Removal of endrin and dieldrin isomeric pesticides through stereoselective adsorption behavior on the graphene oxide-magnetic nanoparticles
A novel stereoselective removal behavior of isomeric endrin and dieldrin pesticides from sample solution is demonstrated using nanocomposite of graphene oxide (GO) and iron oxide (Fe 3 O 4 ) magnetic nanoparticles (MNPs). The removal efficiency of endrin and dieldrin was found higher when GO-MNPs wa...
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| Veröffentlicht in: | Environmental science and pollution research international 2017-11, Vol.24 (32), p.24980-24988 |
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| creator | Shrivas, Kamlesh Ghosale, Archana Nirmalkar, Nidhi Srivastava, Arti Singh, Sunil Kumar Shinde, Sandip S. |
| description | A novel stereoselective removal behavior of isomeric endrin and dieldrin pesticides from sample solution is demonstrated using nanocomposite of graphene oxide (GO) and iron oxide (Fe
3
O
4
) magnetic nanoparticles (MNPs). The removal efficiency of endrin and dieldrin was found higher when GO-MNPs was used as a separating probe than the individual use of GO and MNPs. The removal efficiency of both the pesticides was found to be more favorable when the dosage amount of GO-MNPs was 30 mg for 30-min contact time with pH 4.0 at room temperature. The good correlation of determination (
R
2
) with 0.975 and 0.973 values obtained for endrin and dieldrin, respectively demonstrated a well fitting of Langmuir adsorption isotherm model. The higher removal percentage (86.0%) and higher slope value of Langmuir adsorption isotherm were estimated for endrin compared to dieldrin (74.0%). The reason for higher adsorption percentage of endrin is due to the endo-position of oxygen atom in molecule favors more interaction of molecules with GO-MNPs compared to the exo-position of oxygen present in dieldrin. In addition, the higher value of
R
2
for endrin and dieldrin demonstrated better suitability of pseudo-first-order and pseudo-second-order kinetic models, respectively. The advantages of the present method are use of simple UV-vis spectrophotometry for monitoring and low-cost use of GO-MNPs nanomaterial for the removal of pesticides from sample solution. |
| doi_str_mv | 10.1007/s11356-017-0159-z |
| format | Article |
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3
O
4
) magnetic nanoparticles (MNPs). The removal efficiency of endrin and dieldrin was found higher when GO-MNPs was used as a separating probe than the individual use of GO and MNPs. The removal efficiency of both the pesticides was found to be more favorable when the dosage amount of GO-MNPs was 30 mg for 30-min contact time with pH 4.0 at room temperature. The good correlation of determination (
R
2
) with 0.975 and 0.973 values obtained for endrin and dieldrin, respectively demonstrated a well fitting of Langmuir adsorption isotherm model. The higher removal percentage (86.0%) and higher slope value of Langmuir adsorption isotherm were estimated for endrin compared to dieldrin (74.0%). The reason for higher adsorption percentage of endrin is due to the endo-position of oxygen atom in molecule favors more interaction of molecules with GO-MNPs compared to the exo-position of oxygen present in dieldrin. In addition, the higher value of
R
2
for endrin and dieldrin demonstrated better suitability of pseudo-first-order and pseudo-second-order kinetic models, respectively. The advantages of the present method are use of simple UV-vis spectrophotometry for monitoring and low-cost use of GO-MNPs nanomaterial for the removal of pesticides from sample solution.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-017-0159-z</identifier><identifier>PMID: 28918582</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorption ; Agrochemicals ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Dieldrin ; Dieldrin - chemistry ; Earth and Environmental Science ; Ecotoxicology ; Endrin ; Endrin - chemistry ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Ferric Compounds - chemistry ; Graphene ; Graphite - chemistry ; Iron oxides ; Isotherms ; Kinetics ; Magnetics ; Magnetite Nanoparticles ; Nanocomposites ; Nanomaterials ; Nanoparticles ; Oxygen ; Pesticides ; pH effects ; Pollutant removal ; Research Article ; Spectrophotometry ; Waste Water Technology ; Water Management ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2017-11, Vol.24 (32), p.24980-24988</ispartof><rights>Springer-Verlag GmbH Germany 2017</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, (2017). All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c409t-8cb47da0d191073a5c2ec2aef3ca0ced2085aafdabb8fd6279f13b65389b6b503</citedby><cites>FETCH-LOGICAL-c409t-8cb47da0d191073a5c2ec2aef3ca0ced2085aafdabb8fd6279f13b65389b6b503</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-017-0159-z$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-017-0159-z$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/28918582$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Shrivas, Kamlesh</creatorcontrib><creatorcontrib>Ghosale, Archana</creatorcontrib><creatorcontrib>Nirmalkar, Nidhi</creatorcontrib><creatorcontrib>Srivastava, Arti</creatorcontrib><creatorcontrib>Singh, Sunil Kumar</creatorcontrib><creatorcontrib>Shinde, Sandip S.</creatorcontrib><title>Removal of endrin and dieldrin isomeric pesticides through stereoselective adsorption behavior on the graphene oxide-magnetic nanoparticles</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>A novel stereoselective removal behavior of isomeric endrin and dieldrin pesticides from sample solution is demonstrated using nanocomposite of graphene oxide (GO) and iron oxide (Fe
3
O
4
) magnetic nanoparticles (MNPs). The removal efficiency of endrin and dieldrin was found higher when GO-MNPs was used as a separating probe than the individual use of GO and MNPs. The removal efficiency of both the pesticides was found to be more favorable when the dosage amount of GO-MNPs was 30 mg for 30-min contact time with pH 4.0 at room temperature. The good correlation of determination (
R
2
) with 0.975 and 0.973 values obtained for endrin and dieldrin, respectively demonstrated a well fitting of Langmuir adsorption isotherm model. The higher removal percentage (86.0%) and higher slope value of Langmuir adsorption isotherm were estimated for endrin compared to dieldrin (74.0%). The reason for higher adsorption percentage of endrin is due to the endo-position of oxygen atom in molecule favors more interaction of molecules with GO-MNPs compared to the exo-position of oxygen present in dieldrin. In addition, the higher value of
R
2
for endrin and dieldrin demonstrated better suitability of pseudo-first-order and pseudo-second-order kinetic models, respectively. The advantages of the present method are use of simple UV-vis spectrophotometry for monitoring and low-cost use of GO-MNPs nanomaterial for the removal of pesticides from sample solution.</description><subject>Adsorption</subject><subject>Agrochemicals</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Dieldrin</subject><subject>Dieldrin - chemistry</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Endrin</subject><subject>Endrin - chemistry</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Ferric Compounds - chemistry</subject><subject>Graphene</subject><subject>Graphite - chemistry</subject><subject>Iron oxides</subject><subject>Isotherms</subject><subject>Kinetics</subject><subject>Magnetics</subject><subject>Magnetite Nanoparticles</subject><subject>Nanocomposites</subject><subject>Nanomaterials</subject><subject>Nanoparticles</subject><subject>Oxygen</subject><subject>Pesticides</subject><subject>pH effects</subject><subject>Pollutant removal</subject><subject>Research Article</subject><subject>Spectrophotometry</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>BENPR</sourceid><recordid>eNp1kc9KHTEUh4NU6q3tA3RTAt24GU0ymT9ZFqltQSiIXYczyZk7kZlkmsxcrK_gSxu9KqXQRcgJ-c53En6EfOTslDPWnCXOy6ouGG_yqlRxd0A2vOayaKRSb8iGKSkLXkp5RN6ldMOYYEo0b8mRaBVvq1ZsyP0VTmEHIw09RW-j8xS8pdbh-HRwKUwYnaEzpsUZZzHRZYhh3Q40LRgxJBzRLG6HFGwKcV5c8LTDAXYuRJrrZUC6jTAP6JGG26woJth6zDrqwYcZYi5HTO_JYQ9jwg_P-zH5dfH1-vx7cfnz24_zL5eFkUwtRWs62VhglivOmhIqI9AIwL40wAxawdoKoLfQdW1va9GonpddXZWt6uquYuUxOdl75xh-r_lfenLJ4DiCx7AmzZVkXNWylBn9_A96E9bo8-sy1dZ5lHwS8j1lYkgpYq_n6CaIfzRn-jEpvU9K56T0Y1L6Lvd8ejav3YT2teMlmgyIPZDyld9i_Gv0f60PSdajKw</recordid><startdate>20171101</startdate><enddate>20171101</enddate><creator>Shrivas, Kamlesh</creator><creator>Ghosale, Archana</creator><creator>Nirmalkar, Nidhi</creator><creator>Srivastava, Arti</creator><creator>Singh, Sunil Kumar</creator><creator>Shinde, Sandip S.</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QL</scope><scope>7SN</scope><scope>7T7</scope><scope>7TV</scope><scope>7U7</scope><scope>7WY</scope><scope>7WZ</scope><scope>7X7</scope><scope>7XB</scope><scope>87Z</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8FL</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BEZIV</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FRNLG</scope><scope>FYUFA</scope><scope>F~G</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K60</scope><scope>K6~</scope><scope>K9.</scope><scope>L.-</scope><scope>M0C</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7N</scope><scope>P64</scope><scope>PATMY</scope><scope>PQBIZ</scope><scope>PQBZA</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>7X8</scope></search><sort><creationdate>20171101</creationdate><title>Removal of endrin and dieldrin isomeric pesticides through stereoselective adsorption behavior on the graphene oxide-magnetic nanoparticles</title><author>Shrivas, Kamlesh ; Ghosale, Archana ; Nirmalkar, Nidhi ; Srivastava, Arti ; Singh, Sunil Kumar ; Shinde, Sandip S.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c409t-8cb47da0d191073a5c2ec2aef3ca0ced2085aafdabb8fd6279f13b65389b6b503</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><topic>Adsorption</topic><topic>Agrochemicals</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Dieldrin</topic><topic>Dieldrin - chemistry</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Endrin</topic><topic>Endrin - chemistry</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental science</topic><topic>Ferric Compounds - chemistry</topic><topic>Graphene</topic><topic>Graphite - chemistry</topic><topic>Iron oxides</topic><topic>Isotherms</topic><topic>Kinetics</topic><topic>Magnetics</topic><topic>Magnetite Nanoparticles</topic><topic>Nanocomposites</topic><topic>Nanomaterials</topic><topic>Nanoparticles</topic><topic>Oxygen</topic><topic>Pesticides</topic><topic>pH effects</topic><topic>Pollutant removal</topic><topic>Research Article</topic><topic>Spectrophotometry</topic><topic>Waste Water Technology</topic><topic>Water Management</topic><topic>Water Pollution Control</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Shrivas, Kamlesh</creatorcontrib><creatorcontrib>Ghosale, Archana</creatorcontrib><creatorcontrib>Nirmalkar, Nidhi</creatorcontrib><creatorcontrib>Srivastava, Arti</creatorcontrib><creatorcontrib>Singh, Sunil Kumar</creatorcontrib><creatorcontrib>Shinde, Sandip S.</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Bacteriology Abstracts (Microbiology B)</collection><collection>Ecology Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>ABI/INFORM Collection</collection><collection>ABI/INFORM Global (PDF only)</collection><collection>Health & Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>ABI/INFORM Global (Alumni Edition)</collection><collection>Medical Database (Alumni Edition)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest Pharma Collection</collection><collection>Public Health Database</collection><collection>Technology Research Database</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>ABI/INFORM Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest One Sustainability</collection><collection>ProQuest Central UK/Ireland</collection><collection>Agricultural & Environmental Science Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Business Premium Collection</collection><collection>Natural Science Collection</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>Engineering Research Database</collection><collection>Business Premium Collection (Alumni)</collection><collection>Health Research Premium Collection</collection><collection>ABI/INFORM Global (Corporate)</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Business Collection (Alumni Edition)</collection><collection>ProQuest Business Collection</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>ABI/INFORM Professional Advanced</collection><collection>ABI/INFORM Global</collection><collection>Health & Medical Collection (Alumni Edition)</collection><collection>Medical Database</collection><collection>Science Database</collection><collection>Algology Mycology and Protozoology Abstracts (Microbiology C)</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Environmental Science Database</collection><collection>One Business (ProQuest)</collection><collection>ProQuest One Business (Alumni)</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Environmental Science Collection</collection><collection>ProQuest Central Basic</collection><collection>MEDLINE - Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Shrivas, Kamlesh</au><au>Ghosale, Archana</au><au>Nirmalkar, Nidhi</au><au>Srivastava, Arti</au><au>Singh, Sunil Kumar</au><au>Shinde, Sandip S.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Removal of endrin and dieldrin isomeric pesticides through stereoselective adsorption behavior on the graphene oxide-magnetic nanoparticles</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2017-11-01</date><risdate>2017</risdate><volume>24</volume><issue>32</issue><spage>24980</spage><epage>24988</epage><pages>24980-24988</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>A novel stereoselective removal behavior of isomeric endrin and dieldrin pesticides from sample solution is demonstrated using nanocomposite of graphene oxide (GO) and iron oxide (Fe
3
O
4
) magnetic nanoparticles (MNPs). The removal efficiency of endrin and dieldrin was found higher when GO-MNPs was used as a separating probe than the individual use of GO and MNPs. The removal efficiency of both the pesticides was found to be more favorable when the dosage amount of GO-MNPs was 30 mg for 30-min contact time with pH 4.0 at room temperature. The good correlation of determination (
R
2
) with 0.975 and 0.973 values obtained for endrin and dieldrin, respectively demonstrated a well fitting of Langmuir adsorption isotherm model. The higher removal percentage (86.0%) and higher slope value of Langmuir adsorption isotherm were estimated for endrin compared to dieldrin (74.0%). The reason for higher adsorption percentage of endrin is due to the endo-position of oxygen atom in molecule favors more interaction of molecules with GO-MNPs compared to the exo-position of oxygen present in dieldrin. In addition, the higher value of
R
2
for endrin and dieldrin demonstrated better suitability of pseudo-first-order and pseudo-second-order kinetic models, respectively. The advantages of the present method are use of simple UV-vis spectrophotometry for monitoring and low-cost use of GO-MNPs nanomaterial for the removal of pesticides from sample solution.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>28918582</pmid><doi>10.1007/s11356-017-0159-z</doi><tpages>9</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0944-1344 |
| ispartof | Environmental science and pollution research international, 2017-11, Vol.24 (32), p.24980-24988 |
| issn | 0944-1344 1614-7499 |
| language | eng |
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| source | MEDLINE; SpringerLink Journals - AutoHoldings |
| subjects | Adsorption Agrochemicals Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Dieldrin Dieldrin - chemistry Earth and Environmental Science Ecotoxicology Endrin Endrin - chemistry Environment Environmental Chemistry Environmental Health Environmental science Ferric Compounds - chemistry Graphene Graphite - chemistry Iron oxides Isotherms Kinetics Magnetics Magnetite Nanoparticles Nanocomposites Nanomaterials Nanoparticles Oxygen Pesticides pH effects Pollutant removal Research Article Spectrophotometry Waste Water Technology Water Management Water Pollution Control |
| title | Removal of endrin and dieldrin isomeric pesticides through stereoselective adsorption behavior on the graphene oxide-magnetic nanoparticles |
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