Dioxygen Activation on Cu-MOR Zeolite: Theoretical Insights into the Formation of Cu2O and Cu3O3 Active Species

The utilization of low-cost and abundant oxygen (O2) as an oxidant in the activation of copper-exchanged zeolites is highly important for the direct, selective oxidation of methane to methanol at low temperatures. While two motifs of active sites, i.e., the [Cu2(μ-O)]2+ and [Cu3(μ-O)3]2+, have been...

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Veröffentlicht in:	Inorganic chemistry 2018-08, Vol.57 (16), p.10146-10152
Hauptverfasser:	Mahyuddin, M. Haris, Tanaka, Takahiro, Staykov, Aleksandar, Shiota, Yoshihito, Yoshizawa, Kazunari
Format:	Artikel
Sprache:	eng
Online-Zugang:	Volltext
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