Location matters: cooperativity of catalytic partners in porous organic polymers for enhanced CO2 transformation
Herein, we show that by following molecular engineering of the inter-site distance between the two functionalities in porous organic materials, it is possible to enable them to work in a concerted manner. Specifically, the activity can be amplified by the placement of the hydroxyl group in the meta...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2019-08, Vol.55 (62), p.9180-9183 |
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| container_issue | 62 |
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| container_title | Chemical communications (Cambridge, England) |
| container_volume | 55 |
| creator | Hu, Kewei Tang, Yongquan Cui, Jia Gong, Qihan Hu, Changlu Wang, Sai Dong, Ke Meng, Xiangju Sun, Qi Feng-Shou, Xiao |
| description | Herein, we show that by following molecular engineering of the inter-site distance between the two functionalities in porous organic materials, it is possible to enable them to work in a concerted manner. Specifically, the activity can be amplified by the placement of the hydroxyl group in the meta position of the phosphonium salts in the representative cycloaddition of epoxides and CO2. |
| doi_str_mv | 10.1039/c9cc05051e |
| format | Article |
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| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2019-08, Vol.55 (62), p.9180-9183 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_proquest_miscellaneous_2258155053 |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Carbon dioxide Catalysis Cycloaddition Hydroxyl groups Organic materials Porous materials |
| title | Location matters: cooperativity of catalytic partners in porous organic polymers for enhanced CO2 transformation |
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