Ice nuclei emissions from biomass burning
Biomass burning is a significant source of carbonaceous aerosol in many regions of the world. When present, biomass burning particles may affect the microphysical properties of clouds through their ability to function as cloud condensation nuclei or ice nuclei. We report on measurements of the ice n...
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Veröffentlicht in: | Journal of Geophysical Research - Atmospheres 2009-05, Vol.114 (D7), p.D07209-n/a |
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creator | Petters, Markus D. Parsons, Matthew T. Prenni, Anthony J. DeMott, Paul J. Kreidenweis, Sonia M. Carrico, Christian M. Sullivan, Amy P. McMeeking, Gavin R. Levin, Ezra Wold, Cyle E. Collett Jr, Jeffrey L. Moosmüller, Hans |
description | Biomass burning is a significant source of carbonaceous aerosol in many regions of the world. When present, biomass burning particles may affect the microphysical properties of clouds through their ability to function as cloud condensation nuclei or ice nuclei. We report on measurements of the ice nucleation ability of biomass burning particles performed on laboratory‐generated aerosols at the second Fire Lab at Missoula Experiment. During the experiment we generated smoke through controlled burns of 21 biomass fuels from the United States and Asia. Using a Colorado State University continuous flow diffusion chamber, we measured the condensation/immersion freezing potential at temperatures relevant to cold cumulus clouds (−30°C). Smokes from 9 of the 21 fuels acted as ice nuclei at fractions of 1:10,000 to 1:100 particles in at least one burn of each fuel; emissions from the remaining fuels were below the ice nuclei detection limit for all burns of each fuel. Using a bottom‐up emission model, we estimate that smokes that emit ice nuclei fractions exceeding 1:10,000 particles can perturb ice nuclei concentrations on a regional scale. |
doi_str_mv | 10.1029/2008JD011532 |
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When present, biomass burning particles may affect the microphysical properties of clouds through their ability to function as cloud condensation nuclei or ice nuclei. We report on measurements of the ice nucleation ability of biomass burning particles performed on laboratory‐generated aerosols at the second Fire Lab at Missoula Experiment. During the experiment we generated smoke through controlled burns of 21 biomass fuels from the United States and Asia. Using a Colorado State University continuous flow diffusion chamber, we measured the condensation/immersion freezing potential at temperatures relevant to cold cumulus clouds (−30°C). Smokes from 9 of the 21 fuels acted as ice nuclei at fractions of 1:10,000 to 1:100 particles in at least one burn of each fuel; emissions from the remaining fuels were below the ice nuclei detection limit for all burns of each fuel. Using a bottom‐up emission model, we estimate that smokes that emit ice nuclei fractions exceeding 1:10,000 particles can perturb ice nuclei concentrations on a regional scale.</description><identifier>ISSN: 0148-0227</identifier><identifier>ISSN: 2169-897X</identifier><identifier>EISSN: 2156-2202</identifier><identifier>EISSN: 2169-8996</identifier><identifier>DOI: 10.1029/2008JD011532</identifier><language>eng</language><publisher>Washington, DC: American Geophysical Union</publisher><subject>aerosol-cloud interactions ; Aerosols and particles ; Atmospheric Composition and Structure ; biomass burning ; Biosphere/atmosphere interactions ; Cloud physics and chemistry ; Cloud/radiation interaction ; Earth sciences ; Earth, ocean, space ; Exact sciences and technology ; ice nuclei</subject><ispartof>Journal of Geophysical Research - Atmospheres, 2009-05, Vol.114 (D7), p.D07209-n/a</ispartof><rights>2008 American Geophysical Union</rights><rights>Copyright 2009 by the American Geophysical Union.</rights><rights>2009 INIST-CNRS</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a5315-b2f013d168d4d50d3994c14d925242ebc733c7633d14aa3e805c4a711ec5f013</citedby><cites>FETCH-LOGICAL-a5315-b2f013d168d4d50d3994c14d925242ebc733c7633d14aa3e805c4a711ec5f013</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1029%2F2008JD011532$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1029%2F2008JD011532$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>315,782,786,1419,1435,11523,27933,27934,45583,45584,46418,46477,46842,46901</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=21453692$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Petters, Markus D.</creatorcontrib><creatorcontrib>Parsons, Matthew T.</creatorcontrib><creatorcontrib>Prenni, Anthony J.</creatorcontrib><creatorcontrib>DeMott, Paul J.</creatorcontrib><creatorcontrib>Kreidenweis, Sonia M.</creatorcontrib><creatorcontrib>Carrico, Christian M.</creatorcontrib><creatorcontrib>Sullivan, Amy P.</creatorcontrib><creatorcontrib>McMeeking, Gavin R.</creatorcontrib><creatorcontrib>Levin, Ezra</creatorcontrib><creatorcontrib>Wold, Cyle E.</creatorcontrib><creatorcontrib>Collett Jr, Jeffrey L.</creatorcontrib><creatorcontrib>Moosmüller, Hans</creatorcontrib><title>Ice nuclei emissions from biomass burning</title><title>Journal of Geophysical Research - Atmospheres</title><addtitle>J. Geophys. Res</addtitle><description>Biomass burning is a significant source of carbonaceous aerosol in many regions of the world. When present, biomass burning particles may affect the microphysical properties of clouds through their ability to function as cloud condensation nuclei or ice nuclei. We report on measurements of the ice nucleation ability of biomass burning particles performed on laboratory‐generated aerosols at the second Fire Lab at Missoula Experiment. During the experiment we generated smoke through controlled burns of 21 biomass fuels from the United States and Asia. Using a Colorado State University continuous flow diffusion chamber, we measured the condensation/immersion freezing potential at temperatures relevant to cold cumulus clouds (−30°C). Smokes from 9 of the 21 fuels acted as ice nuclei at fractions of 1:10,000 to 1:100 particles in at least one burn of each fuel; emissions from the remaining fuels were below the ice nuclei detection limit for all burns of each fuel. Using a bottom‐up emission model, we estimate that smokes that emit ice nuclei fractions exceeding 1:10,000 particles can perturb ice nuclei concentrations on a regional scale.</description><subject>aerosol-cloud interactions</subject><subject>Aerosols and particles</subject><subject>Atmospheric Composition and Structure</subject><subject>biomass burning</subject><subject>Biosphere/atmosphere interactions</subject><subject>Cloud physics and chemistry</subject><subject>Cloud/radiation interaction</subject><subject>Earth sciences</subject><subject>Earth, ocean, space</subject><subject>Exact sciences and technology</subject><subject>ice nuclei</subject><issn>0148-0227</issn><issn>2169-897X</issn><issn>2156-2202</issn><issn>2169-8996</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2009</creationdate><recordtype>article</recordtype><recordid>eNqF0M1LwzAYBvAgCo7pzbu9qAhW33y2OerUqgzFD_AYsjQd0a6diUX9782o6E4zlzeH3_Py8CK0g-EYA5EnBCC_OQeMOSVraEAwFykhQNbRADDLUyAk20TbIbxAfIwLBniADq-NTZrO1NYlduZCcG0Tksq3s2Ti2pkOIZl0vnHNdAttVLoOdvtnDtHT5cXT6Cod3xXXo9NxqjnFPJ2QCjAtschLVnIoqZTMYFZKwgkjdmIySk0maCRMa2pz4IbpDGNr-CI5RAf92rlv3zob3lVsZWxd68a2XVASqMASZBbl_kpJGQPBhfgXEuCc5VJGeNRD49sQvK3U3LuZ9l8Kg1ocWS0fOfK9n706GF1XXjfGhd8MwYxTIReO9u7D1fZr5U51Uzycx4_kMZX2KRfe7edvSvtXJTKacfV8W6jHy7P7cXH7rPLod3uvp91fh-W-3wvGn6c</recordid><startdate>20090501</startdate><enddate>20090501</enddate><creator>Petters, Markus D.</creator><creator>Parsons, Matthew T.</creator><creator>Prenni, Anthony J.</creator><creator>DeMott, Paul J.</creator><creator>Kreidenweis, Sonia M.</creator><creator>Carrico, Christian M.</creator><creator>Sullivan, Amy P.</creator><creator>McMeeking, Gavin R.</creator><creator>Levin, Ezra</creator><creator>Wold, Cyle E.</creator><creator>Collett Jr, Jeffrey L.</creator><creator>Moosmüller, Hans</creator><general>American Geophysical Union</general><general>Blackwell Publishing Ltd</general><scope>BSCLL</scope><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7TG</scope><scope>7TV</scope><scope>C1K</scope><scope>KL.</scope><scope>7SM</scope><scope>8FD</scope><scope>FR3</scope><scope>H8D</scope><scope>KR7</scope><scope>L7M</scope></search><sort><creationdate>20090501</creationdate><title>Ice nuclei emissions from biomass burning</title><author>Petters, Markus D. ; Parsons, Matthew T. ; Prenni, Anthony J. ; DeMott, Paul J. ; Kreidenweis, Sonia M. ; Carrico, Christian M. ; Sullivan, Amy P. ; McMeeking, Gavin R. ; Levin, Ezra ; Wold, Cyle E. ; Collett Jr, Jeffrey L. ; Moosmüller, Hans</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a5315-b2f013d168d4d50d3994c14d925242ebc733c7633d14aa3e805c4a711ec5f013</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2009</creationdate><topic>aerosol-cloud interactions</topic><topic>Aerosols and particles</topic><topic>Atmospheric Composition and Structure</topic><topic>biomass burning</topic><topic>Biosphere/atmosphere interactions</topic><topic>Cloud physics and chemistry</topic><topic>Cloud/radiation interaction</topic><topic>Earth sciences</topic><topic>Earth, ocean, space</topic><topic>Exact sciences and technology</topic><topic>ice nuclei</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Petters, Markus D.</creatorcontrib><creatorcontrib>Parsons, Matthew T.</creatorcontrib><creatorcontrib>Prenni, Anthony J.</creatorcontrib><creatorcontrib>DeMott, Paul J.</creatorcontrib><creatorcontrib>Kreidenweis, Sonia M.</creatorcontrib><creatorcontrib>Carrico, Christian M.</creatorcontrib><creatorcontrib>Sullivan, Amy P.</creatorcontrib><creatorcontrib>McMeeking, Gavin R.</creatorcontrib><creatorcontrib>Levin, Ezra</creatorcontrib><creatorcontrib>Wold, Cyle E.</creatorcontrib><creatorcontrib>Collett Jr, Jeffrey L.</creatorcontrib><creatorcontrib>Moosmüller, Hans</creatorcontrib><collection>Istex</collection><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Pollution Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Earthquake Engineering Abstracts</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Aerospace Database</collection><collection>Civil Engineering Abstracts</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Journal of Geophysical Research - Atmospheres</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Petters, Markus D.</au><au>Parsons, Matthew T.</au><au>Prenni, Anthony J.</au><au>DeMott, Paul J.</au><au>Kreidenweis, Sonia M.</au><au>Carrico, Christian M.</au><au>Sullivan, Amy P.</au><au>McMeeking, Gavin R.</au><au>Levin, Ezra</au><au>Wold, Cyle E.</au><au>Collett Jr, Jeffrey L.</au><au>Moosmüller, Hans</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Ice nuclei emissions from biomass burning</atitle><jtitle>Journal of Geophysical Research - Atmospheres</jtitle><addtitle>J. Geophys. Res</addtitle><date>2009-05-01</date><risdate>2009</risdate><volume>114</volume><issue>D7</issue><spage>D07209</spage><epage>n/a</epage><pages>D07209-n/a</pages><issn>0148-0227</issn><issn>2169-897X</issn><eissn>2156-2202</eissn><eissn>2169-8996</eissn><abstract>Biomass burning is a significant source of carbonaceous aerosol in many regions of the world. When present, biomass burning particles may affect the microphysical properties of clouds through their ability to function as cloud condensation nuclei or ice nuclei. We report on measurements of the ice nucleation ability of biomass burning particles performed on laboratory‐generated aerosols at the second Fire Lab at Missoula Experiment. During the experiment we generated smoke through controlled burns of 21 biomass fuels from the United States and Asia. Using a Colorado State University continuous flow diffusion chamber, we measured the condensation/immersion freezing potential at temperatures relevant to cold cumulus clouds (−30°C). Smokes from 9 of the 21 fuels acted as ice nuclei at fractions of 1:10,000 to 1:100 particles in at least one burn of each fuel; emissions from the remaining fuels were below the ice nuclei detection limit for all burns of each fuel. Using a bottom‐up emission model, we estimate that smokes that emit ice nuclei fractions exceeding 1:10,000 particles can perturb ice nuclei concentrations on a regional scale.</abstract><cop>Washington, DC</cop><pub>American Geophysical Union</pub><doi>10.1029/2008JD011532</doi><tpages>10</tpages><oa>free_for_read</oa></addata></record> |
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subjects | aerosol-cloud interactions Aerosols and particles Atmospheric Composition and Structure biomass burning Biosphere/atmosphere interactions Cloud physics and chemistry Cloud/radiation interaction Earth sciences Earth, ocean, space Exact sciences and technology ice nuclei |
title | Ice nuclei emissions from biomass burning |
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