Occurrence and sources of polychlorinated dibenzo- p-dioxins, dibenzofurans and dioxin-like polychlorinated biphenyls in surficial sediments of Lakes Superior and Huron
Concentrations and congener profile patterns of 2378-substituted PCDD/Fs and DLPCBs in offshore, nearshore and tributary sediments of Lakes Superior and Huron are reported, and spatial trends and source contributions assessed. PCDD/F concentrations ranged from 5 to 18 000 pg/g dw (Lake Superior) and...
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creator | Shen, Li Gewurtz, Sarah B. Reiner, Eric J. MacPherson, Karen A. Kolic, Terry M. Khurana, Vin Helm, Paul A. Howell, E. Todd Burniston, Debbie A. Brindle, Ian D. Marvin, Chris H. |
description | Concentrations and congener profile patterns of 2378-substituted PCDD/Fs and DLPCBs in offshore, nearshore and tributary sediments of Lakes Superior and Huron are reported, and spatial trends and source contributions assessed. PCDD/F concentrations ranged from 5 to 18 000 pg/g dw (Lake Superior) and 3 to 6100 pg/g dw (Lake Huron); DLPCBs ranged from 9 to 11 000 pg/g dw (Lake Superior) and 9 to 27 000 pg/g dw (Lake Huron). Our analysis indicated atmospheric deposition is a primary source to depositional areas of both lakes; however, greater PCDD/F and DLPCB concentrations were observed at several nearshore and tributary sites, and were attributed to corresponding land use in the watershed. Statistical analysis and pattern comparison suggested that industrial inputs mainly associated with wood treatment plants, pulp and paper mills, mining operations, and chlorine-based chemical manufacturing also contributed to contamination by PCDD/Fs and DLPCBs in certain nearshore and offshore areas of Lakes Superior and Huron.
Lake-wide 2378-PCDD/F and DLPCB concentrations, spatial trends, and congener patterns are first reported in Lakes Superior and Huron sediments. |
doi_str_mv | 10.1016/j.envpol.2008.12.012 |
format | Article |
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Lake-wide 2378-PCDD/F and DLPCB concentrations, spatial trends, and congener patterns are first reported in Lakes Superior and Huron sediments.</description><identifier>ISSN: 0269-7491</identifier><identifier>EISSN: 1873-6424</identifier><identifier>DOI: 10.1016/j.envpol.2008.12.012</identifier><identifier>PMID: 19167794</identifier><identifier>CODEN: ENVPAF</identifier><language>eng</language><publisher>Kidlington: Elsevier Ltd</publisher><subject>Air Pollutants - analysis ; Applied sciences ; Benzofurans - analysis ; Benzofurans - chemistry ; Canada ; Congener pattern ; Dioxin-like polychlorinated biphenyls ; Earth sciences ; Earth, ocean, space ; Engineering and environment geology. Geothermics ; Environmental Monitoring - methods ; Exact sciences and technology ; Fresh Water ; Geologic Sediments - chemistry ; industrial wastes ; lakes ; Pesticides - analysis ; Pesticides - chemistry ; point source pollution ; Pollution ; Pollution sources. Measurement results ; Pollution, environment geology ; polychlorinated biphenyls ; Polychlorinated Biphenyls - analysis ; Polychlorinated Biphenyls - chemistry ; Polychlorinated dibenzo- p-dioxins ; polychlorinated dibenzodioxins ; Polychlorinated Dibenzodioxins - analogs & derivatives ; Polychlorinated Dibenzodioxins - analysis ; Polychlorinated Dibenzodioxins - chemistry ; Polychlorinated dibenzofurans ; Sediment ; sediment contamination ; Soil and sediments pollution ; Spatial trend ; spatial variation ; Water Pollutants, Chemical - analysis ; Water Pollutants, Chemical - chemistry ; water pollution</subject><ispartof>Environmental pollution (1987), 2009-04, Vol.157 (4), p.1210-1218</ispartof><rights>2008</rights><rights>2009 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a468t-cea66b19f134f0568fd298edd7297995525b62219f36fd642a1538eab4cb50c13</citedby><cites>FETCH-LOGICAL-a468t-cea66b19f134f0568fd298edd7297995525b62219f36fd642a1538eab4cb50c13</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.envpol.2008.12.012$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,778,782,3539,27911,27912,45982</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=21234509$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/19167794$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Shen, Li</creatorcontrib><creatorcontrib>Gewurtz, Sarah B.</creatorcontrib><creatorcontrib>Reiner, Eric J.</creatorcontrib><creatorcontrib>MacPherson, Karen A.</creatorcontrib><creatorcontrib>Kolic, Terry M.</creatorcontrib><creatorcontrib>Khurana, Vin</creatorcontrib><creatorcontrib>Helm, Paul A.</creatorcontrib><creatorcontrib>Howell, E. Todd</creatorcontrib><creatorcontrib>Burniston, Debbie A.</creatorcontrib><creatorcontrib>Brindle, Ian D.</creatorcontrib><creatorcontrib>Marvin, Chris H.</creatorcontrib><title>Occurrence and sources of polychlorinated dibenzo- p-dioxins, dibenzofurans and dioxin-like polychlorinated biphenyls in surficial sediments of Lakes Superior and Huron</title><title>Environmental pollution (1987)</title><addtitle>Environ Pollut</addtitle><description>Concentrations and congener profile patterns of 2378-substituted PCDD/Fs and DLPCBs in offshore, nearshore and tributary sediments of Lakes Superior and Huron are reported, and spatial trends and source contributions assessed. PCDD/F concentrations ranged from 5 to 18 000 pg/g dw (Lake Superior) and 3 to 6100 pg/g dw (Lake Huron); DLPCBs ranged from 9 to 11 000 pg/g dw (Lake Superior) and 9 to 27 000 pg/g dw (Lake Huron). Our analysis indicated atmospheric deposition is a primary source to depositional areas of both lakes; however, greater PCDD/F and DLPCB concentrations were observed at several nearshore and tributary sites, and were attributed to corresponding land use in the watershed. Statistical analysis and pattern comparison suggested that industrial inputs mainly associated with wood treatment plants, pulp and paper mills, mining operations, and chlorine-based chemical manufacturing also contributed to contamination by PCDD/Fs and DLPCBs in certain nearshore and offshore areas of Lakes Superior and Huron.
Lake-wide 2378-PCDD/F and DLPCB concentrations, spatial trends, and congener patterns are first reported in Lakes Superior and Huron sediments.</description><subject>Air Pollutants - analysis</subject><subject>Applied sciences</subject><subject>Benzofurans - analysis</subject><subject>Benzofurans - chemistry</subject><subject>Canada</subject><subject>Congener pattern</subject><subject>Dioxin-like polychlorinated biphenyls</subject><subject>Earth sciences</subject><subject>Earth, ocean, space</subject><subject>Engineering and environment geology. Geothermics</subject><subject>Environmental Monitoring - methods</subject><subject>Exact sciences and technology</subject><subject>Fresh Water</subject><subject>Geologic Sediments - chemistry</subject><subject>industrial wastes</subject><subject>lakes</subject><subject>Pesticides - analysis</subject><subject>Pesticides - chemistry</subject><subject>point source pollution</subject><subject>Pollution</subject><subject>Pollution sources. Measurement results</subject><subject>Pollution, environment geology</subject><subject>polychlorinated biphenyls</subject><subject>Polychlorinated Biphenyls - analysis</subject><subject>Polychlorinated Biphenyls - chemistry</subject><subject>Polychlorinated dibenzo- p-dioxins</subject><subject>polychlorinated dibenzodioxins</subject><subject>Polychlorinated Dibenzodioxins - analogs & derivatives</subject><subject>Polychlorinated Dibenzodioxins - analysis</subject><subject>Polychlorinated Dibenzodioxins - chemistry</subject><subject>Polychlorinated dibenzofurans</subject><subject>Sediment</subject><subject>sediment contamination</subject><subject>Soil and sediments pollution</subject><subject>Spatial trend</subject><subject>spatial variation</subject><subject>Water Pollutants, Chemical - analysis</subject><subject>Water Pollutants, Chemical - chemistry</subject><subject>water pollution</subject><issn>0269-7491</issn><issn>1873-6424</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2009</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNp9kcFu1DAQhi1ERZfCGyDIBU4k2I7jxBckVAFFWqmHtmfLscfU26wd7KRieSIeE-9mgUOlnizZ33wznh-hVwRXBBP-YVOBvx_DUFGMu4rQChP6BK1I19YlZ5Q9RStMuShbJsgpep7SBmPM6rp-hk6JILxtBVuh35dazzGC11Aob4oU5qghFcEW2b3Tt0OIzqsJTGFcD_5XKIuxNC78dD69_3tn56h8OgiWp3Jwd_DA0LvxFvxuSIXzRZqjddqpoUhg3Bb8dOi6Vne5_dU8QnQhHpQXcwz-BTqxakjw8nieoZsvn6_PL8r15ddv55_WpWK8m0oNivOeCEtqZnHDO2uo6MCYlopWiKahTc8pzUDNrcl7UqSpO1A9032DNanP0LvFO8bwY4Y0ya1LGoZBeQhzkhQzzFqxB9kC6hhSimDlGN1WxZ0kWO4Tkhu5JCT3CUlCZU4ol70--ud-C-Z_0TGSDLw9AippNdi8We3SP45mB2uwyNybhbMqSPU9ZubmimJS59aU5H9m4uNCQN7XvYMok3b7pI2LoCdpgnt81j8rgb5i</recordid><startdate>20090401</startdate><enddate>20090401</enddate><creator>Shen, Li</creator><creator>Gewurtz, Sarah B.</creator><creator>Reiner, Eric J.</creator><creator>MacPherson, Karen A.</creator><creator>Kolic, Terry M.</creator><creator>Khurana, Vin</creator><creator>Helm, Paul A.</creator><creator>Howell, E. 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Geothermics</topic><topic>Environmental Monitoring - methods</topic><topic>Exact sciences and technology</topic><topic>Fresh Water</topic><topic>Geologic Sediments - chemistry</topic><topic>industrial wastes</topic><topic>lakes</topic><topic>Pesticides - analysis</topic><topic>Pesticides - chemistry</topic><topic>point source pollution</topic><topic>Pollution</topic><topic>Pollution sources. Measurement results</topic><topic>Pollution, environment geology</topic><topic>polychlorinated biphenyls</topic><topic>Polychlorinated Biphenyls - analysis</topic><topic>Polychlorinated Biphenyls - chemistry</topic><topic>Polychlorinated dibenzo- p-dioxins</topic><topic>polychlorinated dibenzodioxins</topic><topic>Polychlorinated Dibenzodioxins - analogs & derivatives</topic><topic>Polychlorinated Dibenzodioxins - analysis</topic><topic>Polychlorinated Dibenzodioxins - chemistry</topic><topic>Polychlorinated dibenzofurans</topic><topic>Sediment</topic><topic>sediment contamination</topic><topic>Soil and sediments pollution</topic><topic>Spatial trend</topic><topic>spatial variation</topic><topic>Water Pollutants, Chemical - analysis</topic><topic>Water Pollutants, Chemical - chemistry</topic><topic>water pollution</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Shen, Li</creatorcontrib><creatorcontrib>Gewurtz, Sarah B.</creatorcontrib><creatorcontrib>Reiner, Eric J.</creatorcontrib><creatorcontrib>MacPherson, Karen A.</creatorcontrib><creatorcontrib>Kolic, Terry M.</creatorcontrib><creatorcontrib>Khurana, Vin</creatorcontrib><creatorcontrib>Helm, Paul A.</creatorcontrib><creatorcontrib>Howell, E. 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Todd</au><au>Burniston, Debbie A.</au><au>Brindle, Ian D.</au><au>Marvin, Chris H.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Occurrence and sources of polychlorinated dibenzo- p-dioxins, dibenzofurans and dioxin-like polychlorinated biphenyls in surficial sediments of Lakes Superior and Huron</atitle><jtitle>Environmental pollution (1987)</jtitle><addtitle>Environ Pollut</addtitle><date>2009-04-01</date><risdate>2009</risdate><volume>157</volume><issue>4</issue><spage>1210</spage><epage>1218</epage><pages>1210-1218</pages><issn>0269-7491</issn><eissn>1873-6424</eissn><coden>ENVPAF</coden><abstract>Concentrations and congener profile patterns of 2378-substituted PCDD/Fs and DLPCBs in offshore, nearshore and tributary sediments of Lakes Superior and Huron are reported, and spatial trends and source contributions assessed. PCDD/F concentrations ranged from 5 to 18 000 pg/g dw (Lake Superior) and 3 to 6100 pg/g dw (Lake Huron); DLPCBs ranged from 9 to 11 000 pg/g dw (Lake Superior) and 9 to 27 000 pg/g dw (Lake Huron). Our analysis indicated atmospheric deposition is a primary source to depositional areas of both lakes; however, greater PCDD/F and DLPCB concentrations were observed at several nearshore and tributary sites, and were attributed to corresponding land use in the watershed. Statistical analysis and pattern comparison suggested that industrial inputs mainly associated with wood treatment plants, pulp and paper mills, mining operations, and chlorine-based chemical manufacturing also contributed to contamination by PCDD/Fs and DLPCBs in certain nearshore and offshore areas of Lakes Superior and Huron.
Lake-wide 2378-PCDD/F and DLPCB concentrations, spatial trends, and congener patterns are first reported in Lakes Superior and Huron sediments.</abstract><cop>Kidlington</cop><pub>Elsevier Ltd</pub><pmid>19167794</pmid><doi>10.1016/j.envpol.2008.12.012</doi><tpages>9</tpages></addata></record> |
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subjects | Air Pollutants - analysis Applied sciences Benzofurans - analysis Benzofurans - chemistry Canada Congener pattern Dioxin-like polychlorinated biphenyls Earth sciences Earth, ocean, space Engineering and environment geology. Geothermics Environmental Monitoring - methods Exact sciences and technology Fresh Water Geologic Sediments - chemistry industrial wastes lakes Pesticides - analysis Pesticides - chemistry point source pollution Pollution Pollution sources. Measurement results Pollution, environment geology polychlorinated biphenyls Polychlorinated Biphenyls - analysis Polychlorinated Biphenyls - chemistry Polychlorinated dibenzo- p-dioxins polychlorinated dibenzodioxins Polychlorinated Dibenzodioxins - analogs & derivatives Polychlorinated Dibenzodioxins - analysis Polychlorinated Dibenzodioxins - chemistry Polychlorinated dibenzofurans Sediment sediment contamination Soil and sediments pollution Spatial trend spatial variation Water Pollutants, Chemical - analysis Water Pollutants, Chemical - chemistry water pollution |
title | Occurrence and sources of polychlorinated dibenzo- p-dioxins, dibenzofurans and dioxin-like polychlorinated biphenyls in surficial sediments of Lakes Superior and Huron |
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