Multicomponent metal-organic framework derivatives for optimizing the selective catalytic performance of styrene epoxidation reaction

Multicomponent metal-organic framework (MOF) derivatives have attracted strong interest in energy and environmental fields. However, most of the papers focus on single MOF derivatives; reports on multicomponent MOF derivatives and their catalytic studies are relatively few. Here, we report an easy-t...

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Veröffentlicht in:Nanoscale 2018-01, Vol.10 (18), p.8772-8778
Hauptverfasser: Hui, Junfeng, Chu, Huimin, Zhang, Wenlei, Shen, Yu, Chen, Wanzheng, Hu, Yu, Liu, Wan, Gao, Cong, Guo, Shaohua, Xiao, Gengwu, Li, Sheng, Fu, Yu, Fan, Daidi, Zhang, Weina, Huo, Fengwei
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container_end_page 8778
container_issue 18
container_start_page 8772
container_title Nanoscale
container_volume 10
creator Hui, Junfeng
Chu, Huimin
Zhang, Wenlei
Shen, Yu
Chen, Wanzheng
Hu, Yu
Liu, Wan
Gao, Cong
Guo, Shaohua
Xiao, Gengwu
Li, Sheng
Fu, Yu
Fan, Daidi
Zhang, Weina
Huo, Fengwei
description Multicomponent metal-organic framework (MOF) derivatives have attracted strong interest in energy and environmental fields. However, most of the papers focus on single MOF derivatives; reports on multicomponent MOF derivatives and their catalytic studies are relatively few. Here, we report an easy-to-operate strategy to obtain multicomponent MOF derivatives by treating multicomponent MOFs under a suitable gas atmosphere and at high temperature. We used ZIF-67 as a template to introduce Zn and successfully obtained multicomponent MOFs. After carbonization, the multicomponent MOF derivatives with Co and CoO nanoparticles exhibit higher conversion of styrene (≈99%), higher selectivity (≈70%) and better stability compared to MOFs and single component MOF derivatives.
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subjects Carbonization
Catalysis
Derivatives
Epoxidation
Metal-organic frameworks
title Multicomponent metal-organic framework derivatives for optimizing the selective catalytic performance of styrene epoxidation reaction
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