Harmonic Generation from Neutral Manganese Atoms in the Vicinity of the Giant Autoionization Resonance
High harmonics from laser-ablated plumes are mostly generated from ionic species. We demonstrate that with ultrashort infrared (∼1.82 μm) driving lasers, high harmonics from laser-ablated manganese are predominantly generated from neutral atoms, a transition metal atom with an ionization potential...
Gespeichert in:
| Veröffentlicht in: | Physical review letters 2018-07, Vol.121 (2), p.023201-023201, Article 023201 |
|---|---|
| Hauptverfasser: | , , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 023201 |
|---|---|
| container_issue | 2 |
| container_start_page | 023201 |
| container_title | Physical review letters |
| container_volume | 121 |
| creator | Fareed, M A Strelkov, V V Singh, M Thiré, N Mondal, S Schmidt, B E Légaré, F Ozaki, T |
| description | High harmonics from laser-ablated plumes are mostly generated from ionic species. We demonstrate that with ultrashort infrared (∼1.82 μm) driving lasers, high harmonics from laser-ablated manganese are predominantly generated from neutral atoms, a transition metal atom with an ionization potential of 7.4 eV. Our results open the possibility to advance laser-ablation technique to study the dynamics of neutral atoms of low ionization potential. Moreover, as manganese contains giant autoionizing resonance, intense and broadband high harmonics have been demonstrated from this resonance at energies from 49 to 53 eV. This opens the possibility to generate intense attosecond pulses directly from the giant resonances, as well as to study these resonances using high-harmonic spectroscopy. |
| doi_str_mv | 10.1103/PhysRevLett.121.023201 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_2085659184</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2085659184</sourcerecordid><originalsourceid>FETCH-LOGICAL-c453t-fd602550e6dc107f02904a6b1e50fb245392efd62559aef2716f98f613692e403</originalsourceid><addsrcrecordid>eNpdkUFvEzEQhS1ERUPhL1SWuHDZMGPvetfHqKIpUoCqarlazmZMXWXtYnuRwq_HkIIQp9FovnmaN4-xc4QlIsh31_eHfEPfN1TKEgUuQUgB-IwtEHrd9Ijtc7YAkNhogP6Uvcz5AQBQqOEFO5UAQ9dLWDB3ZdMUgx_5mgIlW3wM3KU48U80l2T3_KMNX22gTHxV4pS5D7zcE__iRx98OfDofvdrb0Phq7nEquB_HIVuKMdgw0iv2Imz-0yvn-oZu7t8f3tx1Ww-rz9crDbN2HayNG6nQHQdkNqN1YgDoaG1aovUgduKymhBFaqMtuREj8rpwSmUqg5akGfs7VH3McVvM-ViJp9H2u-rgzhnI6pv1Wkc2oq--Q99iHMK9TojEAepUKOulDpSY4o5J3LmMfnJpoNBML-SMP8kYWoS5phEXTx_kp-3E-3-rv15vfwJZ_OGuQ</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2118361919</pqid></control><display><type>article</type><title>Harmonic Generation from Neutral Manganese Atoms in the Vicinity of the Giant Autoionization Resonance</title><source>American Physical Society Journals</source><source>EZB-FREE-00999 freely available EZB journals</source><creator>Fareed, M A ; Strelkov, V V ; Singh, M ; Thiré, N ; Mondal, S ; Schmidt, B E ; Légaré, F ; Ozaki, T</creator><creatorcontrib>Fareed, M A ; Strelkov, V V ; Singh, M ; Thiré, N ; Mondal, S ; Schmidt, B E ; Légaré, F ; Ozaki, T</creatorcontrib><description>High harmonics from laser-ablated plumes are mostly generated from ionic species. We demonstrate that with ultrashort infrared (∼1.82 μm) driving lasers, high harmonics from laser-ablated manganese are predominantly generated from neutral atoms, a transition metal atom with an ionization potential of 7.4 eV. Our results open the possibility to advance laser-ablation technique to study the dynamics of neutral atoms of low ionization potential. Moreover, as manganese contains giant autoionizing resonance, intense and broadband high harmonics have been demonstrated from this resonance at energies from 49 to 53 eV. This opens the possibility to generate intense attosecond pulses directly from the giant resonances, as well as to study these resonances using high-harmonic spectroscopy.</description><identifier>ISSN: 0031-9007</identifier><identifier>EISSN: 1079-7114</identifier><identifier>DOI: 10.1103/PhysRevLett.121.023201</identifier><identifier>PMID: 30085730</identifier><language>eng</language><publisher>United States: American Physical Society</publisher><subject>Attosecond pulses ; Autoionization ; Broadband ; Harmonic generations ; Ionization potentials ; Laser ablation ; Lasers ; Manganese ; Neutral atoms ; Transition metals</subject><ispartof>Physical review letters, 2018-07, Vol.121 (2), p.023201-023201, Article 023201</ispartof><rights>Copyright American Physical Society Jul 13, 2018</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c453t-fd602550e6dc107f02904a6b1e50fb245392efd62559aef2716f98f613692e403</citedby><cites>FETCH-LOGICAL-c453t-fd602550e6dc107f02904a6b1e50fb245392efd62559aef2716f98f613692e403</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,2863,2864,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/30085730$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Fareed, M A</creatorcontrib><creatorcontrib>Strelkov, V V</creatorcontrib><creatorcontrib>Singh, M</creatorcontrib><creatorcontrib>Thiré, N</creatorcontrib><creatorcontrib>Mondal, S</creatorcontrib><creatorcontrib>Schmidt, B E</creatorcontrib><creatorcontrib>Légaré, F</creatorcontrib><creatorcontrib>Ozaki, T</creatorcontrib><title>Harmonic Generation from Neutral Manganese Atoms in the Vicinity of the Giant Autoionization Resonance</title><title>Physical review letters</title><addtitle>Phys Rev Lett</addtitle><description>High harmonics from laser-ablated plumes are mostly generated from ionic species. We demonstrate that with ultrashort infrared (∼1.82 μm) driving lasers, high harmonics from laser-ablated manganese are predominantly generated from neutral atoms, a transition metal atom with an ionization potential of 7.4 eV. Our results open the possibility to advance laser-ablation technique to study the dynamics of neutral atoms of low ionization potential. Moreover, as manganese contains giant autoionizing resonance, intense and broadband high harmonics have been demonstrated from this resonance at energies from 49 to 53 eV. This opens the possibility to generate intense attosecond pulses directly from the giant resonances, as well as to study these resonances using high-harmonic spectroscopy.</description><subject>Attosecond pulses</subject><subject>Autoionization</subject><subject>Broadband</subject><subject>Harmonic generations</subject><subject>Ionization potentials</subject><subject>Laser ablation</subject><subject>Lasers</subject><subject>Manganese</subject><subject>Neutral atoms</subject><subject>Transition metals</subject><issn>0031-9007</issn><issn>1079-7114</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNpdkUFvEzEQhS1ERUPhL1SWuHDZMGPvetfHqKIpUoCqarlazmZMXWXtYnuRwq_HkIIQp9FovnmaN4-xc4QlIsh31_eHfEPfN1TKEgUuQUgB-IwtEHrd9Ijtc7YAkNhogP6Uvcz5AQBQqOEFO5UAQ9dLWDB3ZdMUgx_5mgIlW3wM3KU48U80l2T3_KMNX22gTHxV4pS5D7zcE__iRx98OfDofvdrb0Phq7nEquB_HIVuKMdgw0iv2Imz-0yvn-oZu7t8f3tx1Ww-rz9crDbN2HayNG6nQHQdkNqN1YgDoaG1aovUgduKymhBFaqMtuREj8rpwSmUqg5akGfs7VH3McVvM-ViJp9H2u-rgzhnI6pv1Wkc2oq--Q99iHMK9TojEAepUKOulDpSY4o5J3LmMfnJpoNBML-SMP8kYWoS5phEXTx_kp-3E-3-rv15vfwJZ_OGuQ</recordid><startdate>20180713</startdate><enddate>20180713</enddate><creator>Fareed, M A</creator><creator>Strelkov, V V</creator><creator>Singh, M</creator><creator>Thiré, N</creator><creator>Mondal, S</creator><creator>Schmidt, B E</creator><creator>Légaré, F</creator><creator>Ozaki, T</creator><general>American Physical Society</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><scope>7X8</scope></search><sort><creationdate>20180713</creationdate><title>Harmonic Generation from Neutral Manganese Atoms in the Vicinity of the Giant Autoionization Resonance</title><author>Fareed, M A ; Strelkov, V V ; Singh, M ; Thiré, N ; Mondal, S ; Schmidt, B E ; Légaré, F ; Ozaki, T</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c453t-fd602550e6dc107f02904a6b1e50fb245392efd62559aef2716f98f613692e403</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Attosecond pulses</topic><topic>Autoionization</topic><topic>Broadband</topic><topic>Harmonic generations</topic><topic>Ionization potentials</topic><topic>Laser ablation</topic><topic>Lasers</topic><topic>Manganese</topic><topic>Neutral atoms</topic><topic>Transition metals</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Fareed, M A</creatorcontrib><creatorcontrib>Strelkov, V V</creatorcontrib><creatorcontrib>Singh, M</creatorcontrib><creatorcontrib>Thiré, N</creatorcontrib><creatorcontrib>Mondal, S</creatorcontrib><creatorcontrib>Schmidt, B E</creatorcontrib><creatorcontrib>Légaré, F</creatorcontrib><creatorcontrib>Ozaki, T</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Physical review letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Fareed, M A</au><au>Strelkov, V V</au><au>Singh, M</au><au>Thiré, N</au><au>Mondal, S</au><au>Schmidt, B E</au><au>Légaré, F</au><au>Ozaki, T</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Harmonic Generation from Neutral Manganese Atoms in the Vicinity of the Giant Autoionization Resonance</atitle><jtitle>Physical review letters</jtitle><addtitle>Phys Rev Lett</addtitle><date>2018-07-13</date><risdate>2018</risdate><volume>121</volume><issue>2</issue><spage>023201</spage><epage>023201</epage><pages>023201-023201</pages><artnum>023201</artnum><issn>0031-9007</issn><eissn>1079-7114</eissn><abstract>High harmonics from laser-ablated plumes are mostly generated from ionic species. We demonstrate that with ultrashort infrared (∼1.82 μm) driving lasers, high harmonics from laser-ablated manganese are predominantly generated from neutral atoms, a transition metal atom with an ionization potential of 7.4 eV. Our results open the possibility to advance laser-ablation technique to study the dynamics of neutral atoms of low ionization potential. Moreover, as manganese contains giant autoionizing resonance, intense and broadband high harmonics have been demonstrated from this resonance at energies from 49 to 53 eV. This opens the possibility to generate intense attosecond pulses directly from the giant resonances, as well as to study these resonances using high-harmonic spectroscopy.</abstract><cop>United States</cop><pub>American Physical Society</pub><pmid>30085730</pmid><doi>10.1103/PhysRevLett.121.023201</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0031-9007 |
| ispartof | Physical review letters, 2018-07, Vol.121 (2), p.023201-023201, Article 023201 |
| issn | 0031-9007 1079-7114 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_2085659184 |
| source | American Physical Society Journals; EZB-FREE-00999 freely available EZB journals |
| subjects | Attosecond pulses Autoionization Broadband Harmonic generations Ionization potentials Laser ablation Lasers Manganese Neutral atoms Transition metals |
| title | Harmonic Generation from Neutral Manganese Atoms in the Vicinity of the Giant Autoionization Resonance |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-10T15%3A59%3A07IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Harmonic%20Generation%20from%20Neutral%20Manganese%20Atoms%20in%20the%20Vicinity%20of%20the%20Giant%20Autoionization%20Resonance&rft.jtitle=Physical%20review%20letters&rft.au=Fareed,%20M%20A&rft.date=2018-07-13&rft.volume=121&rft.issue=2&rft.spage=023201&rft.epage=023201&rft.pages=023201-023201&rft.artnum=023201&rft.issn=0031-9007&rft.eissn=1079-7114&rft_id=info:doi/10.1103/PhysRevLett.121.023201&rft_dat=%3Cproquest_cross%3E2085659184%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2118361919&rft_id=info:pmid/30085730&rfr_iscdi=true |