Magnetic chitosan/anaerobic granular sludge composite: Synthesis, characterization and application in heavy metal ions removal
[Display omitted] In present study, magnetic anaerobic granule sludge/chitosan (M-CS-AnGS) composite was synthesized and applied to remove Pb(II) and Cu(II) from aqueous solution. The physicochemical properties of prepared M-CS-AnGS were characterized by using scanning electron microscopy (SEM), Fou...
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Veröffentlicht in: | Journal of colloid and interface science 2017-12, Vol.508, p.405-414 |
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container_title | Journal of colloid and interface science |
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creator | Liu, Ting Han, Xiao Wang, Yaoguang Yan, Liangguo Du, Bin Wei, Qin Wei, Dong |
description | [Display omitted]
In present study, magnetic anaerobic granule sludge/chitosan (M-CS-AnGS) composite was synthesized and applied to remove Pb(II) and Cu(II) from aqueous solution. The physicochemical properties of prepared M-CS-AnGS were characterized by using scanning electron microscopy (SEM), Fourier-transform infrared spectroscopy (FTIR), Zeta potential analysis and X-ray photoelectron spectroscopy (XPS). The factors affecting adsorption performance in view of different sorbents, adsorbent dosage, pH value and contact time were conducted to obtain optimum conditions of Pb(II) and Cu(II) onto M-CS-AnGS. The adsorption kinetics of Pb(II) and Cu(II) were better fitted with pseudo-second-order kinetic mode and Langmuir isotherm. The maximum adsorption capacities for Pb(II) and Cu(II) were 97.97 and 83.65mg/g, respectively. According to FTIR, Zeta potential and XPS analysis, it was found that the adsorption mechanisms Pb(II) and Cu(II) onto M-CS-AnGS were mainly caused by surface complexation and electrostatic attraction. In addition, M-CS-AnGS could be easily separated under an external magnetic field. The obtained result suggested that M-CS-AnGS composite could be used as a promising adsorbent for metal removal from aqueous solution. |
doi_str_mv | 10.1016/j.jcis.2017.08.067 |
format | Article |
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In present study, magnetic anaerobic granule sludge/chitosan (M-CS-AnGS) composite was synthesized and applied to remove Pb(II) and Cu(II) from aqueous solution. The physicochemical properties of prepared M-CS-AnGS were characterized by using scanning electron microscopy (SEM), Fourier-transform infrared spectroscopy (FTIR), Zeta potential analysis and X-ray photoelectron spectroscopy (XPS). The factors affecting adsorption performance in view of different sorbents, adsorbent dosage, pH value and contact time were conducted to obtain optimum conditions of Pb(II) and Cu(II) onto M-CS-AnGS. The adsorption kinetics of Pb(II) and Cu(II) were better fitted with pseudo-second-order kinetic mode and Langmuir isotherm. The maximum adsorption capacities for Pb(II) and Cu(II) were 97.97 and 83.65mg/g, respectively. According to FTIR, Zeta potential and XPS analysis, it was found that the adsorption mechanisms Pb(II) and Cu(II) onto M-CS-AnGS were mainly caused by surface complexation and electrostatic attraction. In addition, M-CS-AnGS could be easily separated under an external magnetic field. The obtained result suggested that M-CS-AnGS composite could be used as a promising adsorbent for metal removal from aqueous solution.</description><identifier>ISSN: 0021-9797</identifier><identifier>EISSN: 1095-7103</identifier><identifier>DOI: 10.1016/j.jcis.2017.08.067</identifier><identifier>PMID: 28858649</identifier><language>eng</language><publisher>United States: Elsevier Inc</publisher><subject>Anaerobic granular sludge ; Biosorption ; Chitosan ; Heavy metal ; Magnetic</subject><ispartof>Journal of colloid and interface science, 2017-12, Vol.508, p.405-414</ispartof><rights>2017 Elsevier Inc.</rights><rights>Copyright © 2017 Elsevier Inc. All rights reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c459t-24407649a0699e4ccd1a20b79541f0d35b5408da37f40056e5b7a47d6a86ce4c3</citedby><cites>FETCH-LOGICAL-c459t-24407649a0699e4ccd1a20b79541f0d35b5408da37f40056e5b7a47d6a86ce4c3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.jcis.2017.08.067$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/28858649$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Liu, Ting</creatorcontrib><creatorcontrib>Han, Xiao</creatorcontrib><creatorcontrib>Wang, Yaoguang</creatorcontrib><creatorcontrib>Yan, Liangguo</creatorcontrib><creatorcontrib>Du, Bin</creatorcontrib><creatorcontrib>Wei, Qin</creatorcontrib><creatorcontrib>Wei, Dong</creatorcontrib><title>Magnetic chitosan/anaerobic granular sludge composite: Synthesis, characterization and application in heavy metal ions removal</title><title>Journal of colloid and interface science</title><addtitle>J Colloid Interface Sci</addtitle><description>[Display omitted]
In present study, magnetic anaerobic granule sludge/chitosan (M-CS-AnGS) composite was synthesized and applied to remove Pb(II) and Cu(II) from aqueous solution. The physicochemical properties of prepared M-CS-AnGS were characterized by using scanning electron microscopy (SEM), Fourier-transform infrared spectroscopy (FTIR), Zeta potential analysis and X-ray photoelectron spectroscopy (XPS). The factors affecting adsorption performance in view of different sorbents, adsorbent dosage, pH value and contact time were conducted to obtain optimum conditions of Pb(II) and Cu(II) onto M-CS-AnGS. The adsorption kinetics of Pb(II) and Cu(II) were better fitted with pseudo-second-order kinetic mode and Langmuir isotherm. The maximum adsorption capacities for Pb(II) and Cu(II) were 97.97 and 83.65mg/g, respectively. According to FTIR, Zeta potential and XPS analysis, it was found that the adsorption mechanisms Pb(II) and Cu(II) onto M-CS-AnGS were mainly caused by surface complexation and electrostatic attraction. In addition, M-CS-AnGS could be easily separated under an external magnetic field. The obtained result suggested that M-CS-AnGS composite could be used as a promising adsorbent for metal removal from aqueous solution.</description><subject>Anaerobic granular sludge</subject><subject>Biosorption</subject><subject>Chitosan</subject><subject>Heavy metal</subject><subject>Magnetic</subject><issn>0021-9797</issn><issn>1095-7103</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><recordid>eNp9kE2P0zAQhi0EYsvCH-CAfORAsuPUjmPEZbXiS1rEAThbE2faukriYjuVyoHfjqsuHDlYlkfP-2r8MPZSQC1AtDf7eu98qhsQuoauhlY_YisBRlVawPoxWwE0ojLa6Cv2LKU9gBBKmafsquk61bXSrNjvL7idKXvH3c7nkHC-wRkphr6MthHnZcTI07gMW-IuTIeQfKa3_NtpzjtKPr0pQYzoMkX_C7MPM8d54Hg4jN5d3n7mO8LjiU-UceRllHikKRxxfM6ebHBM9OLhvmY_Prz_fvepuv_68fPd7X3lpDK5aqQEXfZFaI0h6dwgsIFeGyXFBoa16pWEbsC13kgA1ZLqNUo9tNi1rvDra_b60nuI4edCKdvJJ0fjiDOFJVlhJJRjdFvQ5oK6GFKKtLGH6CeMJyvAnr3bvT17t2fvFjpbvJfQq4f-pZ9o-Bf5K7oA7y4AlV8ePUWbnKfZ0eAjuWyH4P_X_wcoR5aZ</recordid><startdate>20171215</startdate><enddate>20171215</enddate><creator>Liu, Ting</creator><creator>Han, Xiao</creator><creator>Wang, Yaoguang</creator><creator>Yan, Liangguo</creator><creator>Du, Bin</creator><creator>Wei, Qin</creator><creator>Wei, Dong</creator><general>Elsevier Inc</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope></search><sort><creationdate>20171215</creationdate><title>Magnetic chitosan/anaerobic granular sludge composite: Synthesis, characterization and application in heavy metal ions removal</title><author>Liu, Ting ; Han, Xiao ; Wang, Yaoguang ; Yan, Liangguo ; Du, Bin ; Wei, Qin ; Wei, Dong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c459t-24407649a0699e4ccd1a20b79541f0d35b5408da37f40056e5b7a47d6a86ce4c3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><topic>Anaerobic granular sludge</topic><topic>Biosorption</topic><topic>Chitosan</topic><topic>Heavy metal</topic><topic>Magnetic</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Liu, Ting</creatorcontrib><creatorcontrib>Han, Xiao</creatorcontrib><creatorcontrib>Wang, Yaoguang</creatorcontrib><creatorcontrib>Yan, Liangguo</creatorcontrib><creatorcontrib>Du, Bin</creatorcontrib><creatorcontrib>Wei, Qin</creatorcontrib><creatorcontrib>Wei, Dong</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Journal of colloid and interface science</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Liu, Ting</au><au>Han, Xiao</au><au>Wang, Yaoguang</au><au>Yan, Liangguo</au><au>Du, Bin</au><au>Wei, Qin</au><au>Wei, Dong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Magnetic chitosan/anaerobic granular sludge composite: Synthesis, characterization and application in heavy metal ions removal</atitle><jtitle>Journal of colloid and interface science</jtitle><addtitle>J Colloid Interface Sci</addtitle><date>2017-12-15</date><risdate>2017</risdate><volume>508</volume><spage>405</spage><epage>414</epage><pages>405-414</pages><issn>0021-9797</issn><eissn>1095-7103</eissn><abstract>[Display omitted]
In present study, magnetic anaerobic granule sludge/chitosan (M-CS-AnGS) composite was synthesized and applied to remove Pb(II) and Cu(II) from aqueous solution. The physicochemical properties of prepared M-CS-AnGS were characterized by using scanning electron microscopy (SEM), Fourier-transform infrared spectroscopy (FTIR), Zeta potential analysis and X-ray photoelectron spectroscopy (XPS). The factors affecting adsorption performance in view of different sorbents, adsorbent dosage, pH value and contact time were conducted to obtain optimum conditions of Pb(II) and Cu(II) onto M-CS-AnGS. The adsorption kinetics of Pb(II) and Cu(II) were better fitted with pseudo-second-order kinetic mode and Langmuir isotherm. The maximum adsorption capacities for Pb(II) and Cu(II) were 97.97 and 83.65mg/g, respectively. According to FTIR, Zeta potential and XPS analysis, it was found that the adsorption mechanisms Pb(II) and Cu(II) onto M-CS-AnGS were mainly caused by surface complexation and electrostatic attraction. In addition, M-CS-AnGS could be easily separated under an external magnetic field. The obtained result suggested that M-CS-AnGS composite could be used as a promising adsorbent for metal removal from aqueous solution.</abstract><cop>United States</cop><pub>Elsevier Inc</pub><pmid>28858649</pmid><doi>10.1016/j.jcis.2017.08.067</doi><tpages>10</tpages></addata></record> |
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subjects | Anaerobic granular sludge Biosorption Chitosan Heavy metal Magnetic |
title | Magnetic chitosan/anaerobic granular sludge composite: Synthesis, characterization and application in heavy metal ions removal |
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