The woven fiber organic electrochemical transistors based on polypyrrole nanowires/reduced graphene oxide composites for glucose sensing

Novel woven fiber organic electrochemical transistors based on polypyrrole (PPy) nanowires and reduced graphene oxide (rGO) have been prepared. SEM revealed that the introduction of rGO nanosheets could induce the growth and increase the amount of PPy nanowires. Moreover, it could enhance the electr...

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Veröffentlicht in:Biosensors & bioelectronics 2017-09, Vol.95, p.138-145
Hauptverfasser: Wang, Yuedan, Qing, Xing, Zhou, Quan, Zhang, Yang, Liu, Qiongzhen, Liu, Ke, Wang, Wenwen, Li, Mufang, Lu, Zhentan, Chen, Yuanli, Wang, Dong
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container_start_page 138
container_title Biosensors & bioelectronics
container_volume 95
creator Wang, Yuedan
Qing, Xing
Zhou, Quan
Zhang, Yang
Liu, Qiongzhen
Liu, Ke
Wang, Wenwen
Li, Mufang
Lu, Zhentan
Chen, Yuanli
Wang, Dong
description Novel woven fiber organic electrochemical transistors based on polypyrrole (PPy) nanowires and reduced graphene oxide (rGO) have been prepared. SEM revealed that the introduction of rGO nanosheets could induce the growth and increase the amount of PPy nanowires. Moreover, it could enhance the electrical performance of fiber transistors. The hybrid transistors showed high on/off ratio of 102, fast switch speed, and long cycling stability. The glucose sensors based on the fiber organic electrochemical transistors have also been investigated, which exhibited outstanding sensitivity, as high as 0.773 NCR/decade, with a response time as fast as 0.5s, a linear range of 1nM to 5μM, a low detection concentration as well as good repeatability. In addition, the glucose could be selectively detected in the presence of ascorbic acid and uric acid interferences. The reliability of the proposed glucose sensor was evaluated in real samples of rabbit blood. All the results indicate that the novel fiber transistors pave the way for portable and wearable electronics devices, which have a promising future for healthcare and biological applications. •Novel woven fiber electrochemical transistors based on polypyrrole nanowires and rGO were prepared.•rGO could induce the growth and increase the amount of polypyrrole nanowires.•The fiber electrochemical transistors show good performance with on/off of 102, fast response, and stability.•High sensitivity, outstanding selectivity, and reproducibility were achieved by the glucose sensor.•The sensors have been successfully applied for determination of glucose in rabbit blood serum.
doi_str_mv 10.1016/j.bios.2017.04.018
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SEM revealed that the introduction of rGO nanosheets could induce the growth and increase the amount of PPy nanowires. Moreover, it could enhance the electrical performance of fiber transistors. The hybrid transistors showed high on/off ratio of 102, fast switch speed, and long cycling stability. The glucose sensors based on the fiber organic electrochemical transistors have also been investigated, which exhibited outstanding sensitivity, as high as 0.773 NCR/decade, with a response time as fast as 0.5s, a linear range of 1nM to 5μM, a low detection concentration as well as good repeatability. In addition, the glucose could be selectively detected in the presence of ascorbic acid and uric acid interferences. The reliability of the proposed glucose sensor was evaluated in real samples of rabbit blood. All the results indicate that the novel fiber transistors pave the way for portable and wearable electronics devices, which have a promising future for healthcare and biological applications. •Novel woven fiber electrochemical transistors based on polypyrrole nanowires and rGO were prepared.•rGO could induce the growth and increase the amount of polypyrrole nanowires.•The fiber electrochemical transistors show good performance with on/off of 102, fast response, and stability.•High sensitivity, outstanding selectivity, and reproducibility were achieved by the glucose sensor.•The sensors have been successfully applied for determination of glucose in rabbit blood serum.</description><identifier>ISSN: 0956-5663</identifier><identifier>EISSN: 1873-4235</identifier><identifier>DOI: 10.1016/j.bios.2017.04.018</identifier><identifier>PMID: 28437640</identifier><language>eng</language><publisher>England: Elsevier B.V</publisher><subject>Animals ; Biosensing Techniques ; Electrochemical Techniques ; Fiber ; Glucose - chemistry ; Glucose - isolation &amp; purification ; Glucose sensor ; Graphite - chemistry ; Nanowires - chemistry ; Organic electrochemical transistors ; Polymers - chemistry ; Polypyrrole nanowires ; Pyrroles - chemistry ; Rabbits ; Reduced graphene oxide</subject><ispartof>Biosensors &amp; bioelectronics, 2017-09, Vol.95, p.138-145</ispartof><rights>2017 Elsevier B.V.</rights><rights>Copyright © 2017 Elsevier B.V. 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SEM revealed that the introduction of rGO nanosheets could induce the growth and increase the amount of PPy nanowires. Moreover, it could enhance the electrical performance of fiber transistors. The hybrid transistors showed high on/off ratio of 102, fast switch speed, and long cycling stability. The glucose sensors based on the fiber organic electrochemical transistors have also been investigated, which exhibited outstanding sensitivity, as high as 0.773 NCR/decade, with a response time as fast as 0.5s, a linear range of 1nM to 5μM, a low detection concentration as well as good repeatability. In addition, the glucose could be selectively detected in the presence of ascorbic acid and uric acid interferences. The reliability of the proposed glucose sensor was evaluated in real samples of rabbit blood. 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subjects Animals
Biosensing Techniques
Electrochemical Techniques
Fiber
Glucose - chemistry
Glucose - isolation & purification
Glucose sensor
Graphite - chemistry
Nanowires - chemistry
Organic electrochemical transistors
Polymers - chemistry
Polypyrrole nanowires
Pyrroles - chemistry
Rabbits
Reduced graphene oxide
title The woven fiber organic electrochemical transistors based on polypyrrole nanowires/reduced graphene oxide composites for glucose sensing
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