Magnetic Ground State Stabilized by Three-Site Interactions: Fe/Rh(111)

We report the direct observation of a theoretically predicted magnetic ground state in a monolayer Fe on Rh(111), which is referred to as an up-up-down-down (↑↑↓↓) double-row-wise antiferromagnetic spin structure, using spin-polarized scanning tunneling microscopy. This exotic phase, which exists in...

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Veröffentlicht in:Physical review letters 2018-05, Vol.120 (20), p.207202-207202, Article 207202
Hauptverfasser: Krönlein, Andreas, Schmitt, Martin, Hoffmann, Markus, Kemmer, Jeannette, Seubert, Nicolai, Vogt, Matthias, Küspert, Julia, Böhme, Markus, Alonazi, Bandar, Kügel, Jens, Albrithen, Hamad A, Bode, Matthias, Bihlmayer, Gustav, Blügel, Stefan
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container_end_page 207202
container_issue 20
container_start_page 207202
container_title Physical review letters
container_volume 120
creator Krönlein, Andreas
Schmitt, Martin
Hoffmann, Markus
Kemmer, Jeannette
Seubert, Nicolai
Vogt, Matthias
Küspert, Julia
Böhme, Markus
Alonazi, Bandar
Kügel, Jens
Albrithen, Hamad A
Bode, Matthias
Bihlmayer, Gustav
Blügel, Stefan
description We report the direct observation of a theoretically predicted magnetic ground state in a monolayer Fe on Rh(111), which is referred to as an up-up-down-down (↑↑↓↓) double-row-wise antiferromagnetic spin structure, using spin-polarized scanning tunneling microscopy. This exotic phase, which exists in three orientational domains, is revealed by experiments with magnetic probe tips performed in external magnetic fields. It is shown that a hitherto unconsidered four-spin-three-site beyond-Heisenberg interaction distinctly contributes to the spin coupling of atoms with S≥1 spins. The observation of the ↑↑↓↓ order substantiates the presence of higher-order, in particular, three-site interactions, in thin magnetic films of itinerant magnets.
doi_str_mv 10.1103/PhysRevLett.120.207202
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source American Physical Society Journals; EZB-FREE-00999 freely available EZB journals
subjects Antiferromagnetism
Domains
Ground state
Iron
Magnetic films
Magnetic probes
Magnets
Spin structure
Thin films
Tips
title Magnetic Ground State Stabilized by Three-Site Interactions: Fe/Rh(111)
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