Simultaneous removal of nitrogen oxides and sulfur dioxide using ultrasonically atomized hydrogen peroxide
A new method was developed for denitrification and desulfurization using hydrogen peroxide with the aid of an ultrasonic nebulizer to obtain high removal efficiency of NOx and SO 2 . Comparing with the atomizing nozzles having the aperture size of 0.01~0.02 mm, the droplets generated using the ultra...
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| Veröffentlicht in: | Environmental science and pollution research international 2019-08, Vol.26 (22), p.22351-22361 |
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| creator | Wei, Jiaqi Gu, Junjie Guo, Junheng Li, Wei Wang, Chenglong Zhang, Jinli |
| description | A new method was developed for denitrification and desulfurization using hydrogen peroxide with the aid of an ultrasonic nebulizer to obtain high removal efficiency of NOx and SO
2
. Comparing with the atomizing nozzles having the aperture size of 0.01~0.02 mm, the droplets generated using the ultrasonic nebulizer show the smallest
d
50
value of 7.2 μm, with 72% possessing the size less than 10 μm. Based on the numerical simulation of the vaporization rate of droplets, it is indicated that the droplets with the size of 7.2 μm can be vaporized totally at very short residence time (0.11 s) under 130 °C. Effects of influence factors including the reaction temperature, the initial H
2
O
2
concentration, pH value, and the flue gas flow rate were studied on the removal efficiencies of NO and SO
2
. Using the in-series double-oxidation subsystems with H
2
O
2
concentration of 6 wt%, pH 5.0, and the reaction temperature of 130 °C, the removal efficiencies of SO
2
and NO are respectively 100% and 89.3% at the short residence time of 1.8 s, and the removal efficiency of NO can be increased to 100% as the residence time is longer than 3.7 s. It is confirmed that the ultrasonically atomized H
2
O
2
can indeed enhance the removal efficiencies of NO and SO
2
at the optimal temperature, owing to the fast vaporization rate of fine droplets as well as the formation of more active radicals to be captured by NO and SO
2
simultaneously. The results here provide a promising route to remove effectively the emissions of NO and SO
2
simultaneously.
Graphical abstract |
| doi_str_mv | 10.1007/s11356-019-05531-1 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_2234487139</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2233217562</sourcerecordid><originalsourceid>FETCH-LOGICAL-c412t-ce5d64da994478e4a0f6f6376b4bce19fd049d0e5d6db8eff24f7bf6ede3506e3</originalsourceid><addsrcrecordid>eNp9kUtv3CAUhVHVqJkm-QNdVEjddOOECxgPyyjqS4rURZI1wuYyZWSbKdhRp78-zDhtpC66Qrp859zHIeQdsEtgrLnKAKJWFQNdsboWUMErsgIFsmqk1q_JimkpKxBSnpK3OW8Z40zz5g05FQC1VDWsyPYuDHM_2RHjnGnCIT7ankZPxzCluMGRxl_BYaZ2dDTPvZ8TdeFYo3MO44YWdbI5jqGzfb-ndopD-I2O_ti7xWCH6cifkxNv-4wXz-8Zefj86f7ma3X7_cu3m-vbqpPAp6rD2inprC7DN2uUlnnllWhUK9sOQXvHpHbsQLl2jd5z6ZvWK3QoaqZQnJGPi-8uxZ8z5skMIXfY98uShvNykXUDQhf0wz_oNs5pLNMdKMGhqRUvFF-oLsWcE3qzS2GwaW-AmUMSZknClCTMMQkDRfT-2XpuB3R_JX9OXwCxALl8jRtML73_Y_sE1mWWoQ</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2233217562</pqid></control><display><type>article</type><title>Simultaneous removal of nitrogen oxides and sulfur dioxide using ultrasonically atomized hydrogen peroxide</title><source>SpringerNature Journals</source><creator>Wei, Jiaqi ; Gu, Junjie ; Guo, Junheng ; Li, Wei ; Wang, Chenglong ; Zhang, Jinli</creator><creatorcontrib>Wei, Jiaqi ; Gu, Junjie ; Guo, Junheng ; Li, Wei ; Wang, Chenglong ; Zhang, Jinli</creatorcontrib><description>A new method was developed for denitrification and desulfurization using hydrogen peroxide with the aid of an ultrasonic nebulizer to obtain high removal efficiency of NOx and SO
2
. Comparing with the atomizing nozzles having the aperture size of 0.01~0.02 mm, the droplets generated using the ultrasonic nebulizer show the smallest
d
50
value of 7.2 μm, with 72% possessing the size less than 10 μm. Based on the numerical simulation of the vaporization rate of droplets, it is indicated that the droplets with the size of 7.2 μm can be vaporized totally at very short residence time (0.11 s) under 130 °C. Effects of influence factors including the reaction temperature, the initial H
2
O
2
concentration, pH value, and the flue gas flow rate were studied on the removal efficiencies of NO and SO
2
. Using the in-series double-oxidation subsystems with H
2
O
2
concentration of 6 wt%, pH 5.0, and the reaction temperature of 130 °C, the removal efficiencies of SO
2
and NO are respectively 100% and 89.3% at the short residence time of 1.8 s, and the removal efficiency of NO can be increased to 100% as the residence time is longer than 3.7 s. It is confirmed that the ultrasonically atomized H
2
O
2
can indeed enhance the removal efficiencies of NO and SO
2
at the optimal temperature, owing to the fast vaporization rate of fine droplets as well as the formation of more active radicals to be captured by NO and SO
2
simultaneously. The results here provide a promising route to remove effectively the emissions of NO and SO
2
simultaneously.
Graphical abstract</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-019-05531-1</identifier><identifier>PMID: 31154651</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Apertures ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Atomizing ; Chemical engineering ; Compressed air ; Computer simulation ; Denitrification ; Droplets ; Earth and Environmental Science ; Ecotoxicology ; Efficiency ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Flow rates ; Flow velocity ; Flue gas ; Gas flow ; Hydrogen peroxide ; Mathematical models ; Nitrogen ; Nitrogen oxides ; Nitrogen removal ; Nozzles ; Oxidation ; Oxides ; pH effects ; Photochemicals ; Research Article ; Residence time distribution ; Simulation ; Subsystems ; Sulfur ; Sulfur dioxide ; Temperature effects ; Vaporization ; Waste Water Technology ; Water Management ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2019-08, Vol.26 (22), p.22351-22361</ispartof><rights>Springer-Verlag GmbH Germany, part of Springer Nature 2019</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, (2019). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c412t-ce5d64da994478e4a0f6f6376b4bce19fd049d0e5d6db8eff24f7bf6ede3506e3</citedby><cites>FETCH-LOGICAL-c412t-ce5d64da994478e4a0f6f6376b4bce19fd049d0e5d6db8eff24f7bf6ede3506e3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-019-05531-1$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-019-05531-1$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/31154651$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Wei, Jiaqi</creatorcontrib><creatorcontrib>Gu, Junjie</creatorcontrib><creatorcontrib>Guo, Junheng</creatorcontrib><creatorcontrib>Li, Wei</creatorcontrib><creatorcontrib>Wang, Chenglong</creatorcontrib><creatorcontrib>Zhang, Jinli</creatorcontrib><title>Simultaneous removal of nitrogen oxides and sulfur dioxide using ultrasonically atomized hydrogen peroxide</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>A new method was developed for denitrification and desulfurization using hydrogen peroxide with the aid of an ultrasonic nebulizer to obtain high removal efficiency of NOx and SO
2
. Comparing with the atomizing nozzles having the aperture size of 0.01~0.02 mm, the droplets generated using the ultrasonic nebulizer show the smallest
d
50
value of 7.2 μm, with 72% possessing the size less than 10 μm. Based on the numerical simulation of the vaporization rate of droplets, it is indicated that the droplets with the size of 7.2 μm can be vaporized totally at very short residence time (0.11 s) under 130 °C. Effects of influence factors including the reaction temperature, the initial H
2
O
2
concentration, pH value, and the flue gas flow rate were studied on the removal efficiencies of NO and SO
2
. Using the in-series double-oxidation subsystems with H
2
O
2
concentration of 6 wt%, pH 5.0, and the reaction temperature of 130 °C, the removal efficiencies of SO
2
and NO are respectively 100% and 89.3% at the short residence time of 1.8 s, and the removal efficiency of NO can be increased to 100% as the residence time is longer than 3.7 s. It is confirmed that the ultrasonically atomized H
2
O
2
can indeed enhance the removal efficiencies of NO and SO
2
at the optimal temperature, owing to the fast vaporization rate of fine droplets as well as the formation of more active radicals to be captured by NO and SO
2
simultaneously. The results here provide a promising route to remove effectively the emissions of NO and SO
2
simultaneously.
Graphical abstract</description><subject>Apertures</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Atomizing</subject><subject>Chemical engineering</subject><subject>Compressed air</subject><subject>Computer simulation</subject><subject>Denitrification</subject><subject>Droplets</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Efficiency</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Flow rates</subject><subject>Flow velocity</subject><subject>Flue gas</subject><subject>Gas flow</subject><subject>Hydrogen peroxide</subject><subject>Mathematical models</subject><subject>Nitrogen</subject><subject>Nitrogen oxides</subject><subject>Nitrogen removal</subject><subject>Nozzles</subject><subject>Oxidation</subject><subject>Oxides</subject><subject>pH effects</subject><subject>Photochemicals</subject><subject>Research Article</subject><subject>Residence time distribution</subject><subject>Simulation</subject><subject>Subsystems</subject><subject>Sulfur</subject><subject>Sulfur dioxide</subject><subject>Temperature effects</subject><subject>Vaporization</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp9kUtv3CAUhVHVqJkm-QNdVEjddOOECxgPyyjqS4rURZI1wuYyZWSbKdhRp78-zDhtpC66Qrp859zHIeQdsEtgrLnKAKJWFQNdsboWUMErsgIFsmqk1q_JimkpKxBSnpK3OW8Z40zz5g05FQC1VDWsyPYuDHM_2RHjnGnCIT7ankZPxzCluMGRxl_BYaZ2dDTPvZ8TdeFYo3MO44YWdbI5jqGzfb-ndopD-I2O_ti7xWCH6cifkxNv-4wXz-8Zefj86f7ma3X7_cu3m-vbqpPAp6rD2inprC7DN2uUlnnllWhUK9sOQXvHpHbsQLl2jd5z6ZvWK3QoaqZQnJGPi-8uxZ8z5skMIXfY98uShvNykXUDQhf0wz_oNs5pLNMdKMGhqRUvFF-oLsWcE3qzS2GwaW-AmUMSZknClCTMMQkDRfT-2XpuB3R_JX9OXwCxALl8jRtML73_Y_sE1mWWoQ</recordid><startdate>20190801</startdate><enddate>20190801</enddate><creator>Wei, Jiaqi</creator><creator>Gu, Junjie</creator><creator>Guo, 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removal of nitrogen oxides and sulfur dioxide using ultrasonically atomized hydrogen peroxide</title><author>Wei, Jiaqi ; Gu, Junjie ; Guo, Junheng ; Li, Wei ; Wang, Chenglong ; Zhang, Jinli</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c412t-ce5d64da994478e4a0f6f6376b4bce19fd049d0e5d6db8eff24f7bf6ede3506e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Apertures</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Atomizing</topic><topic>Chemical engineering</topic><topic>Compressed air</topic><topic>Computer simulation</topic><topic>Denitrification</topic><topic>Droplets</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Efficiency</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental science</topic><topic>Flow rates</topic><topic>Flow velocity</topic><topic>Flue gas</topic><topic>Gas flow</topic><topic>Hydrogen peroxide</topic><topic>Mathematical models</topic><topic>Nitrogen</topic><topic>Nitrogen oxides</topic><topic>Nitrogen removal</topic><topic>Nozzles</topic><topic>Oxidation</topic><topic>Oxides</topic><topic>pH effects</topic><topic>Photochemicals</topic><topic>Research Article</topic><topic>Residence time distribution</topic><topic>Simulation</topic><topic>Subsystems</topic><topic>Sulfur</topic><topic>Sulfur dioxide</topic><topic>Temperature effects</topic><topic>Vaporization</topic><topic>Waste Water Technology</topic><topic>Water Management</topic><topic>Water Pollution Control</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wei, Jiaqi</creatorcontrib><creatorcontrib>Gu, Junjie</creatorcontrib><creatorcontrib>Guo, Junheng</creatorcontrib><creatorcontrib>Li, Wei</creatorcontrib><creatorcontrib>Wang, 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Int</addtitle><date>2019-08-01</date><risdate>2019</risdate><volume>26</volume><issue>22</issue><spage>22351</spage><epage>22361</epage><pages>22351-22361</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>A new method was developed for denitrification and desulfurization using hydrogen peroxide with the aid of an ultrasonic nebulizer to obtain high removal efficiency of NOx and SO
2
. Comparing with the atomizing nozzles having the aperture size of 0.01~0.02 mm, the droplets generated using the ultrasonic nebulizer show the smallest
d
50
value of 7.2 μm, with 72% possessing the size less than 10 μm. Based on the numerical simulation of the vaporization rate of droplets, it is indicated that the droplets with the size of 7.2 μm can be vaporized totally at very short residence time (0.11 s) under 130 °C. Effects of influence factors including the reaction temperature, the initial H
2
O
2
concentration, pH value, and the flue gas flow rate were studied on the removal efficiencies of NO and SO
2
. Using the in-series double-oxidation subsystems with H
2
O
2
concentration of 6 wt%, pH 5.0, and the reaction temperature of 130 °C, the removal efficiencies of SO
2
and NO are respectively 100% and 89.3% at the short residence time of 1.8 s, and the removal efficiency of NO can be increased to 100% as the residence time is longer than 3.7 s. It is confirmed that the ultrasonically atomized H
2
O
2
can indeed enhance the removal efficiencies of NO and SO
2
at the optimal temperature, owing to the fast vaporization rate of fine droplets as well as the formation of more active radicals to be captured by NO and SO
2
simultaneously. The results here provide a promising route to remove effectively the emissions of NO and SO
2
simultaneously.
Graphical abstract</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>31154651</pmid><doi>10.1007/s11356-019-05531-1</doi><tpages>11</tpages></addata></record> |
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| ispartof | Environmental science and pollution research international, 2019-08, Vol.26 (22), p.22351-22361 |
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| language | eng |
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| source | SpringerNature Journals |
| subjects | Apertures Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Atomizing Chemical engineering Compressed air Computer simulation Denitrification Droplets Earth and Environmental Science Ecotoxicology Efficiency Environment Environmental Chemistry Environmental Health Environmental science Flow rates Flow velocity Flue gas Gas flow Hydrogen peroxide Mathematical models Nitrogen Nitrogen oxides Nitrogen removal Nozzles Oxidation Oxides pH effects Photochemicals Research Article Residence time distribution Simulation Subsystems Sulfur Sulfur dioxide Temperature effects Vaporization Waste Water Technology Water Management Water Pollution Control |
| title | Simultaneous removal of nitrogen oxides and sulfur dioxide using ultrasonically atomized hydrogen peroxide |
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