Stable carbon and nitrogen isotopic composition of PM10 over Indo-Gangetic Plains (IGP), adjoining regions and Indo-Himalayan Range (IHR) during a winter 2014 campaign

For source identification, a field campaign involving simultaneous sampling of particulate matter (PM 10 ) was conducted at eight sampling sites in the Indian mainland during winter 2014. The sampling sites include Delhi (upper IGP), Lucknow (middle IGP), and Kolkata (lower IGP) in the Indo-Gangetic...

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Veröffentlicht in:Environmental science and pollution research international 2018-09, Vol.25 (26), p.26279-26296
Hauptverfasser: Sen, Avirup, Karapurkar, Supriya G., Saxena, Mohit, Shenoy, Damodar M., Chaterjee, Abhijit, Choudhuri, Anil K., Das, Trupti, Khan, Altaf H., Kuniyal, Jagdish Chandra, Pal, Srimata, Singh, Dharam Pal, Sharma, Sudhir Kumar, Kotnala, Ravindra Kumar, Mandal, Tuhin Kumar
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container_end_page 26296
container_issue 26
container_start_page 26279
container_title Environmental science and pollution research international
container_volume 25
creator Sen, Avirup
Karapurkar, Supriya G.
Saxena, Mohit
Shenoy, Damodar M.
Chaterjee, Abhijit
Choudhuri, Anil K.
Das, Trupti
Khan, Altaf H.
Kuniyal, Jagdish Chandra
Pal, Srimata
Singh, Dharam Pal
Sharma, Sudhir Kumar
Kotnala, Ravindra Kumar
Mandal, Tuhin Kumar
description For source identification, a field campaign involving simultaneous sampling of particulate matter (PM 10 ) was conducted at eight sampling sites in the Indian mainland during winter 2014. The sampling sites include Delhi (upper IGP), Lucknow (middle IGP), and Kolkata (lower IGP) in the Indo-Gangetic Plains (IGP); Mohal-Kullu and Darjeeling in the Indo-Himalayan Range (IHR). In addition, Ajmer, located upwind of the IGP in NW-India and Giridih and Bhubaneswar, in the downwind to the IGP has also been chosen. To characterize the sources of the ambient PM 10 , stable isotope ratios of carbon (δ 13 C TC ) and nitrogen (δ 15 N TN ) for the total carbon (TC) and total nitrogen (TN) fractions have been considered. Ancillary chemical parameters, such as organic carbon (OC), elemental carbon (EC), and water-soluble ionic components (WSIC) mass concentrations are also presented in this paper. There was very small variation in the daily average δ 13 C TC ratios (− 24.8 to − 25.9‰) among the sites. Comparison with end-member stable C isotopic signatures of major typical sources suggests that the PM 10 at the sites was mainly from fossil fuel and biofuel and biomass combustion. Daily average δ 15 N TN ratios were not observed to vary much between sites either (8.3 to 11.0‰), and the low δ 15 N TN levels also indicate substantial contributions from biofuel and biomass burning of primarily C3 andC4 plant matter. Graphical abstract Scatter plot of the average (± 1 standard deviation (SD)) δ 13 C TC (‰) compared to δ 15 N TN (‰) at the sampling sites.
doi_str_mv 10.1007/s11356-018-2567-0
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The sampling sites include Delhi (upper IGP), Lucknow (middle IGP), and Kolkata (lower IGP) in the Indo-Gangetic Plains (IGP); Mohal-Kullu and Darjeeling in the Indo-Himalayan Range (IHR). In addition, Ajmer, located upwind of the IGP in NW-India and Giridih and Bhubaneswar, in the downwind to the IGP has also been chosen. To characterize the sources of the ambient PM 10 , stable isotope ratios of carbon (δ 13 C TC ) and nitrogen (δ 15 N TN ) for the total carbon (TC) and total nitrogen (TN) fractions have been considered. Ancillary chemical parameters, such as organic carbon (OC), elemental carbon (EC), and water-soluble ionic components (WSIC) mass concentrations are also presented in this paper. There was very small variation in the daily average δ 13 C TC ratios (− 24.8 to − 25.9‰) among the sites. Comparison with end-member stable C isotopic signatures of major typical sources suggests that the PM 10 at the sites was mainly from fossil fuel and biofuel and biomass combustion. 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Daily average δ 15 N TN ratios were not observed to vary much between sites either (8.3 to 11.0‰), and the low δ 15 N TN levels also indicate substantial contributions from biofuel and biomass burning of primarily C3 andC4 plant matter. 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Daily average δ 15 N TN ratios were not observed to vary much between sites either (8.3 to 11.0‰), and the low δ 15 N TN levels also indicate substantial contributions from biofuel and biomass burning of primarily C3 andC4 plant matter. Graphical abstract Scatter plot of the average (± 1 standard deviation (SD)) δ 13 C TC (‰) compared to δ 15 N TN (‰) at the sampling sites.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s11356-018-2567-0</doi><tpages>18</tpages><orcidid>https://orcid.org/0000-0003-0142-1512</orcidid></addata></record>
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ispartof Environmental science and pollution research international, 2018-09, Vol.25 (26), p.26279-26296
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1614-7499
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source SpringerLink Journals - AutoHoldings
subjects Aquatic Pollution
Atmospheric Protection/Air Quality Control/Air Pollution
Biodiesel fuels
Biofuels
Biomass
Biomass burning
Burning
Carbon
combustion
Earth and Environmental Science
Ecotoxicology
Environment
Environmental Chemistry
Environmental Health
Environmental science
Fossil fuels
India
Indo-Gangetic Plain
Isotope ratios
Isotopes
Nitrogen
Organic carbon
Organic chemistry
Particulate emissions
Particulate matter
particulates
Research Article
Sampling
Stable isotopes
standard deviation
total nitrogen
Waste Water Technology
Water Management
Water Pollution Control
water solubility
Winter
title Stable carbon and nitrogen isotopic composition of PM10 over Indo-Gangetic Plains (IGP), adjoining regions and Indo-Himalayan Range (IHR) during a winter 2014 campaign
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