In Situ Methods for Identifying Reactive Surface Intermediates during Hydrogenolysis Reactions: C–O Bond Cleavage on Nanoparticles of Nickel and Nickel Phosphides

Identifying individual reactive intermediates within the “zoo” of organometallic species that form on catalytic surfaces during reactions is a long-standing challenge in heterogeneous catalysis. Here, we identify distinct reactive intermediates, all of which exist at low coverages, that lead to dist...

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Veröffentlicht in:	Journal of the American Chemical Society 2019-10, Vol.141 (42), p.16671-16684
Hauptverfasser:	Witzke, Megan E, Almithn, Abdulrahman, Coonrod, Christian L, Triezenberg, Mark D, Hibbitts, David D, Flaherty, David W
Format:	Artikel
Sprache:	eng
Online-Zugang:	Volltext
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