Hydrous ferric oxide nanoparticles hosted porous polyethersulfone adsorptive membrane: chromium (VI) adsorptive studies and its applicability for water/wastewater treatment
In this present study, adsorptive membranes for Cr(VI) ion removal were prepared by blending polyethersulfone (PES) with hydrous ferric oxide (HFO) nanoparticles (NPs). The effects of HFO NPs to PES weight ratio (0–1.5) on the physicochemical properties of the resultant HFO/PES adsorptive membranes...
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Veröffentlicht in: | Environmental science and pollution research international 2019-07, Vol.26 (20), p.20386-20399 |
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creator | Abdullah, Norfadhilatuladha Yusof, Norhaniza Abu Shah, Muhammad Hafiz Wan Ikhsan, Syarifah Nazirah Ng, Zhi-Chien Maji, Subrata Lau, Woei Jye Jaafar, Juhana Ismail, Ahmad Fauzi Ariga, Katsuhiko |
description | In this present study, adsorptive membranes for Cr(VI) ion removal were prepared by blending polyethersulfone (PES) with hydrous ferric oxide (HFO) nanoparticles (NPs). The effects of HFO NPs to PES weight ratio (0–1.5) on the physicochemical properties of the resultant HFO/PES adsorptive membranes were investigated with respect to the surface chemistry and roughness as well as structural morphologies using different analytical instruments. The adsorptive performance of the HFO NPs/PES membranes was studied via batch adsorption experiments under various conditions by varying solution pH, initial concentration of Cr(VI), and contact time. The results showed that the membrane made of HFO/PES at a weight ratio of 1.0 exhibited the highest adsorption capacity which is 13.5 mg/g. Isotherm and kinetic studies revealed that the mechanism is best fitted to the Langmuir model and pseudo-second-order model. For filtration of Cr(VI), the best promising membranes showed improved water flux (629.3 L/m
2
h) with Cr(VI) ion removal of 75%. More importantly, the newly developed membrane maintained the Cr(VI) concentration below the maximum contamination level (MCL) for up to 9 h. |
doi_str_mv | 10.1007/s11356-019-05208-9 |
format | Article |
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2
h) with Cr(VI) ion removal of 75%. More importantly, the newly developed membrane maintained the Cr(VI) concentration below the maximum contamination level (MCL) for up to 9 h.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-019-05208-9</identifier><identifier>PMID: 31102226</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorption ; Adsorptivity ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Blending effects ; Chromium ; Contamination ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Ferric oxide ; Hematite ; Membranes ; Morphology ; Nanoparticles ; Organic chemistry ; Physicochemical properties ; Polyethersulfones ; Research Article ; Surface chemistry ; Waste Water Technology ; Wastewater treatment ; Water Management ; Water Pollution Control ; Water purification ; Water treatment ; Weight</subject><ispartof>Environmental science and pollution research international, 2019-07, Vol.26 (20), p.20386-20399</ispartof><rights>Springer-Verlag GmbH Germany, part of Springer Nature 2019</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, (2019). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c478t-f238a8005c4669c280a327460e03c8a9c8df80f3b4a5e9a062adf4243e369c473</citedby><cites>FETCH-LOGICAL-c478t-f238a8005c4669c280a327460e03c8a9c8df80f3b4a5e9a062adf4243e369c473</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-019-05208-9$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-019-05208-9$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/31102226$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Abdullah, Norfadhilatuladha</creatorcontrib><creatorcontrib>Yusof, Norhaniza</creatorcontrib><creatorcontrib>Abu Shah, Muhammad Hafiz</creatorcontrib><creatorcontrib>Wan Ikhsan, Syarifah Nazirah</creatorcontrib><creatorcontrib>Ng, Zhi-Chien</creatorcontrib><creatorcontrib>Maji, Subrata</creatorcontrib><creatorcontrib>Lau, Woei Jye</creatorcontrib><creatorcontrib>Jaafar, Juhana</creatorcontrib><creatorcontrib>Ismail, Ahmad Fauzi</creatorcontrib><creatorcontrib>Ariga, Katsuhiko</creatorcontrib><title>Hydrous ferric oxide nanoparticles hosted porous polyethersulfone adsorptive membrane: chromium (VI) adsorptive studies and its applicability for water/wastewater treatment</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>In this present study, adsorptive membranes for Cr(VI) ion removal were prepared by blending polyethersulfone (PES) with hydrous ferric oxide (HFO) nanoparticles (NPs). The effects of HFO NPs to PES weight ratio (0–1.5) on the physicochemical properties of the resultant HFO/PES adsorptive membranes were investigated with respect to the surface chemistry and roughness as well as structural morphologies using different analytical instruments. The adsorptive performance of the HFO NPs/PES membranes was studied via batch adsorption experiments under various conditions by varying solution pH, initial concentration of Cr(VI), and contact time. The results showed that the membrane made of HFO/PES at a weight ratio of 1.0 exhibited the highest adsorption capacity which is 13.5 mg/g. Isotherm and kinetic studies revealed that the mechanism is best fitted to the Langmuir model and pseudo-second-order model. For filtration of Cr(VI), the best promising membranes showed improved water flux (629.3 L/m
2
h) with Cr(VI) ion removal of 75%. More importantly, the newly developed membrane maintained the Cr(VI) concentration below the maximum contamination level (MCL) for up to 9 h.</description><subject>Adsorption</subject><subject>Adsorptivity</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Blending effects</subject><subject>Chromium</subject><subject>Contamination</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Ferric oxide</subject><subject>Hematite</subject><subject>Membranes</subject><subject>Morphology</subject><subject>Nanoparticles</subject><subject>Organic chemistry</subject><subject>Physicochemical properties</subject><subject>Polyethersulfones</subject><subject>Research Article</subject><subject>Surface 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Zhi-Chien</au><au>Maji, Subrata</au><au>Lau, Woei Jye</au><au>Jaafar, Juhana</au><au>Ismail, Ahmad Fauzi</au><au>Ariga, Katsuhiko</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Hydrous ferric oxide nanoparticles hosted porous polyethersulfone adsorptive membrane: chromium (VI) adsorptive studies and its applicability for water/wastewater treatment</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2019-07-01</date><risdate>2019</risdate><volume>26</volume><issue>20</issue><spage>20386</spage><epage>20399</epage><pages>20386-20399</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>In this present study, adsorptive membranes for Cr(VI) ion removal were prepared by blending polyethersulfone (PES) with hydrous ferric oxide (HFO) nanoparticles (NPs). The effects of HFO NPs to PES weight ratio (0–1.5) on the physicochemical properties of the resultant HFO/PES adsorptive membranes were investigated with respect to the surface chemistry and roughness as well as structural morphologies using different analytical instruments. The adsorptive performance of the HFO NPs/PES membranes was studied via batch adsorption experiments under various conditions by varying solution pH, initial concentration of Cr(VI), and contact time. The results showed that the membrane made of HFO/PES at a weight ratio of 1.0 exhibited the highest adsorption capacity which is 13.5 mg/g. Isotherm and kinetic studies revealed that the mechanism is best fitted to the Langmuir model and pseudo-second-order model. For filtration of Cr(VI), the best promising membranes showed improved water flux (629.3 L/m
2
h) with Cr(VI) ion removal of 75%. More importantly, the newly developed membrane maintained the Cr(VI) concentration below the maximum contamination level (MCL) for up to 9 h.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>31102226</pmid><doi>10.1007/s11356-019-05208-9</doi><tpages>14</tpages></addata></record> |
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subjects | Adsorption Adsorptivity Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Blending effects Chromium Contamination Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental science Ferric oxide Hematite Membranes Morphology Nanoparticles Organic chemistry Physicochemical properties Polyethersulfones Research Article Surface chemistry Waste Water Technology Wastewater treatment Water Management Water Pollution Control Water purification Water treatment Weight |
title | Hydrous ferric oxide nanoparticles hosted porous polyethersulfone adsorptive membrane: chromium (VI) adsorptive studies and its applicability for water/wastewater treatment |
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