Phase transition triggered aggregation-induced emission in a photoluminescent uranyl-organic framework
When exposed to water, the two-dimensional uranyl-organic layered compound [(CH ) NH ][(UO )(BCPBA)]·2DMF·H O (H BCPBA = 3,5-bis (4'-carboxylphenoxy) benzoic acid) gradually undergoes a complete single-crystal-to-single-crystal phase transition to [(CH ) NH ][(UO )(BCPBA)]·3.4H O, resulting in...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2018, Vol.54 (6), p.627-630 |
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| container_title | Chemical communications (Cambridge, England) |
| container_volume | 54 |
| creator | Wang, Xia Wang, Yanlong Dai, Xing Silver, Mark A Liu, Wei Li, Yuxiang Bai, Zhuanling Gui, Daxiang Chen, Lanhua Diwu, Juan Zhou, Ruhong Chai, Zhifang Wang, Shuao |
| description | When exposed to water, the two-dimensional uranyl-organic layered compound [(CH
)
NH
][(UO
)(BCPBA)]·2DMF·H
O (H
BCPBA = 3,5-bis (4'-carboxylphenoxy) benzoic acid) gradually undergoes a complete single-crystal-to-single-crystal phase transition to [(CH
)
NH
][(UO
)(BCPBA)]·3.4H
O, resulting in an enhanced ligand-ligand interaction between the adjacent layers. This process gives rise to initial quenching of the uranyl photoluminescence followed by subsequent recovery of the photoluminescence with a much elevated intensity, as a unique case of aggregation-induced emission in an extended solid system, further confirmed by DFT analysis on bonding. |
| doi_str_mv | 10.1039/c7cc09594e |
| format | Article |
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)
NH
][(UO
)(BCPBA)]·2DMF·H
O (H
BCPBA = 3,5-bis (4'-carboxylphenoxy) benzoic acid) gradually undergoes a complete single-crystal-to-single-crystal phase transition to [(CH
)
NH
][(UO
)(BCPBA)]·3.4H
O, resulting in an enhanced ligand-ligand interaction between the adjacent layers. This process gives rise to initial quenching of the uranyl photoluminescence followed by subsequent recovery of the photoluminescence with a much elevated intensity, as a unique case of aggregation-induced emission in an extended solid system, further confirmed by DFT analysis on bonding.</description><identifier>ISSN: 1359-7345</identifier><identifier>EISSN: 1364-548X</identifier><identifier>DOI: 10.1039/c7cc09594e</identifier><identifier>PMID: 29299560</identifier><language>eng</language><publisher>England: Royal Society of Chemistry</publisher><subject>Agglomeration ; Benzoic acid ; Emission analysis ; Ligands ; Phase transitions ; Photoluminescence ; Single crystals ; Uranium dioxide</subject><ispartof>Chemical communications (Cambridge, England), 2018, Vol.54 (6), p.627-630</ispartof><rights>Copyright Royal Society of Chemistry 2018</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c381t-d0bc9d3dea9c6a8f1845cad8c31020da3277666a573989582328af1afb8d9df83</citedby><cites>FETCH-LOGICAL-c381t-d0bc9d3dea9c6a8f1845cad8c31020da3277666a573989582328af1afb8d9df83</cites><orcidid>0000-0001-8624-5591 ; 0000-0002-1526-1102</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,4010,27900,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/29299560$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Wang, Xia</creatorcontrib><creatorcontrib>Wang, Yanlong</creatorcontrib><creatorcontrib>Dai, Xing</creatorcontrib><creatorcontrib>Silver, Mark A</creatorcontrib><creatorcontrib>Liu, Wei</creatorcontrib><creatorcontrib>Li, Yuxiang</creatorcontrib><creatorcontrib>Bai, Zhuanling</creatorcontrib><creatorcontrib>Gui, Daxiang</creatorcontrib><creatorcontrib>Chen, Lanhua</creatorcontrib><creatorcontrib>Diwu, Juan</creatorcontrib><creatorcontrib>Zhou, Ruhong</creatorcontrib><creatorcontrib>Chai, Zhifang</creatorcontrib><creatorcontrib>Wang, Shuao</creatorcontrib><title>Phase transition triggered aggregation-induced emission in a photoluminescent uranyl-organic framework</title><title>Chemical communications (Cambridge, England)</title><addtitle>Chem Commun (Camb)</addtitle><description>When exposed to water, the two-dimensional uranyl-organic layered compound [(CH
)
NH
][(UO
)(BCPBA)]·2DMF·H
O (H
BCPBA = 3,5-bis (4'-carboxylphenoxy) benzoic acid) gradually undergoes a complete single-crystal-to-single-crystal phase transition to [(CH
)
NH
][(UO
)(BCPBA)]·3.4H
O, resulting in an enhanced ligand-ligand interaction between the adjacent layers. This process gives rise to initial quenching of the uranyl photoluminescence followed by subsequent recovery of the photoluminescence with a much elevated intensity, as a unique case of aggregation-induced emission in an extended solid system, further confirmed by DFT analysis on bonding.</description><subject>Agglomeration</subject><subject>Benzoic acid</subject><subject>Emission analysis</subject><subject>Ligands</subject><subject>Phase transitions</subject><subject>Photoluminescence</subject><subject>Single crystals</subject><subject>Uranium dioxide</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNpdkE9LxDAQxYMo7rp68QNIwYsI1aRp2uQoZf0DC3pQ8FZmk7RG22RNWsRvb6qrB-cyw-PHm8dD6JjgC4KpuJSllFgwkesdNCe0yFOW8-fd6WYiLWnOZugghFcchzC-j2aZyIRgBZ6j5uEFgk4GDzaYwTgbT9O22muVQNt63cKkpsaqUUZN9yaECTM2gWTz4gbXjb2xOkhth2SMPp9d6nwL1sik8dDrD-ffDtFeA13QR9u9QE_Xy8fqNl3d39xVV6tUUk6GVOG1FIoqDUIWwBvCcyZBcUkJzrACmpVlURTASiq4YDyjGYeGQLPmSqiG0wU6-_HdePc-6jDUMa_UXQdWuzHURPC8ZHkWDRbo9B_66kZvY7o6wwTz-CufqPMfSnoXgtdNvfGmB_9ZE1xP7ddVWVXf7S8jfLK1HNe9Vn_ob930C9HYgWg</recordid><startdate>2018</startdate><enddate>2018</enddate><creator>Wang, Xia</creator><creator>Wang, Yanlong</creator><creator>Dai, Xing</creator><creator>Silver, Mark A</creator><creator>Liu, Wei</creator><creator>Li, Yuxiang</creator><creator>Bai, Zhuanling</creator><creator>Gui, Daxiang</creator><creator>Chen, Lanhua</creator><creator>Diwu, Juan</creator><creator>Zhou, Ruhong</creator><creator>Chai, Zhifang</creator><creator>Wang, Shuao</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0001-8624-5591</orcidid><orcidid>https://orcid.org/0000-0002-1526-1102</orcidid></search><sort><creationdate>2018</creationdate><title>Phase transition triggered aggregation-induced emission in a photoluminescent uranyl-organic framework</title><author>Wang, Xia ; Wang, Yanlong ; Dai, Xing ; Silver, Mark A ; Liu, Wei ; Li, Yuxiang ; Bai, Zhuanling ; Gui, Daxiang ; Chen, Lanhua ; Diwu, Juan ; Zhou, Ruhong ; Chai, Zhifang ; Wang, Shuao</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c381t-d0bc9d3dea9c6a8f1845cad8c31020da3277666a573989582328af1afb8d9df83</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Agglomeration</topic><topic>Benzoic acid</topic><topic>Emission analysis</topic><topic>Ligands</topic><topic>Phase transitions</topic><topic>Photoluminescence</topic><topic>Single crystals</topic><topic>Uranium dioxide</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Xia</creatorcontrib><creatorcontrib>Wang, Yanlong</creatorcontrib><creatorcontrib>Dai, Xing</creatorcontrib><creatorcontrib>Silver, Mark A</creatorcontrib><creatorcontrib>Liu, Wei</creatorcontrib><creatorcontrib>Li, Yuxiang</creatorcontrib><creatorcontrib>Bai, Zhuanling</creatorcontrib><creatorcontrib>Gui, Daxiang</creatorcontrib><creatorcontrib>Chen, Lanhua</creatorcontrib><creatorcontrib>Diwu, Juan</creatorcontrib><creatorcontrib>Zhou, Ruhong</creatorcontrib><creatorcontrib>Chai, Zhifang</creatorcontrib><creatorcontrib>Wang, Shuao</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wang, Xia</au><au>Wang, Yanlong</au><au>Dai, Xing</au><au>Silver, Mark A</au><au>Liu, Wei</au><au>Li, Yuxiang</au><au>Bai, Zhuanling</au><au>Gui, Daxiang</au><au>Chen, Lanhua</au><au>Diwu, Juan</au><au>Zhou, Ruhong</au><au>Chai, Zhifang</au><au>Wang, Shuao</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Phase transition triggered aggregation-induced emission in a photoluminescent uranyl-organic framework</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2018</date><risdate>2018</risdate><volume>54</volume><issue>6</issue><spage>627</spage><epage>630</epage><pages>627-630</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>When exposed to water, the two-dimensional uranyl-organic layered compound [(CH
)
NH
][(UO
)(BCPBA)]·2DMF·H
O (H
BCPBA = 3,5-bis (4'-carboxylphenoxy) benzoic acid) gradually undergoes a complete single-crystal-to-single-crystal phase transition to [(CH
)
NH
][(UO
)(BCPBA)]·3.4H
O, resulting in an enhanced ligand-ligand interaction between the adjacent layers. This process gives rise to initial quenching of the uranyl photoluminescence followed by subsequent recovery of the photoluminescence with a much elevated intensity, as a unique case of aggregation-induced emission in an extended solid system, further confirmed by DFT analysis on bonding.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>29299560</pmid><doi>10.1039/c7cc09594e</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0001-8624-5591</orcidid><orcidid>https://orcid.org/0000-0002-1526-1102</orcidid></addata></record> |
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| ispartof | Chemical communications (Cambridge, England), 2018, Vol.54 (6), p.627-630 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_proquest_miscellaneous_1984754257 |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Agglomeration Benzoic acid Emission analysis Ligands Phase transitions Photoluminescence Single crystals Uranium dioxide |
| title | Phase transition triggered aggregation-induced emission in a photoluminescent uranyl-organic framework |
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