice by phonons. Using a quantum dot in an optical nanocavity, we resolve these interactions in both time and frequency domains, going beyond the atomic picture to develop a comprehensive model of light scattering from solid-state emitters. We find that even in the presence of a low-Q cavity with high Purcell enhancement, phonon coupling leads to a sideband that is completely insensitive to excitation conditions and to a nonmonotonic relationship between laser detuning and coherent fraction, both of which are major deviations from atomlike behavior.</abstract><cop>College Park</cop><pub>American Physical Society</pub><doi>10.1103/PhysRevLett.123.167403</doi><orcidid>https://orcid.org/0000-0001-5717-6793</orcidid><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0031-9007 |
| ispartof | Physical review letters, 2019-10, Vol.123 (16), p.1-167403, Article 167403 |
| issn | 0031-9007 1079-7114 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_2313376631 |
| source | American Physical Society Journals; Elektronische Zeitschriftenbibliothek - Frei zugängliche E-Journals |
| subjects | Coherent scattering Emitters Light scattering Phonons Quantum dots Solid state |
| title | Light Scattering from Solid-State Quantum Emitters: Beyond the Atomic Picture |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-01T19%3A55%3A07IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Light%20Scattering%20from%20Solid-State%20Quantum%20Emitters:%20Beyond%20the%20Atomic%20Picture&rft.jtitle=Physical%20review%20letters&rft.au=Brash,%20Alistair%20J.&rft.date=2019-10-16&rft.volume=123&rft.issue=16&rft.spage=1&rft.epage=167403&rft.pages=1-167403&rft.artnum=167403&rft.issn=0031-9007&rft.eissn=1079-7114&rft_id=info:doi/10.1103/PhysRevLett.123.167403&rft_dat=%3Cproquest_cross%3E2313376631%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2308854828&rft_id=info:pmid/&rfr_iscdi=true |