Photoelectron spin polarization in the Bi sub(2) Te sub(3)(0001) topological insulator: Initial- and final-state effects in the photoemission process
The photoelectron spin polarization in angle-resolved photoemission from the topological surface state in Bi sub(2) Te sub(3)(0001) has been investigated in a combined experimental and theoretical study. Our measurements show significant photon-energy-dependent deviations in the three-dimensional sp...
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Veröffentlicht in: | Physical review. B 2016-06, Vol.93 (24) |
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creator | Seibel, Christoph Braun, Jurgen Maass, Henriette Bentmann, Hendrik Minar, Jan Kuznetsova, Tatyana V Kokh, Konstantin A Tereshchenko, Oleg E Okuda, Taichi Ebert, Hubert Reinert, Friedrich |
description | The photoelectron spin polarization in angle-resolved photoemission from the topological surface state in Bi sub(2) Te sub(3)(0001) has been investigated in a combined experimental and theoretical study. Our measurements show significant photon-energy-dependent deviations in the three-dimensional spin polarization of the photoelectron when compared to the expected intrinsic spin polarization of the surface state. The experimental observations are in line with relativistic one-step photoemission calculations. Our theoretical analysis confirms that spin-orbit coupling in the initial-state wave functions in combination with the dipole selection rules strongly influences the photoelectron spin polarization. Furthermore, spin-dependent final-state effects are found to influence the spin polarization significantly. A quantitative access to the three-dimensional spin-polarization vector in topological insulators is thus challenged by a complex interplay of initial- and final-state effects in the photoemission process. |
doi_str_mv | 10.1103/PhysRevB.93.245150 |
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Our measurements show significant photon-energy-dependent deviations in the three-dimensional spin polarization of the photoelectron when compared to the expected intrinsic spin polarization of the surface state. The experimental observations are in line with relativistic one-step photoemission calculations. Our theoretical analysis confirms that spin-orbit coupling in the initial-state wave functions in combination with the dipole selection rules strongly influences the photoelectron spin polarization. Furthermore, spin-dependent final-state effects are found to influence the spin polarization significantly. A quantitative access to the three-dimensional spin-polarization vector in topological insulators is thus challenged by a complex interplay of initial- and final-state effects in the photoemission process.</description><identifier>ISSN: 2469-9950</identifier><identifier>EISSN: 2469-9969</identifier><identifier>DOI: 10.1103/PhysRevB.93.245150</identifier><language>eng</language><subject>Condensed matter ; Deviation ; Insulators ; Mathematical analysis ; Photoelectrons ; Photoemission ; Polarization ; Topology</subject><ispartof>Physical review. 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B</jtitle><date>2016-06-15</date><risdate>2016</risdate><volume>93</volume><issue>24</issue><issn>2469-9950</issn><eissn>2469-9969</eissn><abstract>The photoelectron spin polarization in angle-resolved photoemission from the topological surface state in Bi sub(2) Te sub(3)(0001) has been investigated in a combined experimental and theoretical study. Our measurements show significant photon-energy-dependent deviations in the three-dimensional spin polarization of the photoelectron when compared to the expected intrinsic spin polarization of the surface state. The experimental observations are in line with relativistic one-step photoemission calculations. Our theoretical analysis confirms that spin-orbit coupling in the initial-state wave functions in combination with the dipole selection rules strongly influences the photoelectron spin polarization. Furthermore, spin-dependent final-state effects are found to influence the spin polarization significantly. 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subjects | Condensed matter Deviation Insulators Mathematical analysis Photoelectrons Photoemission Polarization Topology |
title | Photoelectron spin polarization in the Bi sub(2) Te sub(3)(0001) topological insulator: Initial- and final-state effects in the photoemission process |
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