Efficiency of Cathodoluminescence Emission by Nitrogen‐Vacancy Color Centers in Nanodiamonds
Correlated electron microscopy and cathodoluminescence (CL) imaging using functionalized nanoparticles is a promising nanoscale probe of biological structure and function. Nanodiamonds (NDs) that contain CL‐emitting color centers are particularly well suited for such applications. The intensity of C...
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| Veröffentlicht in: | Small (Weinheim an der Bergstrasse, Germany) Germany), 2017-06, Vol.13 (22), p.1700543-n/a |
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| creator | Zhang, Huiliang Glenn, David R. Schalek, Richard Lichtman, Jeff W. Walsworth, Ronald L. |
| description | Correlated electron microscopy and cathodoluminescence (CL) imaging using functionalized nanoparticles is a promising nanoscale probe of biological structure and function. Nanodiamonds (NDs) that contain CL‐emitting color centers are particularly well suited for such applications. The intensity of CL emission from NDs is determined by a combination of factors, including particle size, density of color centers, efficiency of energy deposition by electrons passing through the particle, and conversion efficiency from deposited energy to CL emission. This paper reports experiments and numerical simulations that investigate the relative importance of each of these factors in determining CL emission intensity from NDs containing nitrogen‐vacancy (NV) color centers. In particular, it is found that CL can be detected from NV‐doped NDs with dimensions as small as ≈40 nm, although CL emission decreases significantly for smaller NDs.
The cathodoluminescence (CL) emission properties of nanodiamonds containing nitrogen‐vacancy centers are investigated. Coregistered images of nanodiamonds obtained by secondary electron imaging, atomic force microscopy, photoluminescence, and cathodoluminescence, enable precise characterization of CL intensity as a function of nanodiamond size and doping concentration, for applications in correlative microscopy. |
| doi_str_mv | 10.1002/smll.201700543 |
| format | Article |
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The cathodoluminescence (CL) emission properties of nanodiamonds containing nitrogen‐vacancy centers are investigated. Coregistered images of nanodiamonds obtained by secondary electron imaging, atomic force microscopy, photoluminescence, and cathodoluminescence, enable precise characterization of CL intensity as a function of nanodiamond size and doping concentration, for applications in correlative microscopy.</description><identifier>ISSN: 1613-6810</identifier><identifier>EISSN: 1613-6829</identifier><identifier>DOI: 10.1002/smll.201700543</identifier><identifier>PMID: 28417543</identifier><language>eng</language><publisher>Germany: Wiley Subscription Services, Inc</publisher><subject>Cathodoluminescence ; Color centers ; Computer simulation ; Correlation ; correlative microscopy ; Density ; Deposition ; Diamonds ; Direct power generation ; Efficiency ; Electron microscopy ; Emission analysis ; Energy conversion efficiency ; Energy management ; Imaging ; Mathematical models ; nanodiamond ; Nanoparticles ; Nanotechnology ; Nitrogen ; nitrogen‐vacancy ; Particle size ; Quartz ; scanning electron microscopy ; Vacancies</subject><ispartof>Small (Weinheim an der Bergstrasse, Germany), 2017-06, Vol.13 (22), p.1700543-n/a</ispartof><rights>2017 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim</rights><rights>2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.</rights><rights>2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c4793-bf12294b6d28c6576f40a60f591a7db08e049978d579c2b16625313074d49c413</citedby><cites>FETCH-LOGICAL-c4793-bf12294b6d28c6576f40a60f591a7db08e049978d579c2b16625313074d49c413</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fsmll.201700543$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fsmll.201700543$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>315,781,785,1418,27929,27930,45579,45580</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/28417543$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhang, Huiliang</creatorcontrib><creatorcontrib>Glenn, David R.</creatorcontrib><creatorcontrib>Schalek, Richard</creatorcontrib><creatorcontrib>Lichtman, Jeff W.</creatorcontrib><creatorcontrib>Walsworth, Ronald L.</creatorcontrib><title>Efficiency of Cathodoluminescence Emission by Nitrogen‐Vacancy Color Centers in Nanodiamonds</title><title>Small (Weinheim an der Bergstrasse, Germany)</title><addtitle>Small</addtitle><description>Correlated electron microscopy and cathodoluminescence (CL) imaging using functionalized nanoparticles is a promising nanoscale probe of biological structure and function. Nanodiamonds (NDs) that contain CL‐emitting color centers are particularly well suited for such applications. The intensity of CL emission from NDs is determined by a combination of factors, including particle size, density of color centers, efficiency of energy deposition by electrons passing through the particle, and conversion efficiency from deposited energy to CL emission. This paper reports experiments and numerical simulations that investigate the relative importance of each of these factors in determining CL emission intensity from NDs containing nitrogen‐vacancy (NV) color centers. In particular, it is found that CL can be detected from NV‐doped NDs with dimensions as small as ≈40 nm, although CL emission decreases significantly for smaller NDs.
The cathodoluminescence (CL) emission properties of nanodiamonds containing nitrogen‐vacancy centers are investigated. Coregistered images of nanodiamonds obtained by secondary electron imaging, atomic force microscopy, photoluminescence, and cathodoluminescence, enable precise characterization of CL intensity as a function of nanodiamond size and doping concentration, for applications in correlative microscopy.</description><subject>Cathodoluminescence</subject><subject>Color centers</subject><subject>Computer simulation</subject><subject>Correlation</subject><subject>correlative microscopy</subject><subject>Density</subject><subject>Deposition</subject><subject>Diamonds</subject><subject>Direct power generation</subject><subject>Efficiency</subject><subject>Electron microscopy</subject><subject>Emission analysis</subject><subject>Energy conversion efficiency</subject><subject>Energy management</subject><subject>Imaging</subject><subject>Mathematical models</subject><subject>nanodiamond</subject><subject>Nanoparticles</subject><subject>Nanotechnology</subject><subject>Nitrogen</subject><subject>nitrogen‐vacancy</subject><subject>Particle size</subject><subject>Quartz</subject><subject>scanning electron microscopy</subject><subject>Vacancies</subject><issn>1613-6810</issn><issn>1613-6829</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2017</creationdate><recordtype>article</recordtype><recordid>eNqFkLtOwzAUhi0EolBYGVEkFpYWH8ex4xFF5SIVGLiMWI7jgKvEBrsR6sYj8Iw8CakKRWJhOkdH3__r6EPoAPAYMCYnsW2aMcHAMc5ouoF2gEE6YjkRm-sd8ADtxjjDOAVC-TYakJwC7_kd9Dipa6utcXqR-Dop1PzZV77pWutM1P3ZJJPWxmi9S8pFcm3nwT8Z9_n-8aC0WqYK3_iQFMbNTYiJdcm1cr6yqvWuintoq1ZNNPvfc4juzyZ3xcVoenN-WZxOR5pykY7KGggRtGQVyTXLOKspVgzXmQDFqxLnBlMheF5lXGhSAmMkSyHFnFZUaArpEB2vel-Cf-1MnMv-aW2aRjnjuyghz0WaA-sVDNHRH3Tmu-D67yQIzBjjhGc9NV5ROvgYg6nlS7CtCgsJWC7Ny6V5uTbfBw6_a7uyNdUa_1HdA2IFvNnGLP6pk7dX0-lv-RduBo-X</recordid><startdate>201706</startdate><enddate>201706</enddate><creator>Zhang, Huiliang</creator><creator>Glenn, David R.</creator><creator>Schalek, Richard</creator><creator>Lichtman, Jeff W.</creator><creator>Walsworth, Ronald L.</creator><general>Wiley Subscription Services, Inc</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope></search><sort><creationdate>201706</creationdate><title>Efficiency of Cathodoluminescence Emission by Nitrogen‐Vacancy Color Centers in Nanodiamonds</title><author>Zhang, Huiliang ; Glenn, David R. ; Schalek, Richard ; Lichtman, Jeff W. ; Walsworth, Ronald L.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c4793-bf12294b6d28c6576f40a60f591a7db08e049978d579c2b16625313074d49c413</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2017</creationdate><topic>Cathodoluminescence</topic><topic>Color centers</topic><topic>Computer simulation</topic><topic>Correlation</topic><topic>correlative microscopy</topic><topic>Density</topic><topic>Deposition</topic><topic>Diamonds</topic><topic>Direct power generation</topic><topic>Efficiency</topic><topic>Electron microscopy</topic><topic>Emission analysis</topic><topic>Energy conversion efficiency</topic><topic>Energy management</topic><topic>Imaging</topic><topic>Mathematical models</topic><topic>nanodiamond</topic><topic>Nanoparticles</topic><topic>Nanotechnology</topic><topic>Nitrogen</topic><topic>nitrogen‐vacancy</topic><topic>Particle size</topic><topic>Quartz</topic><topic>scanning electron microscopy</topic><topic>Vacancies</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Huiliang</creatorcontrib><creatorcontrib>Glenn, David R.</creatorcontrib><creatorcontrib>Schalek, Richard</creatorcontrib><creatorcontrib>Lichtman, Jeff W.</creatorcontrib><creatorcontrib>Walsworth, Ronald L.</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Small (Weinheim an der Bergstrasse, Germany)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhang, Huiliang</au><au>Glenn, David R.</au><au>Schalek, Richard</au><au>Lichtman, Jeff W.</au><au>Walsworth, Ronald L.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Efficiency of Cathodoluminescence Emission by Nitrogen‐Vacancy Color Centers in Nanodiamonds</atitle><jtitle>Small (Weinheim an der Bergstrasse, Germany)</jtitle><addtitle>Small</addtitle><date>2017-06</date><risdate>2017</risdate><volume>13</volume><issue>22</issue><spage>1700543</spage><epage>n/a</epage><pages>1700543-n/a</pages><issn>1613-6810</issn><eissn>1613-6829</eissn><abstract>Correlated electron microscopy and cathodoluminescence (CL) imaging using functionalized nanoparticles is a promising nanoscale probe of biological structure and function. Nanodiamonds (NDs) that contain CL‐emitting color centers are particularly well suited for such applications. The intensity of CL emission from NDs is determined by a combination of factors, including particle size, density of color centers, efficiency of energy deposition by electrons passing through the particle, and conversion efficiency from deposited energy to CL emission. This paper reports experiments and numerical simulations that investigate the relative importance of each of these factors in determining CL emission intensity from NDs containing nitrogen‐vacancy (NV) color centers. In particular, it is found that CL can be detected from NV‐doped NDs with dimensions as small as ≈40 nm, although CL emission decreases significantly for smaller NDs.
The cathodoluminescence (CL) emission properties of nanodiamonds containing nitrogen‐vacancy centers are investigated. Coregistered images of nanodiamonds obtained by secondary electron imaging, atomic force microscopy, photoluminescence, and cathodoluminescence, enable precise characterization of CL intensity as a function of nanodiamond size and doping concentration, for applications in correlative microscopy.</abstract><cop>Germany</cop><pub>Wiley Subscription Services, Inc</pub><pmid>28417543</pmid><doi>10.1002/smll.201700543</doi><tpages>9</tpages><oa>free_for_read</oa></addata></record> |
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| source | Wiley Online Library - AutoHoldings Journals |
| subjects | Cathodoluminescence Color centers Computer simulation Correlation correlative microscopy Density Deposition Diamonds Direct power generation Efficiency Electron microscopy Emission analysis Energy conversion efficiency Energy management Imaging Mathematical models nanodiamond Nanoparticles Nanotechnology Nitrogen nitrogen‐vacancy Particle size Quartz scanning electron microscopy Vacancies |
| title | Efficiency of Cathodoluminescence Emission by Nitrogen‐Vacancy Color Centers in Nanodiamonds |
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