Pulsed EPR Dipolar Spectroscopy under the Breakdown of the High‐Field Approximation: The High‐Spin Iron(III) Case

Pulsed EPR dipolar spectroscopy (PDS) offers several methods for measuring dipolar coupling and thus the distance between electron‐spin centers. To date, PDS measurements to metal centers were limited to ions that adhere to the high‐field approximation. Here, the PDS methodology is extended to cases...

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