Tuning the Carbon Nanotube Selectivity: Optimizing Reduction Potentials and Distortion Angles in Perylenediimides
Different water-soluble perylenediimides (PDIs) have been used to individualize and stabilize single-walled carbon nanotubes (SWCNTs) in aqueous media. A key feature of the PDIs is that they can be substituted at the bay positions via the addition of two and/or four bromines. This enables control ov...
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| Veröffentlicht in: | Journal of the American Chemical Society 2018-04, Vol.140 (16), p.5427-5433 |
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| container_title | Journal of the American Chemical Society |
| container_volume | 140 |
| creator | Münich, Peter W Schierl, Christoph Dirian, Konstantin Volland, Michel Bauroth, Stefan Wibmer, Leonie Syrgiannis, Zois Clark, Timothy Prato, Maurizio Guldi, Dirk M |
| description | Different water-soluble perylenediimides (PDIs) have been used to individualize and stabilize single-walled carbon nanotubes (SWCNTs) in aqueous media. A key feature of the PDIs is that they can be substituted at the bay positions via the addition of two and/or four bromines. This enables control over structural and electronic PDI characteristics, which prompted us to conduct comparative assays with focus on SWCNTs’ chirality and charge transfer. Electrochemical, microscopic, and spectroscopic experiments were used to investigate the SWCNT chiral selectivity of PDIs, on the one hand, and charge-transfer reactions between SWCNTs and PDIs, on the other hand. |
| doi_str_mv | 10.1021/jacs.8b00452 |
| format | Article |
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| issn | 0002-7863 1520-5126 |
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| source | ACS Publications |
| title | Tuning the Carbon Nanotube Selectivity: Optimizing Reduction Potentials and Distortion Angles in Perylenediimides |
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