Evaluation of hydrochar efficiency for simultaneous removal of diclofenac and ibuprofen from aqueous system using surface response methodology
Pharmaceutically active compounds like diclofenac (DFS), ibuprofen (IBP), and other drugs that persist in the environment are listed as emerging contaminants. These escape from normal wastewater treatment plants and find their way to water streams; therefore, alternate treatment processes are needed...
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| Veröffentlicht in: | Environmental science and pollution research international 2019-04, Vol.26 (10), p.9796-9804 |
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| creator | Qureshi, Tahira Memon, Najma Memon, Saima Q. Yavuz, Handan Lachgar, Abdesadek Denizli, Adil |
| description | Pharmaceutically active compounds like diclofenac (DFS), ibuprofen (IBP), and other drugs that persist in the environment are listed as emerging contaminants. These escape from normal wastewater treatment plants and find their way to water streams; therefore, alternate treatment processes are needed. Herein, a sorbent material is reported that is prepared through hydrotermal carbonization from dried fruit powder of
Zizipus mauritiana
L
.
(HTC-ZM) and applied for simultaneous removal of DFS and IBP. Carbonized material (HTC-ZM) was found as agglomerates of approximately 1 μm particle size with surface area of 1160 m
2
/g having oxygen functional groups (e.g., COO, O, C=O) on surface. Simultaneous removal of IBP and DFS onto HTC-ZM was studied using response surface methodology with a set of 18 experiments using factors such as pH, amount of sorbent, contact time, and sorbate concentration. Maximum removal efficiency was obtained 88% and 97% for DFS and for IBP, respectively, with adsorption capacity of 2.03 mmol g
−1
for DFS and 2.54 mmol g
−1
for IBP. Kinetics modeling and “mean free energy” values predicted that sorption is mainly governed by physical interactions followed by “pore filling” mechanism for uptake of DFS and IBP. |
| doi_str_mv | 10.1007/s11356-019-04359-z |
| format | Article |
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Zizipus mauritiana
L
.
(HTC-ZM) and applied for simultaneous removal of DFS and IBP. Carbonized material (HTC-ZM) was found as agglomerates of approximately 1 μm particle size with surface area of 1160 m
2
/g having oxygen functional groups (e.g., COO, O, C=O) on surface. Simultaneous removal of IBP and DFS onto HTC-ZM was studied using response surface methodology with a set of 18 experiments using factors such as pH, amount of sorbent, contact time, and sorbate concentration. Maximum removal efficiency was obtained 88% and 97% for DFS and for IBP, respectively, with adsorption capacity of 2.03 mmol g
−1
for DFS and 2.54 mmol g
−1
for IBP. Kinetics modeling and “mean free energy” values predicted that sorption is mainly governed by physical interactions followed by “pore filling” mechanism for uptake of DFS and IBP.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-019-04359-z</identifier><identifier>PMID: 30729442</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorption ; Agglomerates ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Carbon - chemistry ; Carbonization ; Charcoal - chemistry ; Contaminants ; Diclofenac ; Diclofenac - analysis ; Diclofenac - chemistry ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Free energy ; Functional groups ; Ibuprofen ; Ibuprofen - analysis ; Ibuprofen - chemistry ; Kinetics ; Nonsteroidal anti-inflammatory drugs ; Particle Size ; Powder ; Research Article ; Response surface methodology ; Sorbents ; Waste Disposal, Fluid - methods ; Waste Water ; Waste Water Technology ; Wastewater treatment ; Wastewater treatment plants ; Water Management ; Water Pollutants, Chemical - analysis ; Water Pollutants, Chemical - chemistry ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2019-04, Vol.26 (10), p.9796-9804</ispartof><rights>Springer-Verlag GmbH Germany, part of Springer Nature 2019. corrected publication 2019</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, (2019). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c412t-ac5ea142d20f6e83e665912a128c535018d0106118169a92878b31eacc9f20983</citedby><cites>FETCH-LOGICAL-c412t-ac5ea142d20f6e83e665912a128c535018d0106118169a92878b31eacc9f20983</cites><orcidid>0000-0002-6424-7462</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-019-04359-z$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-019-04359-z$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/30729442$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Qureshi, Tahira</creatorcontrib><creatorcontrib>Memon, Najma</creatorcontrib><creatorcontrib>Memon, Saima Q.</creatorcontrib><creatorcontrib>Yavuz, Handan</creatorcontrib><creatorcontrib>Lachgar, Abdesadek</creatorcontrib><creatorcontrib>Denizli, Adil</creatorcontrib><title>Evaluation of hydrochar efficiency for simultaneous removal of diclofenac and ibuprofen from aqueous system using surface response methodology</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Pharmaceutically active compounds like diclofenac (DFS), ibuprofen (IBP), and other drugs that persist in the environment are listed as emerging contaminants. These escape from normal wastewater treatment plants and find their way to water streams; therefore, alternate treatment processes are needed. Herein, a sorbent material is reported that is prepared through hydrotermal carbonization from dried fruit powder of
Zizipus mauritiana
L
.
(HTC-ZM) and applied for simultaneous removal of DFS and IBP. Carbonized material (HTC-ZM) was found as agglomerates of approximately 1 μm particle size with surface area of 1160 m
2
/g having oxygen functional groups (e.g., COO, O, C=O) on surface. Simultaneous removal of IBP and DFS onto HTC-ZM was studied using response surface methodology with a set of 18 experiments using factors such as pH, amount of sorbent, contact time, and sorbate concentration. Maximum removal efficiency was obtained 88% and 97% for DFS and for IBP, respectively, with adsorption capacity of 2.03 mmol g
−1
for DFS and 2.54 mmol g
−1
for IBP. Kinetics modeling and “mean free energy” values predicted that sorption is mainly governed by physical interactions followed by “pore filling” mechanism for uptake of DFS and IBP.</description><subject>Adsorption</subject><subject>Agglomerates</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Carbon - chemistry</subject><subject>Carbonization</subject><subject>Charcoal - chemistry</subject><subject>Contaminants</subject><subject>Diclofenac</subject><subject>Diclofenac - analysis</subject><subject>Diclofenac - chemistry</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Free energy</subject><subject>Functional groups</subject><subject>Ibuprofen</subject><subject>Ibuprofen - analysis</subject><subject>Ibuprofen - chemistry</subject><subject>Kinetics</subject><subject>Nonsteroidal anti-inflammatory drugs</subject><subject>Particle Size</subject><subject>Powder</subject><subject>Research Article</subject><subject>Response surface methodology</subject><subject>Sorbents</subject><subject>Waste Disposal, Fluid - methods</subject><subject>Waste Water</subject><subject>Waste Water Technology</subject><subject>Wastewater treatment</subject><subject>Wastewater treatment plants</subject><subject>Water Management</subject><subject>Water Pollutants, Chemical - analysis</subject><subject>Water Pollutants, Chemical - chemistry</subject><subject>Water Pollution Control</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp9kc2OFCEUhYnROO3oC7gwJG7clHKBomBpJuNPMokbXROagm4mVdBCYVLzED6z9NSoiQtXhNzvHA73IPQSyFsgZHhXAFgvOgKqI5z1qrt7hHYggHcDV-ox2hHFeQeM8wv0rJRbQihRdHiKLhgZaJvRHfp5_cNM1SwhRZw8Pq5jTvZoMnbeBxtctCv2KeMS5jotJrpUC85uTk12FozBTsm7aCw2ccRhX0_5fMc-pxmb7_VeUNayuBnXEuIBl5q9sa65lFOKxeHZLcc0pikd1ufoiTdTcS8ezkv07cP116tP3c2Xj5-v3t90lgNdOmN7Z4DTkRIvnGROiF4BNUCl7VlPQI4EiACQIJRRVA5yz8AZa5VvO5DsEr3ZfFvalrEseg7FumnafqgpqLZiqaRq6Ot_0NtUc2zpGjWIXihFhkbRjbI5lZKd16ccZpNXDUSf29JbW7q1pe_b0ndN9OrBuu5nN_6R_K6nAWwDShvFg8t_3_6P7S85YaLe</recordid><startdate>20190401</startdate><enddate>20190401</enddate><creator>Qureshi, Tahira</creator><creator>Memon, Najma</creator><creator>Memon, Saima Q.</creator><creator>Yavuz, Handan</creator><creator>Lachgar, Abdesadek</creator><creator>Denizli, Adil</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QL</scope><scope>7SN</scope><scope>7T7</scope><scope>7TV</scope><scope>7U7</scope><scope>7WY</scope><scope>7WZ</scope><scope>7X7</scope><scope>7XB</scope><scope>87Z</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8FL</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BEZIV</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FRNLG</scope><scope>FYUFA</scope><scope>F~G</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K60</scope><scope>K6~</scope><scope>K9.</scope><scope>L.-</scope><scope>M0C</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7N</scope><scope>P64</scope><scope>PATMY</scope><scope>PQBIZ</scope><scope>PQBZA</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-6424-7462</orcidid></search><sort><creationdate>20190401</creationdate><title>Evaluation of hydrochar efficiency for simultaneous removal of diclofenac and ibuprofen from aqueous system using surface response methodology</title><author>Qureshi, Tahira ; Memon, Najma ; Memon, Saima Q. ; Yavuz, Handan ; Lachgar, Abdesadek ; Denizli, Adil</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c412t-ac5ea142d20f6e83e665912a128c535018d0106118169a92878b31eacc9f20983</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Adsorption</topic><topic>Agglomerates</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Carbon - 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Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Qureshi, Tahira</au><au>Memon, Najma</au><au>Memon, Saima Q.</au><au>Yavuz, Handan</au><au>Lachgar, Abdesadek</au><au>Denizli, Adil</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Evaluation of hydrochar efficiency for simultaneous removal of diclofenac and ibuprofen from aqueous system using surface response methodology</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2019-04-01</date><risdate>2019</risdate><volume>26</volume><issue>10</issue><spage>9796</spage><epage>9804</epage><pages>9796-9804</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Pharmaceutically active compounds like diclofenac (DFS), ibuprofen (IBP), and other drugs that persist in the environment are listed as emerging contaminants. These escape from normal wastewater treatment plants and find their way to water streams; therefore, alternate treatment processes are needed. Herein, a sorbent material is reported that is prepared through hydrotermal carbonization from dried fruit powder of
Zizipus mauritiana
L
.
(HTC-ZM) and applied for simultaneous removal of DFS and IBP. Carbonized material (HTC-ZM) was found as agglomerates of approximately 1 μm particle size with surface area of 1160 m
2
/g having oxygen functional groups (e.g., COO, O, C=O) on surface. Simultaneous removal of IBP and DFS onto HTC-ZM was studied using response surface methodology with a set of 18 experiments using factors such as pH, amount of sorbent, contact time, and sorbate concentration. Maximum removal efficiency was obtained 88% and 97% for DFS and for IBP, respectively, with adsorption capacity of 2.03 mmol g
−1
for DFS and 2.54 mmol g
−1
for IBP. Kinetics modeling and “mean free energy” values predicted that sorption is mainly governed by physical interactions followed by “pore filling” mechanism for uptake of DFS and IBP.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>30729442</pmid><doi>10.1007/s11356-019-04359-z</doi><tpages>9</tpages><orcidid>https://orcid.org/0000-0002-6424-7462</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0944-1344 |
| ispartof | Environmental science and pollution research international, 2019-04, Vol.26 (10), p.9796-9804 |
| issn | 0944-1344 1614-7499 |
| language | eng |
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| source | MEDLINE; SpringerLink Journals - AutoHoldings |
| subjects | Adsorption Agglomerates Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Carbon - chemistry Carbonization Charcoal - chemistry Contaminants Diclofenac Diclofenac - analysis Diclofenac - chemistry Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental science Free energy Functional groups Ibuprofen Ibuprofen - analysis Ibuprofen - chemistry Kinetics Nonsteroidal anti-inflammatory drugs Particle Size Powder Research Article Response surface methodology Sorbents Waste Disposal, Fluid - methods Waste Water Waste Water Technology Wastewater treatment Wastewater treatment plants Water Management Water Pollutants, Chemical - analysis Water Pollutants, Chemical - chemistry Water Pollution Control |
| title | Evaluation of hydrochar efficiency for simultaneous removal of diclofenac and ibuprofen from aqueous system using surface response methodology |
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