Tracking long-distance atmospheric deposition of trace metal emissions from smelters in the upper Columbia River valley using Pb isotope analysis of lake sediments
Heavy metal discharge from mining and smelting operations into aquatic ecosystems can cause long-term biological and ecological impacts. The upper Columbia River is highly contaminated with heavy metal wastes from nearby smelting operations in Trail, British Columbia, Canada, and to a lesser extent,...
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| Veröffentlicht in: | Environmental science and pollution research international 2018-02, Vol.25 (6), p.5501-5513 |
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| creator | Child, Andrew Wright Moore, Barry C. Vervoort, Jeffrey D. Beutel, Marc W. |
| description | Heavy metal discharge from mining and smelting operations into aquatic ecosystems can cause long-term biological and ecological impacts. The upper Columbia River is highly contaminated with heavy metal wastes from nearby smelting operations in Trail, British Columbia, Canada, and to a lesser extent, Northport (Le Roi smelter), Washington, USA. Airborne emissions from the Trail operations were historically and are currently transported by prevailing winds down the Columbia River canyon, where particulate metals can be deposited into lakes and watersheds. In lakes, sediment cores contain records of past environmental conditions, providing a timeline of fundamental chemical and biological relationships within aquatic ecosystems, including records of airborne metal depositions. We analyzed trace metal concentrations (Ni, Cd, Zn, As, Cu, Sb, Pb, Hg) and Pb isotope compositions of sediment cores from six remote eastern Washington lakes to assess potential sources of atmospheric heavy metal deposition. Sediment cores displayed evidence to support trace metal loading as a direct consequence of smelting operations in Trail. Smelter contamination was detected 144 km downwind of the Trail Smelter. Cd, Sb, Pb (
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| doi_str_mv | 10.1007/s11356-017-0914-1 |
| format | Article |
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p
< 0.001), and to a lesser extent As and Hg (
p
< 0.05) concentrations were correlated with Pb isotope compositions, suggesting that the Trail operations were likely the main source for these trace metals.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-017-0914-1</identifier><identifier>PMID: 29218574</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Antimony ; Aquatic ecosystems ; Aquatic Pollution ; atmospheric deposition ; Atmospheric pollution deposition ; Atmospheric Protection/Air Quality Control/Air Pollution ; British Columbia ; Cadmium ; Canyons ; Columbia River ; Contamination ; Copper ; Cores ; Deposition ; Earth and Environmental Science ; Ecological effects ; Ecotoxicology ; Emissions ; Environment ; Environmental Chemistry ; Environmental conditions ; Environmental Health ; Environmental science ; Heavy metals ; Isotopes ; Lake sediments ; Lakes ; Lead ; Mercury ; Metal concentrations ; Metal industry wastes ; Metallurgy ; Nickel ; Pollutant deposition ; Research Article ; river valleys ; Rivers ; Sediments ; Smelters ; Smelting ; trace elements ; Trace metals ; Waste Water Technology ; Water Management ; Water pollution ; Water Pollution Control ; Watersheds ; Zinc</subject><ispartof>Environmental science and pollution research international, 2018-02, Vol.25 (6), p.5501-5513</ispartof><rights>Springer-Verlag GmbH Germany, part of Springer Nature 2017</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, (2017). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c444t-c3b6cd9efefe835bfd202aaf7c42ce4e0b0a6167d4fc9daacd28d6e73003b74e3</citedby><cites>FETCH-LOGICAL-c444t-c3b6cd9efefe835bfd202aaf7c42ce4e0b0a6167d4fc9daacd28d6e73003b74e3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-017-0914-1$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-017-0914-1$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,777,781,27905,27906,41469,42538,51300</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/29218574$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Child, Andrew Wright</creatorcontrib><creatorcontrib>Moore, Barry C.</creatorcontrib><creatorcontrib>Vervoort, Jeffrey D.</creatorcontrib><creatorcontrib>Beutel, Marc W.</creatorcontrib><title>Tracking long-distance atmospheric deposition of trace metal emissions from smelters in the upper Columbia River valley using Pb isotope analysis of lake sediments</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Heavy metal discharge from mining and smelting operations into aquatic ecosystems can cause long-term biological and ecological impacts. The upper Columbia River is highly contaminated with heavy metal wastes from nearby smelting operations in Trail, British Columbia, Canada, and to a lesser extent, Northport (Le Roi smelter), Washington, USA. Airborne emissions from the Trail operations were historically and are currently transported by prevailing winds down the Columbia River canyon, where particulate metals can be deposited into lakes and watersheds. In lakes, sediment cores contain records of past environmental conditions, providing a timeline of fundamental chemical and biological relationships within aquatic ecosystems, including records of airborne metal depositions. We analyzed trace metal concentrations (Ni, Cd, Zn, As, Cu, Sb, Pb, Hg) and Pb isotope compositions of sediment cores from six remote eastern Washington lakes to assess potential sources of atmospheric heavy metal deposition. Sediment cores displayed evidence to support trace metal loading as a direct consequence of smelting operations in Trail. Smelter contamination was detected 144 km downwind of the Trail Smelter. Cd, Sb, Pb (
p
< 0.001), and to a lesser extent As and Hg (
p
< 0.05) concentrations were correlated with Pb isotope compositions, suggesting that the Trail operations were likely the main source for these trace metals.</description><subject>Antimony</subject><subject>Aquatic ecosystems</subject><subject>Aquatic Pollution</subject><subject>atmospheric deposition</subject><subject>Atmospheric pollution deposition</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>British Columbia</subject><subject>Cadmium</subject><subject>Canyons</subject><subject>Columbia River</subject><subject>Contamination</subject><subject>Copper</subject><subject>Cores</subject><subject>Deposition</subject><subject>Earth and Environmental Science</subject><subject>Ecological effects</subject><subject>Ecotoxicology</subject><subject>Emissions</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental conditions</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Heavy metals</subject><subject>Isotopes</subject><subject>Lake sediments</subject><subject>Lakes</subject><subject>Lead</subject><subject>Mercury</subject><subject>Metal concentrations</subject><subject>Metal industry wastes</subject><subject>Metallurgy</subject><subject>Nickel</subject><subject>Pollutant deposition</subject><subject>Research Article</subject><subject>river valleys</subject><subject>Rivers</subject><subject>Sediments</subject><subject>Smelters</subject><subject>Smelting</subject><subject>trace elements</subject><subject>Trace metals</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water pollution</subject><subject>Water Pollution Control</subject><subject>Watersheds</subject><subject>Zinc</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNqFkcGKFDEQhoMo7uzoA3iRgBcvrUk63ek-yrC6woIi6zmkk-rZ7KY7bSq9MM_ji5pxVhFBJIdKKt9fP8VPyAvO3nDG1FvkvG7ainFVsZ7Lij8iG96Wi5J9_5hsWC9Ls5byjJwj3jImWC_UU3ImesG7RskN-X6djL3z856GOO8r5zGb2QI1eYq43EDyljpYIvrs40zjSHMRAJ0gm0Bh8oilj3RMcaI4QciQkPqZ5hug67JAorsY1mnwhn7x9-V5b0KAA13xaPp5oB5jjktxnE04oMejRzB3QBGcn2DO-Iw8GU1AeP5Qt-Tr-4vr3WV19enDx927q8pKKXNl66G1roexnK5uhtEJJowZlZXCggQ2MNPyVjk52t4ZY53oXAuqZqwelIR6S16f5i4pflsBsy7rWQjBzBBX1ILJphOqVvK_KO9VwwSXHSvoq7_Q27imsuxPqm4VV6VsCT9RNkXEBKNekp9MOmjO9DFsfQpbl7D1MWzNi-blw-R1mMD9VvxKtwDiBGD5mveQ_rD-59QfsR-4xA</recordid><startdate>20180201</startdate><enddate>20180201</enddate><creator>Child, 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Wright</au><au>Moore, Barry C.</au><au>Vervoort, Jeffrey D.</au><au>Beutel, Marc W.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Tracking long-distance atmospheric deposition of trace metal emissions from smelters in the upper Columbia River valley using Pb isotope analysis of lake sediments</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2018-02-01</date><risdate>2018</risdate><volume>25</volume><issue>6</issue><spage>5501</spage><epage>5513</epage><pages>5501-5513</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Heavy metal discharge from mining and smelting operations into aquatic ecosystems can cause long-term biological and ecological impacts. The upper Columbia River is highly contaminated with heavy metal wastes from nearby smelting operations in Trail, British Columbia, Canada, and to a lesser extent, Northport (Le Roi smelter), Washington, USA. Airborne emissions from the Trail operations were historically and are currently transported by prevailing winds down the Columbia River canyon, where particulate metals can be deposited into lakes and watersheds. In lakes, sediment cores contain records of past environmental conditions, providing a timeline of fundamental chemical and biological relationships within aquatic ecosystems, including records of airborne metal depositions. We analyzed trace metal concentrations (Ni, Cd, Zn, As, Cu, Sb, Pb, Hg) and Pb isotope compositions of sediment cores from six remote eastern Washington lakes to assess potential sources of atmospheric heavy metal deposition. Sediment cores displayed evidence to support trace metal loading as a direct consequence of smelting operations in Trail. Smelter contamination was detected 144 km downwind of the Trail Smelter. Cd, Sb, Pb (
p
< 0.001), and to a lesser extent As and Hg (
p
< 0.05) concentrations were correlated with Pb isotope compositions, suggesting that the Trail operations were likely the main source for these trace metals.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>29218574</pmid><doi>10.1007/s11356-017-0914-1</doi><tpages>13</tpages></addata></record> |
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| ispartof | Environmental science and pollution research international, 2018-02, Vol.25 (6), p.5501-5513 |
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| source | Springer Nature - Complete Springer Journals |
| subjects | Antimony Aquatic ecosystems Aquatic Pollution atmospheric deposition Atmospheric pollution deposition Atmospheric Protection/Air Quality Control/Air Pollution British Columbia Cadmium Canyons Columbia River Contamination Copper Cores Deposition Earth and Environmental Science Ecological effects Ecotoxicology Emissions Environment Environmental Chemistry Environmental conditions Environmental Health Environmental science Heavy metals Isotopes Lake sediments Lakes Lead Mercury Metal concentrations Metal industry wastes Metallurgy Nickel Pollutant deposition Research Article river valleys Rivers Sediments Smelters Smelting trace elements Trace metals Waste Water Technology Water Management Water pollution Water Pollution Control Watersheds Zinc |
| title | Tracking long-distance atmospheric deposition of trace metal emissions from smelters in the upper Columbia River valley using Pb isotope analysis of lake sediments |
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