Mass balance and long-term fate of PCDD/Fs in a lagoon sediment and paddy soil, Niigata, Japan

Polychlorinated dibenzo- p-dioxins (PCDDs) and polychlorinated dibenzofurans (PCDFs) in a sediment core and in samples of surface sediment and paddy soil collected from the Toyano lagoon and Kameda basin in Niigata, Japan, were analyzed to elucidate the temporal trends of their concentrations in the...

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Veröffentlicht in:Environmental pollution (1987) 2008-12, Vol.156 (3), p.760-768
Hauptverfasser: Sakai, Mizuki, Seike, Nobuyasu, Kobayashi, Jun, Kajihara, Hideo, Takahashi, Yukio
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container_end_page 768
container_issue 3
container_start_page 760
container_title Environmental pollution (1987)
container_volume 156
creator Sakai, Mizuki
Seike, Nobuyasu
Kobayashi, Jun
Kajihara, Hideo
Takahashi, Yukio
description Polychlorinated dibenzo- p-dioxins (PCDDs) and polychlorinated dibenzofurans (PCDFs) in a sediment core and in samples of surface sediment and paddy soil collected from the Toyano lagoon and Kameda basin in Niigata, Japan, were analyzed to elucidate the temporal trends of their concentrations in the lagoon sediment and the relationship between the sediment and the paddy soil. The mass balance of these pollutants was also estimated to determine their long-term fate in surface waters. An analysis by chemical mass balance identified the agrochemicals pentachlorophenol and 2,4,6-trichlorophenyl 4-nitrophenyl ether as the major sources of PCDD/Fs. On the basis of the findings regarding the mass balance in the Kameda basin over the last 40 years, we estimate that more than half the input of PCDD/Fs to the Kameda basin has disappeared. We suggest that the PCDD/Fs that flowed out from the paddy fields have been transferred to the lower basin. The long-term mass balance of PCDD/Fs in sediments from paddy soil is elucidated.
doi_str_mv 10.1016/j.envpol.2008.06.004
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The mass balance of these pollutants was also estimated to determine their long-term fate in surface waters. An analysis by chemical mass balance identified the agrochemicals pentachlorophenol and 2,4,6-trichlorophenyl 4-nitrophenyl ether as the major sources of PCDD/Fs. On the basis of the findings regarding the mass balance in the Kameda basin over the last 40 years, we estimate that more than half the input of PCDD/Fs to the Kameda basin has disappeared. We suggest that the PCDD/Fs that flowed out from the paddy fields have been transferred to the lower basin. 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Interaction in the soil</topic><topic>chemical composition</topic><topic>CMB</topic><topic>Dibenzofurans, Polychlorinated</topic><topic>Earth sciences</topic><topic>Earth, ocean, space</topic><topic>Engineering and environment geology. 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The mass balance of these pollutants was also estimated to determine their long-term fate in surface waters. An analysis by chemical mass balance identified the agrochemicals pentachlorophenol and 2,4,6-trichlorophenyl 4-nitrophenyl ether as the major sources of PCDD/Fs. On the basis of the findings regarding the mass balance in the Kameda basin over the last 40 years, we estimate that more than half the input of PCDD/Fs to the Kameda basin has disappeared. We suggest that the PCDD/Fs that flowed out from the paddy fields have been transferred to the lower basin. The long-term mass balance of PCDD/Fs in sediments from paddy soil is elucidated.</abstract><cop>Kidlington</cop><pub>Elsevier Ltd</pub><pmid>18635299</pmid><doi>10.1016/j.envpol.2008.06.004</doi><tpages>9</tpages></addata></record>
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subjects 2,4,6-trichlorophenl 4-nitrophenyl ether
agrochemicals
Applied sciences
Benzofurans - analysis
Biological and physicochemical properties of pollutants. Interaction in the soil
chemical composition
CMB
Dibenzofurans, Polychlorinated
Earth sciences
Earth, ocean, space
Engineering and environment geology. Geothermics
environmental fate
Environmental Monitoring - methods
Exact sciences and technology
Food Contamination
Geologic Sediments - analysis
Herbicides - analysis
Humans
Japan
Mass balance
mass flow
Oryza
Paddy soil
paddy soils
PCDD/Fs
pentachlorophenol
Pollution
Pollution, environment geology
polychlorinated dibenzodioxins
Polychlorinated Dibenzodioxins - analogs & derivatives
Polychlorinated Dibenzodioxins - analysis
polychlorinated dibenzofurans
Sediment core
sediment transport
sediments
Soil - analysis
Soil and sediments pollution
Soil Pollutants - analysis
soil pollution
surface water
temporal variation
Time Factors
Water Pollutants, Chemical - analysis
water pollution
title Mass balance and long-term fate of PCDD/Fs in a lagoon sediment and paddy soil, Niigata, Japan
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