Effective high-order harmonic generation from metal sulfide quantum dots
In the past, common media for high-order harmonic generation (HHG) has been atoms and molecules. More recently, clusters, and nanoparticles have been introduced as HHG emitting media. Multi-particle media can enhance HHG yields but have more stringent requirements in determining the optimal paramete...
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| Veröffentlicht in: | Optics express 2018-12, Vol.26 (26), p.35013-35025 |
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| container_title | Optics express |
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| creator | Ganeev, Rashid A Boltaev, Ganjaboy S Kim, Vyacheslav V Zhang, Ke Zvyagin, Andrey I Smirnov, Michail S Ovchinnikov, Oleg V Redkin, Pavel V Wöstmann, Michael Zacharias, Helmut Guo, Chunlei |
| description | In the past, common media for high-order harmonic generation (HHG) has been atoms and molecules. More recently, clusters, and nanoparticles have been introduced as HHG emitting media. Multi-particle media can enhance HHG yields but have more stringent requirements in determining the optimal parameters. Here, we demonstrate, for the first time, the effective application of 1-3 nm metal sulfide quantum dots (QDs) for harmonic generation in the 20 - 115 nm extreme ultraviolet range. We report on the syntheses, ablation of Ag
S, CdS, and ZnS QDs, and HHG from laser-produced plasmas by using single- and two-color pumps. We compare HHG efficiency from the ablated QDs to that of bulk metal sulfides and show a seven-fold increase in harmonic yields. Further, the study also allows us to understand the effects of QD-contained plasma spreading dynamics on HHG yield. |
| doi_str_mv | 10.1364/OE.26.035013 |
| format | Article |
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| source | DOAJ Directory of Open Access Journals; EZB-FREE-00999 freely available EZB journals; Alma/SFX Local Collection |
| title | Effective high-order harmonic generation from metal sulfide quantum dots |
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