Chemical behavior of residential lead in urban yards in the United States
Long after federal regulations banned the use of lead-based paints and leaded gasoline, residential lead remains a persistent challenge. Soil lead is a significant contributor to this hazard and an improved understanding of physicochemical properties is likely to be useful for in situ abatement tech...
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Veröffentlicht in: | Environmental pollution (1987) 2007-07, Vol.148 (1), p.291-300 |
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creator | Elless, M.P. Bray, C.A. Blaylock, M.J. |
description | Long after federal regulations banned the use of lead-based paints and leaded gasoline, residential lead remains a persistent challenge. Soil lead is a significant contributor to this hazard and an improved understanding of physicochemical properties is likely to be useful for in situ abatement techniques such as phytoremediation and chemical stabilization. A laboratory characterization of high-lead soils collected from across the United States shows that the lead contaminants were concentrating in the silt and clay fractions, in the form of discrete particles of lead, as observed by scanning electron microscopy coupled with energy dispersive X-ray analysis. Soil lead varied widely in its solubility behavior as assessed by sequential and chelate extractions. Because site-specific factors (e.g., soil pH, texture, etc.) are believed to govern the solubility of the lead, understanding the variability in these characteristics at each site is necessary to optimize in situ remediation or abatement of these soils.
Site-specific solubility behavior of lead in soils has important implications for the selection of remediation approaches. |
doi_str_mv | 10.1016/j.envpol.2006.10.024 |
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Site-specific solubility behavior of lead in soils has important implications for the selection of remediation approaches.</description><subject>Applied sciences</subject><subject>Biological and physicochemical properties of pollutants. Interaction in the soil</subject><subject>Chelate</subject><subject>chelates</subject><subject>Chelating Agents - pharmacology</subject><subject>Cities</subject><subject>clay fraction</subject><subject>Earth sciences</subject><subject>Earth, ocean, space</subject><subject>Engineering and environment geology. Geothermics</subject><subject>Environmental Monitoring - methods</subject><subject>Environmental Restoration and Remediation - methods</subject><subject>Exact sciences and technology</subject><subject>extraction</subject><subject>Housing</subject><subject>Hydrogen-Ion Concentration</subject><subject>lead</subject><subject>Lead - chemistry</subject><subject>Lead-based paint</subject><subject>Microscopy, Electron, Scanning</subject><subject>Particle Size</subject><subject>particles</subject><subject>polluted soils</subject><subject>Pollution</subject><subject>Pollution, environment geology</subject><subject>Residential</subject><subject>residential areas</subject><subject>scanning electron microscopy</subject><subject>silt fraction</subject><subject>Soil and sediments pollution</subject><subject>soil pH</subject><subject>Soil Pollutants - chemistry</subject><subject>soil pollution</subject><subject>soil texture</subject><subject>Solubility</subject><subject>United States</subject><issn>0269-7491</issn><issn>1873-6424</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2007</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkU1rGzEQhkVoSRy3_6C0e0lv644-diVdCsWkaSDQQ-qz0EqjWma960prQ_59ZdaQW3sa9PLoZXiGkA8UVhRo-2W3wuF0GPsVA2hLtAImrsiCKsnrVjDxhiyAtbqWQtMbcpvzDgAE5_ya3FBJlRIUFuRxvcV9dLavOtzaUxxTNYYqYY4ehymWvEfrqzhUx9TZoXqxyefzc9pitRnihL56nuyE-R15G2yf8f1lLsnm-_2v9Y_66efD4_rbU-2EbKfac9pRarmgOrAOQ-tQdKiV1Y3W4ENoPMhGMKmFLCFC0yimhQ6Oei6awJfk89x7SOOfI-bJ7GN22Pd2wPGYDdWNlMXF_0EhtVISCihm0KUx54TBHFLc2_RiKJiza7Mzs2tzdn1O5_6Pl_5jt0f_-ukitwB3F8DmYjgkO7iYXzklGybLQZbk08wFOxr7OxVm88yAcgCpODBaiK8zgUXsKWIy2UUcHPqY0E3Gj_Hfu_4FQqumng</recordid><startdate>20070701</startdate><enddate>20070701</enddate><creator>Elless, M.P.</creator><creator>Bray, C.A.</creator><creator>Blaylock, M.J.</creator><general>Elsevier Ltd</general><general>Elsevier</general><scope>FBQ</scope><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7ST</scope><scope>C1K</scope><scope>SOI</scope><scope>7TV</scope><scope>7U7</scope></search><sort><creationdate>20070701</creationdate><title>Chemical behavior of residential lead in urban yards in the United States</title><author>Elless, M.P. ; Bray, C.A. ; Blaylock, M.J.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c476t-d31b11a3419f2bef6ce4be98a95990dff5d0754279478a9e05582949fc1d345f3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2007</creationdate><topic>Applied sciences</topic><topic>Biological and physicochemical properties of pollutants. Interaction in the soil</topic><topic>Chelate</topic><topic>chelates</topic><topic>Chelating Agents - pharmacology</topic><topic>Cities</topic><topic>clay fraction</topic><topic>Earth sciences</topic><topic>Earth, ocean, space</topic><topic>Engineering and environment geology. Geothermics</topic><topic>Environmental Monitoring - methods</topic><topic>Environmental Restoration and Remediation - methods</topic><topic>Exact sciences and technology</topic><topic>extraction</topic><topic>Housing</topic><topic>Hydrogen-Ion Concentration</topic><topic>lead</topic><topic>Lead - chemistry</topic><topic>Lead-based paint</topic><topic>Microscopy, Electron, Scanning</topic><topic>Particle Size</topic><topic>particles</topic><topic>polluted soils</topic><topic>Pollution</topic><topic>Pollution, environment geology</topic><topic>Residential</topic><topic>residential areas</topic><topic>scanning electron microscopy</topic><topic>silt fraction</topic><topic>Soil and sediments pollution</topic><topic>soil pH</topic><topic>Soil Pollutants - chemistry</topic><topic>soil pollution</topic><topic>soil texture</topic><topic>Solubility</topic><topic>United States</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Elless, M.P.</creatorcontrib><creatorcontrib>Bray, C.A.</creatorcontrib><creatorcontrib>Blaylock, M.J.</creatorcontrib><collection>AGRIS</collection><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Environment Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Environment Abstracts</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><jtitle>Environmental pollution (1987)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Elless, M.P.</au><au>Bray, C.A.</au><au>Blaylock, M.J.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Chemical behavior of residential lead in urban yards in the United States</atitle><jtitle>Environmental pollution (1987)</jtitle><addtitle>Environ Pollut</addtitle><date>2007-07-01</date><risdate>2007</risdate><volume>148</volume><issue>1</issue><spage>291</spage><epage>300</epage><pages>291-300</pages><issn>0269-7491</issn><eissn>1873-6424</eissn><coden>ENVPAF</coden><abstract>Long after federal regulations banned the use of lead-based paints and leaded gasoline, residential lead remains a persistent challenge. Soil lead is a significant contributor to this hazard and an improved understanding of physicochemical properties is likely to be useful for in situ abatement techniques such as phytoremediation and chemical stabilization. A laboratory characterization of high-lead soils collected from across the United States shows that the lead contaminants were concentrating in the silt and clay fractions, in the form of discrete particles of lead, as observed by scanning electron microscopy coupled with energy dispersive X-ray analysis. Soil lead varied widely in its solubility behavior as assessed by sequential and chelate extractions. Because site-specific factors (e.g., soil pH, texture, etc.) are believed to govern the solubility of the lead, understanding the variability in these characteristics at each site is necessary to optimize in situ remediation or abatement of these soils.
Site-specific solubility behavior of lead in soils has important implications for the selection of remediation approaches.</abstract><cop>Oxford</cop><pub>Elsevier Ltd</pub><pmid>17188410</pmid><doi>10.1016/j.envpol.2006.10.024</doi><tpages>10</tpages></addata></record> |
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subjects | Applied sciences Biological and physicochemical properties of pollutants. Interaction in the soil Chelate chelates Chelating Agents - pharmacology Cities clay fraction Earth sciences Earth, ocean, space Engineering and environment geology. Geothermics Environmental Monitoring - methods Environmental Restoration and Remediation - methods Exact sciences and technology extraction Housing Hydrogen-Ion Concentration lead Lead - chemistry Lead-based paint Microscopy, Electron, Scanning Particle Size particles polluted soils Pollution Pollution, environment geology Residential residential areas scanning electron microscopy silt fraction Soil and sediments pollution soil pH Soil Pollutants - chemistry soil pollution soil texture Solubility United States |
title | Chemical behavior of residential lead in urban yards in the United States |
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